The object of this PhD Thesis is light and matter quantum interaction including studies on cavity and circuit quantum electrodynamics (CQED and cQED), quantum information theory and entanglement dynamics in open systems. In recent years both theoretical and experimental efforts have been devoted to study problems regarding the transfer of quantum correlations, quantum memories, entanglement protection against decoherence and new regimes accessible in cQED. One of the fundamental model underlying these topics is the well known Jaynes-Cummings (JC) one for light-matter interaction, introduced in quantum optics already in 1963. This paradigmatic model describes the coherent exchange of a single excitation between a qubit (a two-level system) and a mode of a quantized harmonic oscillator. The JC model describes a lot of purely quantum effects such as Rabi oscillations and generation of entangled quantum states, which were confirmed by several sophisticated experiments in CQED. This model has been then applied in many other frameworks. Analytical results can be derived only under the so-called rotating wave approximation (RWA), which allows to neglect the energy contributions coming from the counter-rotating terms, which describe the simultaneous excitation (or de-excitation) of the qubit and the field mode. In this Thesis a first interesting investigation, based on the JC model, is related to the realization of quantum memories. The main aspect is the transfer of generic quantum entangled states of a propagating radiation to some qubits, such as two-level atoms placed in separated optical cavities. Generalizing previous results for bipartite entangled systems, I investigated the more complex case of tripartite systems, where the very quantification of entanglement is still an open problem. This issue is broadened to open systems in contact with a common environment which induces decoherence effects unavoidable in realistic implementations. The main result of this analysis is that it is possible to map in an optimal way a quantum state from radiation to qubits in the unitary dynamics, and even in the presence of a dissipative environment a significative amount of entanglement can be transferred. This study has been carried on with either theoretical calculations or numerical simulations performed adopting the powerful Monte Carlo wave function method. A second important problem for quantum memories faced in this PhD Thesis, regards the protection of qubits entanglement for long enough times in order to implement quantum information tasks. A possible way to obtain this goal is to add an external coherent field driving two or more two-level atoms interacting with a common mode of a cavity electromagnetic field. In fact it is possible to demonstrate that, under certain conditions, an effective Hamiltonian of the whole system involves, together with the familiar JC terms, also the counter-rotating ones. The main feature that comes out from this analysis is the possibility to freeze, during system dynamics, peculiar quantum entangled states of the atomic qubits in so called decoherence-free subspaces. This important property allows to store the entanglement in matter qubits, isolating the quantum state from environment induced decoherence. Though the system includes dissipation, analytical results have been obtained for multipartite entanglement and decoherence by solving the master equation through a projection on a suitable basis and using the method of characteristics. In particular it is possible to monitor the rate of decoherence via measurements of joint atomic probabilities, shading light on the fascinating border between the quantum and the classical world. A last topic investigated in this Thesis concerns the recently developed and quite promising implementation of the JC model well outside CQED, that is cQED. Here superconductive circuits, which play the role of artificial atoms, interact on-chip with transmission line resonators, instead of the usual electromagnetic cavities. These systems have the advantage of being quite easily engineered exploiting the most advanced available technologies. Moreover they allow a great flexibility in handling the relevant parameters, since the inter-system coupling is here of capacitive or inductive nature, instead of the usual electric dipole interaction in CQED. In this way a strong and ultrastrong coupling regime have become available, giving a direct access to the physics beyond the JC model and its possible applications. I first performed a detailed characterization of system dynamics in order to test the main approximations usually introduced to describe superconductive circuits as qubits. Then I described, both analytically and numerically, the dissipative dynamics of a superconductive qubit coupled to a resonator mode in the deep strong regime.
