Many quantum mechanical systems require large (potentially infinite) numbers of variables to exactly describe their state. In this thesis, I examine two approaches to develop simple, approximate models for such systems, which capture their essential dynamics. I use two bistable regimes of the Jaynes-Cummings model of cavity quantum electrodynamics as example systems to evaluate the effectiveness of each approach. In the phase bistable regime (which occurs with large driving field, and which I study in an on-resonance "bad cavity" regime to make numerical simulations tractable), the cavity field switches between two states with identical amplitude but opposite phase. In the absorptive bistable regime (which I study with small driving field in an on-resonance "good cavity"'), two stable regions of state space differ in cavity field amplitude as well as their shape and qualitative behavior. After introducing these two regimes and their dynamics, I give a short introduction to projecting dynamical equations onto linear subspaces. Proper Orthogonal Decomposition (POD) allows the algorithmic construction of subspaces onto which the dynamics may be projected. I demonstrate that the application of POD to phase bistability results in effective approximate filters, while the asymmetry of the absorptive bistable case requires extensions to POD, developed in this thesis, to create a functional filter. Local Tangent Space Alignment is one of a class of unsupervised manifold learning algorithms which use the local geometry of high-dimensional data, such as quantum trajectories, to calculate the coordinates of that data on a low-dimensional manifold. I show how this algorithm functions, and characterize the manifolds that result from phase and absorptive bistability. I fit the 3-dimensional phase bistable manifold with a small set of system observables, and create a three-dimensional set of equations (similar to the semi-classical Maxwell-Bloch equations) which perform very well as a filter. Absorptive bistability again proves to be more complicated, but I am able to show that the underlying manifold is small, and make some progress on characterizing its relations with system observables.
Many quantum mechanical systems require large (potentially infinite) numbers of variables to exactly describe their state. In this thesis, I examine two approaches to develop simple, approximate models for such systems, which capture their essential dynamics. I use two bistable regimes of the Jaynes-Cummings model of cavity quantum electrodynamics as example systems to evaluate the effectiveness of each approach. In the phase bistable regime (which occurs with large driving field, and which I study in an on-resonance "bad cavity" regime to make numerical simulations tractable), the cavity field switches between two states with identical amplitude but opposite phase. In the absorptive bistable regime (which I study with small driving field in an on-resonance "good cavity"'), two stable regions of state space differ in cavity field amplitude as well as their shape and qualitative behavior. After introducing these two regimes and their dynamics, I give a short introduction to projecting dynamical equations onto linear subspaces. Proper Orthogonal Decomposition (POD) allows the algorithmic construction of subspaces onto which the dynamics may be projected. I demonstrate that the application of POD to phase bistability results in effective approximate filters, while the asymmetry of the absorptive bistable case requires extensions to POD, developed in this thesis, to create a functional filter. Local Tangent Space Alignment is one of a class of unsupervised manifold learning algorithms which use the local geometry of high-dimensional data, such as quantum trajectories, to calculate the coordinates of that data on a low-dimensional manifold. I show how this algorithm functions, and characterize the manifolds that result from phase and absorptive bistability. I fit the 3-dimensional phase bistable manifold with a small set of system observables, and create a three-dimensional set of equations (similar to the semi-classical Maxwell-Bloch equations) which perform very well as a filter. Absorptive bistability again proves to be more complicated, but I am able to show that the underlying manifold is small, and make some progress on characterizing its relations with system observables.
A simple algebraic procedure is described for deriving Maxwell-Bloch-type equations from single-atom cavity quantum electrodynamics (cavity QED) master equations via orthogonal projection onto a manifold of semiclassical states. In particular, the usual Maxwell-Bloch equations are obtained---up to a state-dependent correction factor of order unity---straightforwardly from the unconditional Jaynes-Cummings master equation. The technique of projecting onto a semiclassical manifold can also be applied with conditional master equations (quantum filters), leading to stochastic simulation models that include multiplicative noise terms associated with fluctuations of the atomic dipole. The utility of such models is briefly explored in the context of single-atom absorptive bistability.
