The subject of this dissertation is the experimental discovery and investigation of a new class of collective phases in two-dimensional electron systems. The experiments mainly involve magnetotransport measurements in very high quality GaAs/AlGaAs semiconductor heterostructures, where a large perpendicular magnetic field serves to resolve the electrons? energy spectrum into discrete Landau levels. The most dramatic evidence of a new many-body phase is the huge and unprecedented resistance anisotropy observed only below 150 mK and around the half-filling points of the highly excited Landau levels N > 1. Associated with these anisotropic states are other novel electron phases whose transport signature is a vanishing longitudinal conductivity occurring in the flanks of the same excited Landau levels. Although reminiscent of the well-understood integer quantum Hall states, the insulating phases are exceptional for being driven by electron interactions rather than single-particle localization. A persuasive theoretical picture based on "stripe" and "bubble" charge density wave formation in high Landau levels can account for many of the experimental results. For example, the broken orientational symmetry of the stripe state may underlie the observed transport anisotropy, while disorder-induced pinning of the bubble lattice could give rise to the insulating regions in high Landau levels. Further investigation of the anisotropic transport characteristics has elucidated possible symmetry-breaking mechanisms of the purported stripe phase and has provided evidence that the stripes may be more accurately described as a quantum electronic liquid crystal. In addition, experiments involving the breakdown of the insulating regions at high voltage biases may point to a depinning transition of the bubble phase. These results have spurred intense interest in the field of correlated electron systems in two dimensions and may be an indication of the variety of new phenomena in condensed matter systems still awaiting discovery.
The subject of this dissertation is the experimental discovery and investigation of a new class of collective phases in two-dimensional electron systems. The experiments mainly involve magnetotransport measurements in very high quality GaAs/AlGaAs semiconductor heterostructures, where a large perpendicular magnetic field serves to resolve the electrons? energy spectrum into discrete Landau levels. The most dramatic evidence of a new many-body phase is the huge and unprecedented resistance anisotropy observed only below 150 mK and around the half-filling points of the highly excited Landau levels N > 1. Associated with these anisotropic states are other novel electron phases whose transport signature is a vanishing longitudinal conductivity occurring in the flanks of the same excited Landau levels. Although reminiscent of the well-understood integer quantum Hall states, the insulating phases are exceptional for being driven by electron interactions rather than single-particle localization. A persuasive theoretical picture based on "stripe" and "bubble" charge density wave formation in high Landau levels can account for many of the experimental results. For example, the broken orientational symmetry of the stripe state may underlie the observed transport anisotropy, while disorder-induced pinning of the bubble lattice could give rise to the insulating regions in high Landau levels. Further investigation of the anisotropic transport characteristics has elucidated possible symmetry-breaking mechanisms of the purported stripe phase and has provided evidence that the stripes may be more accurately described as a quantum electronic liquid crystal. In addition, experiments involving the breakdown of the insulating regions at high voltage biases may point to a depinning transition of the bubble phase. These results have spurred intense interest in the field of correlated electron systems in two dimensions and may be an indication of the variety of new phenomena in condensed matter systems still awaiting discovery.
Materials with strongly correlated electrons show a multitude of unconventional phenomena, such as superconductivity or magnetism, that cannot be explained in a single-particle picture and necessitate to take many-body effects into account. A route to explain the origin of these phenomena consists in constructing effective models for these materials that are then solved, often using numerical techniques. Paradigmatic models for two different classes of strongly correlated electron systems are investigated in this thesis: The Hubbard model is a paradigmatic model to describe the Mott metal-insulator transition (MIT) and the Kondo lattice model describes the low-energy physics in heavy fermion compounds. Both models are analyzed numerically using different variations of a quantum cluster technique, the variational cluster approximation (VCA). The first part focuses on the MIT, as it is investigated experimentally in quasi-two-dimensional charge-transfer salts. Its nature and associated universality class are still heavily discussed and both experiments and theoretical approaches come to different conclusions. In this thesis, the Mott transition is investigated on an anisotropic two-dimensional Hubbard model at half-filling. By using a control parameter, which induces this anisotropy, strong evidence for Mott quantum criticality is found in weakly coupled Hubbard chains. The results at zero temperature show that the second-order critical end point Tc of the interaction-driven metal-insulator transition can be tuned down to zero at strong anisotropy. Further results for the antiferromagnetic phase suggest a similar picture and motivate adding the anisotropy as a new axis in the phase diagram to account for a low-temperature critical end point of the Mott transition. The second part of this thesis focuses on unconventional phases that emerge in a paradigmatic model for heavy fermion systems, the Kondo lattice model. Using the VCA, the two-dimensional Kondo lattice model is investigated in the paramagnetic phase as well as in phases with broken symmetry. An antiferromagnetic phase at weak coupling and a phase with Kondo-singlet formation at strong coupling are analyzed. Within the antiferromagnetically ordered region, two phases with different Fermi-surface topology, which are separated by a discontinuous transition, are identified. The model is also tested for s-wave superconductivity as found recently using dynamical mean-field theory, but no indications for robust local pairing are seen within VCA. Instead, nodal d-wave superconductivity is found and analyzed in a large range of couplings and electron fillings, and its interplay with antiferromagnetic order at weak coupling is discussed. This motivates further studies on extended models that might allow for a close comparison with experiments on heavy fermion systems. Understanding the formation of unconventional phases in strongly correlated electron systems is not only of fundamental interest, but it is also essential for designing new functional materials. Although the results of approximate cluster techniques have to be handled with care, the new aspects presented in this thesis pave the way for further investigations in this direction.