The object of this PhD Thesis is light and matter quantum interaction including studies on cavity and circuit quantum electrodynamics (CQED and cQED), quantum information theory and entanglement dynamics in open systems. In recent years both theoretical and experimental efforts have been devoted to study problems regarding the transfer of quantum correlations, quantum memories, entanglement protection against decoherence and new regimes accessible in cQED. One of the fundamental model underlying these topics is the well known Jaynes-Cummings (JC) one for light-matter interaction, introduced in quantum optics already in 1963. This paradigmatic model describes the coherent exchange of a single excitation between a qubit (a two-level system) and a mode of a quantized harmonic oscillator. The JC model describes a lot of purely quantum effects such as Rabi oscillations and generation of entangled quantum states, which were confirmed by several sophisticated experiments in CQED. This model has been then applied in many other frameworks. Analytical results can be derived only under the so-called rotating wave approximation (RWA), which allows to neglect the energy contributions coming from the counter-rotating terms, which describe the simultaneous excitation (or de-excitation) of the qubit and the field mode. In this Thesis a first interesting investigation, based on the JC model, is related to the realization of quantum memories. The main aspect is the transfer of generic quantum entangled states of a propagating radiation to some qubits, such as two-level atoms placed in separated optical cavities. Generalizing previous results for bipartite entangled systems, I investigated the more complex case of tripartite systems, where the very quantification of entanglement is still an open problem. This issue is broadened to open systems in contact with a common environment which induces decoherence effects unavoidable in realistic implementations. The main result of this analysis is that it is possible to map in an optimal way a quantum state from radiation to qubits in the unitary dynamics, and even in the presence of a dissipative environment a significative amount of entanglement can be transferred. This study has been carried on with either theoretical calculations or numerical simulations performed adopting the powerful Monte Carlo wave function method. A second important problem for quantum memories faced in this PhD Thesis, regards the protection of qubits entanglement for long enough times in order to implement quantum information tasks. A possible way to obtain this goal is to add an external coherent field driving two or more two-level atoms interacting with a common mode of a cavity electromagnetic field. In fact it is possible to demonstrate that, under certain conditions, an effective Hamiltonian of the whole system involves, together with the familiar JC terms, also the counter-rotating ones. The main feature that comes out from this analysis is the possibility to freeze, during system dynamics, peculiar quantum entangled states of the atomic qubits in so called decoherence-free subspaces. This important property allows to store the entanglement in matter qubits, isolating the quantum state from environment induced decoherence. Though the system includes dissipation, analytical results have been obtained for multipartite entanglement and decoherence by solving the master equation through a projection on a suitable basis and using the method of characteristics. In particular it is possible to monitor the rate of decoherence via measurements of joint atomic probabilities, shading light on the fascinating border between the quantum and the classical world. A last topic investigated in this Thesis concerns the recently developed and quite promising implementation of the JC model well outside CQED, that is cQED. Here superconductive circuits, which play the role of artificial atoms, interact on-chip with transmission line resonators, instead of the usual electromagnetic cavities. These systems have the advantage of being quite easily engineered exploiting the most advanced available technologies. Moreover they allow a great flexibility in handling the relevant parameters, since the inter-system coupling is here of capacitive or inductive nature, instead of the usual electric dipole interaction in CQED. In this way a strong and ultrastrong coupling regime have become available, giving a direct access to the physics beyond the JC model and its possible applications. I first performed a detailed characterization of system dynamics in order to test the main approximations usually introduced to describe superconductive circuits as qubits. Then I described, both analytically and numerically, the dissipative dynamics of a superconductive qubit coupled to a resonator mode in the deep strong regime.
Non-relativistic quantum mechanics have proven to be a significant framework to understand the non-classical behaviour of light and the microcosmos. Perhaps, one of the first technological revolutions within quantum theory came with the invention of the transistor, whereby a purely quantum mechanical description was required. Currently, another outstanding revolution is taking place in a crossroad where information science meets quantum mechanics (this being the quantum information field). Such an area of work contemplates both the fascinating theoretical aspect of quantum correlations, as well as implementations towards quantum tasks performed by a universal quantum computer; tasks that cannot be realised (or they are hard to implement) within the classical domain. This Thesis is devoted to study the dynamics of quantum entanglement in spin-optomechanics systems. In particular, we explore the quantum stabilization of quantum entanglement, a quantum concentration scheme in opto-mechanics and an interfacing of matter and light towards quantum networking applications. Additionally, we also investigate theoretical aspects of quantum correlations within thermal environments, as well as the topical area of quantum sudden transitions. In Chapter 1, we provide a brief summary of quantum information and of the quantum optics framework to cover elementary concepts and techniques used subsequently in this work. Subsequently, in Chapter 2 we present the stabilization of quantum entanglement in a non-linear qubit-oscillator system. The inclusion of a modest nonlinearity gives three results, i) the loss of periodicity of the system, ii) the occurrence of quadrature squeezing appearing for a short time, and iii) the quantum entanglement reaches higher values in contrast to the case without non-linearity. In Chapter 3, a technique to concentrate/distill a two-mode vacuum state in optomechanics via unsharp measurements is presented. Here, one of the optical modes is injected into a cavity at first, and thereafter, it is nonlinearly coupled to a mechanical oscillator. Afterwards, the position of the oscillator is measured using pulsed optomechanics and homodyne detection. The results show that this measurement can conditionally increase the initial entanglement. Next, in Chapter 4, stimulated by optomechanical transducers and quantum networking, a light-matter system is constructed where a qubit is coupled to a cavity mode mediated through a mechanical oscillator. The qubit-oscillator conditionally displaced Hamiltonian and the oscillator-cavity radiation-pressure interaction generate a maximal qubit-cavity entanglement. Additionally, we consider the case in which the cavity mode is coupled to a waveguide, numerical calculations show a promising qubit-fibre entanglement under a weak matter-light coupling. For the quantum network case, we coupled a generic qubit in the first node to a second qubit-cavity distant Jaynes-Cummings system coupled through an optical fibre, where qubit-qubit correlations can be achieved in the quantum open systems scenario. In Chapter 5, we study the evolution of an open quantum system within the Born-Markov microscopic master equation (MME). Essentially, two distant two-level atoms are trapped in fibre-coupled cavities. Under the approximation of one-excitation allowed in the atom-cavity-fibre basis, we can obtain quantum correlations induced by thermal fluctuations from the environments. Lastly, in Chapter 6, we bring together previously elements explored in this Thesis. The system is a hybrid atomic-mechanical system formed from two remote qubits interacting with individual harmonic oscillators. This system, as in Chapter 4, explores interesting applications in quantum networking schemes. The two qubits are initially prepared in a Bell-diagonal state, and consequently the two-qubit correlations exhibit few interesting effects such as freezing, sudden changes and revivals in the evolution of the quantum entropic discord. To conclude, I summarize my findings in Chapter 7.
