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European Quantum Electronics Conference (EQEC)

Probe spectroscopy of cold rubidium atoms in MOT

Vasily M. Entin, I. I. Ryabtsev

Published Jan 18, 2006• 0 citations
Publisher

Abstract

The experimental results of the probe spectroscopy of laser cooled Rb atoms in a magneto-optical trap (MOT) are presented. The absorption spectra of the probe transition were expected to be significantly different, and indications of coherent population trapping were expected for the dark repumping transition.
DOI
10.1109/eqec.2005.1567376

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Spectral characteristics of rubidium atoms confined in a dark magneto-optical trap (DMOT) are measured, including probe absorption spectra and atom density as a function of the cooling and repumping laser frequencies. The trap can capture and cool more than 2.5 × 10 8 rubidium atoms, confining them in a hyperfine state weakly perturbed by the laser beams used to form the trap. The optical density of the trapped atomic cloud approaches 9. A qualitative model of the DMOT operation is presented, based on the experimental results obtained.
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The interaction of light with atoms and molecules is of fundamental interest in many branches of science. In atomic physics, this interaction can be used to cool and spatially confine (trap) atoms. These traps can be used as the starting point for other experiments, but the dynamics of the cooling and trapping processes is itself of interest. In order to better understand the physics of trapping atoms in an optical dipole force trap, we have conducted a series of spectroscopic measurements of ultracold rubidium atoms in such a trap. The trap was created at the focus of a Nd:YAG laser beam with wavelength 1064nm and nearly Gaussian spatial mode. For rubidium, the trap light is red-detuned and the atoms are confined to the highest intensity in the beam. In order to probe the atoms confined in the trap, we have performed spectroscopy on the 5S1/2 → 5P3/2 transition. Because the polarizability of the ground and excited states is not the same at the trap wavelength, the spectra exhibit both a shift and inhomogeneous broadening. We have investigated the spectra for both linear and circular polarized traps. We also studied the application of a second laser to couple the excited state (5P3/2) to another higher excited state (5D5/2) to reduce the inhomogeneous broadening of the 5S1/2 → 5P 3/2 transition. Finally, two-photon spectroscopy was performed on atoms in the dipole force trap and compared to spectra taken in a magneto optical trap (MOT). Autler-Townes splitting was clearly observed in the MOT and appears to have been observed in the dipole force trap also.
We report an experimental demonstration of optical two-dimensional coherent spectroscopy (2DCS) in cold atoms. The experiment integrates a collinear 2DCS setup with a magneto-optical trap (MOT), in which cold rubidium (Rb) atoms are prepared at a temperature of approximately 200 µK and a number density of 10 10 cm −3 . With a sequence of femtosecond laser pulses, we first obtain one-dimensional second- and fourth-order nonlinear signals and then acquire both one-quantum and zero-quantum 2D spectra of cold Rb atoms. The capability of performing optical 2DCS in cold atoms is an important step toward optical 2DCS study of many-body physics in cold atoms and ultimately in atom arrays and trapped ions. Optical 2DCS in cold atoms/molecules can also be a new avenue to probe chemical reaction dynamics in cold molecules.