Open quantum systems have drawn attention over decades due to its applicability in the foundation of theoretical physics, e.g. statistical mechanics, quantum mechanics and condensed matter physics. The dynamics of open quantum systems has been described as separate entities from their surrounding environment that consists of a very large number of modes, somehow coupled to the mode of the system. Even though the exact solution of the dynamical behavior of the system is impossible to calculate, we obtain a tentative solution using the crucial Markov approximation. The input-output formalism of the quantum Langevin equation (QLE) has been considered as a useful tool which provides a semi-classical description of the dynamics of the system, whereas the master equation provides a complete picture of the dynamics of the system expressed in terms of density matrix. While studying the dynamics of nonlinear system/environment coupling using QLE, we see, for a small value of external field, that the steady state system field does not change much from the steady state field obtained in the absence of nonlinear dissipation. However, in a case where a stronger external field is applied, we see that the deviation becomes substantial from the solution of linear system. We also see that the nonlinear coupling introduces significant difference in the cavity fluctuation spectrum. The description, therefore, provides a potential explanation of parametric effects in terms of nonlinear dissipation phenomena associated with the nonlinear coupling. Even though the theories developed in the context of open quantum systems have proven to be powerful tools, they do not provide a satisfactory platform to be implemented on non-linear Hamiltonians. We often approximate it by linearizing over nonlinear steady state field amplitude, and therefore, the interesting effects are often overlooked. The limitation of the analytics provokes us to simulate open quantum dynamics numerically. The numerical method consists of transformation of the environmental degrees of freedom to a one-dimensional many-body chain, and the computational technique includes numerical diagonalization and renormalization process. The time-adaptive density matrix renormalisation group (t-DMRG) is known as one of the most powerful techniques for the simulation of strongly-correlated many-body quantum systems. In this thesis, along with the theoretical modeling, we implement DMRG numerical scheme for the simulation of canonical S/B model by mapping it to one-dimensional harmonic chain with nearest neighbor interactions, and use the method to investigate the dynamics of the free dissipative system. The thermalization of open quantum systems is also studied by generating minimally entangled typical thermal states (METTS) through imaginary time evolution, and real-time evolving an empty system in the presence of the thermal bath. Further, we simulate coherently driven free dissipative Kerr nonlinear system numerically using Euler's method by solving Heisenberg equation of motion and t-DMRG algorithm, and demonstrate how the numerical results are analogous to classical bistability. By comparing with analytics, we see that the DMRG numerics is analogous to the quantum-mechanical exact solution obtained by mapping the equation of motion of the density matrix of the system to a Fokker-Plank equation. The comparison between two different numerical techniques shows that the semi-classical Euler's method determines the dynamics of the system field of one among two coherent branches, whereas DMRG numerics gives the superposition of both of them. Hence, DMRG-determined time dynamics undergoes generating non-classical states. Our approach of dealing with nonlinearity represents an important contribution in the developments of technique to study the dynamical and steady-state behavior of open quantum systems, which is a fundamental aspect of quantum physics.
Due to the improvement within cavity quantum electrodynamics experiments during the last decades, what was former seen as 'toy models' are today realized in laboratories. A controlled isolated coherent evolution of one or a few atoms coupled to a single mode inside a cavity is achievable. Such systems are well suited for studying purely quantum mechanical effects, and also for performing quantum gates, necessary for quantum computing. The Jaynes-Cummings model has served as a theoretical description of the interaction. However, as the experimental techniques are improved, for example, atom cooling, the use of multi-level atoms or multi-modes and driving of atoms or elds by external lasers, extensions of the original Jaynes-Cummings model are needed. In this thesis we study some of these extended models, and in particular multi-level models, time-dependent models and quantized motion models. Both analytical and numerical analysis are considered. The two-level structure of the Jaynes-Cummings model leads to applications of known solvable time-dependent two-level Schrödinger equations. In other cases, di erent forms of adiabatic approximate solutions are used, and with the analytically solvable models, the amplitudes of non-adiabatic contributions may be estimated. For higher dimensional systems, STIRAP and multi-STIRAP methods are applied. It is shown how the time-dependent models may be used for preparation of various kinds of non-classical states, and also to generate universal sets of quantum gates, both on atomic and eld qubits. When the atoms are cooled to very low temperatures, their velocities must be treated quantum mechanically, and we have studied the dynamics of such cases for di erent coupling shapes. Again numerical and analytical approaches have been used and compared, wave-packet propagations of the atom, approaching and traversing the cavity, have been performed. For periodic couplings, standing wave cavity modes, the dynamics has been described by e ective parameters; group velocity or atomic index of refraction and effective mass. Tunneling resonances for ultra cold atoms have been exhibited in the STIRAP models for certain initial conditions.
We derive simple models for the dynamics of a single atom coupled to a cavity field mode in the absorptive bistable parameter regime by projecting the time evolution of the state of the system onto a suitably chosen nonlinear low-dimensional manifold, which is found by use of local tangent space alignment. The output field from the cavity is detected with a homodyne detector allowing observation of quantum jumps of the system between states with different average numbers of photons in the cavity. We find that the models, which are significantly faster to integrate numerically than the full stochastic master equation, largely reproduce the dynamics of the system, and we demonstrate that they are sufficiently accurate to facilitate feedback control of the state of the system based on the predictions of the models alone.