This thesis studies counter-rotating terms part of an Hamiltonian usually neglected in the so-called Rotating Wave Approximation. Generalising the usual description of light-matter interactions and open quantum systems it is demonstrated that normally neglected counter-rotating terms have the potential to allocate energy among different system degrees of freedom. It is pointed out in examples that this aspect can affect the energy concentration in quantum systems. Initially, a composite quantum system is considered, i.e. bipartite systems like atom-cavity systems and coupled optical resonators without decay. By resorting to methods from quantum field theory it is shown that for such bosonic systems, the Rotating Wave Approximation cannot be applied far off resonance. In fact, the counter-rotating terms are related to an entropy operator that is capable of generating an irreversible time evolution. The vacuum state of the system is shown to evolve into a generalised coherent state exhibiting entanglement of the modes in which the counter-rotating terms are expressed. Furthermore, it is demonstrated that a non-trivial behaviour of the photon emission rate of such composite quantum system can occur when the counter-rotating terms are not dropped. In such a system, there is a coupling to infinitely many modes with most of them being far off resonance. An energy concentrating mechanism is discussed which cannot be described by the Rotating Wave Approximation. Its result is the continuous leakage of photons from open quantum system, even in the absence of external driving. Finally, a model is proposed to explain the origin of the sudden energy concentration in the intriguing phenomenon of sonoluminescence. The model is based on the quantum dynamics of trapped particles and assumes the presence of a weak but highly inhomogeneous electric field. It is shown that the counter-rotating terms can significantly contribute to the energy focussing mechanism in terms of quantum coherences.
Remarkable experimental progress and theoretical advancements in the study of strongly corre- lated systems have opened up new doors towards a better understanding of interesting states of matter. Such states could possibly be used to develop novel technological applications based on the principles of quantum mechanics. In recent years, the investigation of both complex solid state and ultracold atom systems has lead to a number of fascinating discoveries with regards to their non-equilibrium properties. One route to probe non-equilibrium physics is to consider the evolution of open systems defined by the coupling to an external environment introducing dissipation. Engineering the environment according to predefined requirements can then be used to dynamically prepare states which are difficult to access otherwise. This thesis explores the dynamics of many-body open quantum systems aiming at under- standing the effects resulting from the interplay of kinetic motion, interactions and dissipation in different physical settings. First, we build upon recent developments concerning the coupling of ultracold atoms to optical resonators which are subject to photon losses. We show how the dissipation can trigger an attractor dynamics towards a topologically non-trivial steady state that is robust against perturbations. The numerically obtained full open system evolution en- ables us to not only characterize in detail the steady state but also to analyze the features of the approaching dynamics. Second, we study the propagation of two-time correlation functions in interacting quantum spin-1/2 chains in contact with an environment causing dephasing. Pro- vided with the numerically exact full time-evolution, we identify an algebraic scaling regime where time-translation invariance breaks down and uncover the emergence of aging dynam- ics. Finally, we study a system of interacting fermionic atoms in a one-dimensional lattice with particle loss at the central site. There we report on the dissipation-induced deceleration of the non-equilibrium dynamics known as the quantum Zeno effect. As in the majority of cases quantum many-body systems are not solvable analytically, another central aspect of this thesis deals with adapting numerical methods based on matrix product state algorithms to investigate open quantum systems dynamics.
