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Bulletin of the American Physical Society

Quantum information processing and non-linear optics using polar molecules

Susanne F. Yelin

Published May 30, 2008• 0 citations
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We propose a linear-optics-based scheme for local conversion of four Einstein-Podolsky-Rosen photon pairs distributed among five parties into four-photon polarization-entangled decoherence-free states using local operations and classical communication. The proposed setup involves simple linear optical elements and non-photon-number-resolving detectors that can only distinguish between the presence and absence of photons, and no information on the exact number of photons can be obtained. This greatly simplifies the experimental realization for linear optical quantum computation and quantum information processing.
The non-linear optical polarization of an isolated atom or molecule is treated, giving careful consideration to secular and resonant terms in the perturbation expansion. The Method of Averages introduced by Bogoliubov and Mitropolsky is used. The case where resonance-induced excited state populations are negligible, which is relevant to a wide range of non-linear optical experiments, is examined in detail for polarizations through third order in the perturbing fields. This yields concise expressions which are valid for any combination of applied field frequencies, including static fields.