The object of this PhD Thesis is light and matter quantum interaction including studies on cavity and circuit quantum electrodynamics (CQED and cQED), quantum information theory and entanglement dynamics in open systems. In recent years both theoretical and experimental efforts have been devoted to study problems regarding the transfer of quantum correlations, quantum memories, entanglement protection against decoherence and new regimes accessible in cQED. One of the fundamental model underlying these topics is the well known Jaynes-Cummings (JC) one for light-matter interaction, introduced in quantum optics already in 1963. This paradigmatic model describes the coherent exchange of a single excitation between a qubit (a two-level system) and a mode of a quantized harmonic oscillator. The JC model describes a lot of purely quantum effects such as Rabi oscillations and generation of entangled quantum states, which were confirmed by several sophisticated experiments in CQED. This model has been then applied in many other frameworks. Analytical results can be derived only under the so-called rotating wave approximation (RWA), which allows to neglect the energy contributions coming from the counter-rotating terms, which describe the simultaneous excitation (or de-excitation) of the qubit and the field mode. In this Thesis a first interesting investigation, based on the JC model, is related to the realization of quantum memories. The main aspect is the transfer of generic quantum entangled states of a propagating radiation to some qubits, such as two-level atoms placed in separated optical cavities. Generalizing previous results for bipartite entangled systems, I investigated the more complex case of tripartite systems, where the very quantification of entanglement is still an open problem. This issue is broadened to open systems in contact with a common environment which induces decoherence effects unavoidable in realistic implementations. The main result of this analysis is that it is possible to map in an optimal way a quantum state from radiation to qubits in the unitary dynamics, and even in the presence of a dissipative environment a significative amount of entanglement can be transferred. This study has been carried on with either theoretical calculations or numerical simulations performed adopting the powerful Monte Carlo wave function method. A second important problem for quantum memories faced in this PhD Thesis, regards the protection of qubits entanglement for long enough times in order to implement quantum information tasks. A possible way to obtain this goal is to add an external coherent field driving two or more two-level atoms interacting with a common mode of a cavity electromagnetic field. In fact it is possible to demonstrate that, under certain conditions, an effective Hamiltonian of the whole system involves, together with the familiar JC terms, also the counter-rotating ones. The main feature that comes out from this analysis is the possibility to freeze, during system dynamics, peculiar quantum entangled states of the atomic qubits in so called decoherence-free subspaces. This important property allows to store the entanglement in matter qubits, isolating the quantum state from environment induced decoherence. Though the system includes dissipation, analytical results have been obtained for multipartite entanglement and decoherence by solving the master equation through a projection on a suitable basis and using the method of characteristics. In particular it is possible to monitor the rate of decoherence via measurements of joint atomic probabilities, shading light on the fascinating border between the quantum and the classical world. A last topic investigated in this Thesis concerns the recently developed and quite promising implementation of the JC model well outside CQED, that is cQED. Here superconductive circuits, which play the role of artificial atoms, interact on-chip with transmission line resonators, instead of the usual electromagnetic cavities. These systems have the advantage of being quite easily engineered exploiting the most advanced available technologies. Moreover they allow a great flexibility in handling the relevant parameters, since the inter-system coupling is here of capacitive or inductive nature, instead of the usual electric dipole interaction in CQED. In this way a strong and ultrastrong coupling regime have become available, giving a direct access to the physics beyond the JC model and its possible applications. I first performed a detailed characterization of system dynamics in order to test the main approximations usually introduced to describe superconductive circuits as qubits. Then I described, both analytically and numerically, the dissipative dynamics of a superconductive qubit coupled to a resonator mode in the deep strong regime.
The topic of this thesis is a theoretical study of nonequilibrium transitions and quantum statistical properties of nonlinear quantum optical systems driven by an external radiation source. In certain limiting cases, a comparison is made between these transitions and the phase transitions found in equilibrium physical systems. In chapters one and two, the mathematical tools are introduced. In operator terms, the time development is described by a Markovian master equation in the interaction picture. This is equivalent to a corresponding time development equation or Fokker-Planck equation in a vector space of c-numbers. In order to deal with the type of Fokker-Planck equation that results, we introduce a quantum classical correspondence resulting in a distribution function over a complex phase-space, which is a generalisation of the Glauber-Sudarshan P-function. In chapter three this is applied to a model of a coherently driven mode with nonlinear dispersion and absorption. We find in the limit of zero temperature, that the spectrum is symmetric relative to the input frequency, and an exact solution is obtained for the distribution function. For a detuned driving field and nonlinear dispersion, optical bistability can occur. In chapter four a model of sub/second harmonic generation is introduced. This has several non-equilibrium transitions, including dispersive optical bistability, and bistable behaviour with coherent phase-locked input to both modes. Exact solutions occur in the limit of zero temperature and adiabatic elimination of one mode. In both chapters three and four, steady-state photon anti-bunching occurs with an absorptive nonlinearity. In chapter five we include interactions between the radiation mode and a fluorescent atomic system. In this case different behaviour occurs depending on the relative decay rates of the individual atoms and of the radiation mode. In the case of a high-Q interferometer, the atomic variables can be adiabatically eliminated. Both dispersive and absorptive bistability can occur. We show by analytic and numerical calculations (in the case of inhomogeneous broadening) that dispersive operation has advantages in requiring a lower atomic density and input field to observe bistability. When the input field has Gaussian (rather than coherent) photon statistics, there is no bistability, but enhanced photon bunching occurs. Finally, there is a different type of behaviour when the field mode decays rapidly and can be adiabatically eliminated. Within the cooperation lifetime the system can be described by a J²-invariant Hamiltonian, giving the special case of only collective damping. The result is a new type of critical point transition in the thermodynamic limit, with the appearance of a family of solutions like Lotka-Volterra cycles for a coherent driving field above threshold.