The goal of research in quantum information is to investigate how quantum systems can be used to store, transmit and elaborate information and how the non-classical nature of their correlations allows defining protocols that outperform their classical counterparts. Despite of the many progresses, both theoretical and experimental, made in this field in the latest decades, many challenges lie ahead for practical implementations of quantum technologies. One of the most important ones is caused by the unavoidable interaction of quantum systems with their surroundings: The coupling to the environment is generally detrimental to the quantum information contained in the system as the system undergoes decoherence. In the quest for quantum technologies, it is fundamental to overcome the problem of decoherence and loss of information. Different physical implementations of qubits, such as superconducting and solid-state devices, are affected by the interaction with the environment in a way that can be described in terms of classical stochastic noise. The classical noise model can also be used to give an approximate, sometimes equivalent, description of full quantum models of system-environment interaction. This thesis contains my personal contribution to the study of the dynamics of discrete-variable quantum systems affected by classical noise. It covers in particular single- and two-qubit systems affected by Gaussian and non-Gaussian noise. It also discusses the dynamics of a quantum walk affected by spatially correlated classical noise. Analytical solutions for particular forms of noise and interactions, and a general numerical method for simulation of the dynamics are presented. Moreover, the thesis presents the experimental implementation of a quantum optical simulator of noisy dynamics of single-qubit systems. Finally, the use of quantum systems as probes of the spectral properties of large classical environments is discussed, showing that entanglement is a resource for improvements in the precision of the estimation.
This thesis is devoted to theoretically study the systems of single quantum dots (QDs) embedded in various photonic nanostructures, in close relation with experimental data. The word single is essential: due to their nanometer size, QDs have mainly been studied as ensembles. It is only recently that the experimental progress, in particular in the domain of QDs growth, has allowed to address single QDs. This helped to observe that the confined states in a QD resemble those of an atom, leading in turn to the macro-atom picture for QDs. It opened the path to the study of cavity quantum electrodynamics (CQED) in the solid state, as the analogous of a system of an atom in an electromagnetic cavity. However, already at the level of the QD (i.e. without a solid state cavity), the macro-atom picture has been proven to be oversimplified. Various effects related to the solid state environment of the QD have been experimentally and theoretically evidenced, like the influence of acoustic and optical phonons. These are channels of decoherence for the otherwise well isolated and confined QD levels. When adding the cavity, these effects are possibly enhanced, which can lead to very large deviations from the CQED ideal picture. Therefore the clear understanding of these effects is of essential importance, especially in view of the application of solid state systems to quantum information science. In Chapter 2, we address the radiation-matter coupling between two QDs in a nanocavity. This field of research combines the high quality of light resonators to the nonlinearities of the semiconductor material. It is promising in view of manipulating and transferring single long-lived excitations, an essential goal for quantum information science. Then, we study the deviations of a QD from the idealized macroatom picture. First, in Chapter 3, we include the influence of acoustic phonons on the light emitted by a QD-cavity system. We show that the QD modified susceptibility leads to the qualitative explanation of the cavity feeding effects, which is one of the most striking deviations of the QD-cavity system from the ideal CQED picture. In addition to phonons are extended two-dimensional states populated by the non resonant pumping laser in the QD's wetting layer (WL). In Chapters 4 and 5 we build a Monte-Carlo model of the excitation-decay mechanism in a QD-cavity system. We use it to describe the influence of WL states on the dynamics of the QD, leading in turn to a non-CQED behavior. This approach is particularly successful in the case of large QD-cavity detuning, where it predicts both time-dependent and spectral characteristics of the emitted light. Finally, in Chapter 6, we discuss our conclusions, emphasizing in particular that the knowledge of the actual solid state environment of the QD leads to a better control over the parameters allowing to reach the CQED regime. We also discuss the possible extensions of this work, in particular in relation to the analysis of the stimulated emission regime.
The interaction of a two-level atom with a single-mode quantized field is one of the simplest models in quantum optics. Under the rotating wave approximation, it is known as the Jaynes-Cummings model and without it as the Rabi model. Real-world realizations of the Jaynes-Cummings model include cavity, ion trap and circuit quantum electrodynamics. The Rabi model can be realized in circuit quantum electrodynamics. As soon as nonlinear couplings are introduced, feasible experimental realizations in quantum systems are drastically reduced. We propose a set of two photonic lattices that classically simulates the interaction of a single two-level system with a quantized field under field nonlinearities and nonlinear couplings as long as the quantum optics model conserves parity. We describe how to reconstruct the mean value of quantum optics measurements, such as photon number and atomic energy excitation, from the intensity and from the field, such as von Neumann entropy and fidelity, at the output of the photonic lattices. We discuss how typical initial states involving coherent or displaced Fock fields can be engineered from recently discussed Glauber-Fock lattices. As an example, the Buck-Sukumar model, where the coupling depends on the intensity of the field, is classically simulated for separable and entangled initial states.