This thesis investigates interaction-driven phenomena of two-dimensional electrons in strong magnetic fields, with a focus on how the electron-electron (e-e) interaction projected in one Landau level affects the physical properties of the topological bands. The Landau-level-projected interaction favours qualitatively different ground states in different situations, such as topologically ordered fractional quantum Hall liquids that host anyonic quasiparticles, and symmetry-broken electron solids or charge-ordered phases. In the fractional quantum Hall liquid, we study quasiholes as interacting particles rather than featureless point excitations in a dilute and ideal anyon gas. Going beyond model Hamiltonians, we show that realistic e–e interactions generate nontrivial effective anyon–anyon interactions that can endow few-anyon clusters with internal structure and binding, producing “anyon molecules”. Because the same effective interaction also controls how anyons couple to local probes, we compute local density-of-states signatures and show that local tunneling spectra can encode both universal and non-universal information. The analysis is carried out for the Abelian Laughlin states and for the non-Abelian Moore–Read state, the latter one showing characteristic odd–even features tied to its fusion structure. In the high-Landau-level regime, the same interaction-driven physics favors symmetry-broken charge order. We construct a microscopic-to-continuum framework that connects Landau-level-projected Hartree--Fock energetics to elastic constants and, through Kosterlitz--Thouless--Halperin--Nelson--Young defect physics and renormalization-group flow, to a quantitative finite-temperature melting scale. This approach highlights the role of dislocation proliferation-induced thermal renormalization in quantitatively understanding the 2D electron solids' melting, and enables direct comparison with transport signatures of re-entrant insulating phases. Taken together, we provide an interaction-based perspective on both topological quantum Hall liquids and quantum Hall electron solids in Landau levels. This thesis closes by outlining several directions that follow naturally from this work.
"This thesis is devoted to the investigation of the quantum liquid crystal phases in strongly correlated electronic systems. Such phases are characterized by their partially broken spatial symmetries and are observed in various strongly correlated systems as being summarized in Chapter 1. In quantum liquid crystal phases formed by fermions, behaviors beyond Landau's theory of the Fermi liquids appear naturally, signed by the absence of well-defined quasiparticle excitations. Although quantum liquid crystal phases often involve strong-coupling physics, the associated symmetry analysis can often be carried out also in a relatively weak coupling regime and this is the main approach taken in this thesis. Two different quantum liquid crystal phases, the nematic state and the smectic state, are studied in Chapters 2 and 3 respectively, by investigating various instabilities of a Landau Fermi liquid. A nematic phase is a state that breaks the rotational symmetry spontaneously but preserves the translational symmetries. It can be reached by the Pomeranchuk instability of a Landau Fermi liquid. The Pomeranchuk instability in the charge (spin-singlet) sector of a Fermi liquid was studied previously within a random phase approximation and by a high-dimensional bosonization method. In Chapter 2, we concentrate on the Pomeranchuk instability in the spin-triplet sector, and two different classes of ordered phases are discovered, dubbed the a and ,8-phases by analogy to the superfluid 3He-A and B-phases. The Fermi surfaces in the a-phases exhibit spontaneous anisotropic distortions, while in the ,8-phases the Fermi surfaces remain circular or spherical with topologically non-trivial spin configurations in momentum space. The behaviors of the low energy bosonic excitations are studied both in the order phases (a and .B) and at the quantum critical point separating the ordered phases from the Fermi liquid phase. In Chapter 3, the smectic phase and the quantum phase transition between a metallic nematic state and a metallic smectic phase are investigated using the random phase approximation, by considering the formation of a unidirectional charge density wave in an electronic nematic state. The associated quantum critical point is investigated within the Hertz-Millis approach. Non-Fermi liquid behaviors are discovered both at the quantum phase transition and in the smectic ordered phase. The theory we studied here provides a simple description for the so-called ""fluctuating stripe"" phase in cuprates. Similar to its classical counterpart, the phase transition between the nematic and smectic phases are described by a ""gauge-like"" theory as required by the rotational invariance in close analogy with the McMillan-deGennes theory of the smectic-nematic phase transition in classical liquid crystals. However, unlike the classical McMillandeGennes theory, in which the coupling between the ""gauge-like"" nematic fluctuations and the ""matter-like"" smectic fields is relevant, in the sense of renormalization group, this coupling is irrelevant at the quantum phase transition. This property enables the study of low energy fluctuations and the fate of fermions near this quantum critical point. In Chapter 4, quantum liquid crystal phases with a broken time-reversal symmetry are investigated. We start by studying the general scenario of timereversal symmetry breaking phases in the absence of magnetic ordering in systems with long-lived low-energy fermionic quasiparticle excitations in two dimensions. Using a Berry phase approach, we classified possible time-reversal symmetry breaking phases by the accompanying spatial symmetry breaking patterns. Two of the simplest situations are referred to as the type I state, which breaks simultaneously the space-inversion symmetry and the time-reversal symmetry, and the type I I state, in which the chiral symmetry is broken in addition to the breaking of the time-reversal symmetry. Although the starting point is general and has little relation with the quantum liquid crystal phases, both type I and type II states defined above are realized by (generalized) Pomeranchuk instabilities. In fact , a type I I state is usually a nematic state which also breaks the time-reversal symmetry. Interestingly, the type II states also shows spontaneously generated Hall effect even in the absence of a magnetic field, which is known as the spontaneous anomalous Hall effect. In Chapter 5, we investigate the stability of a quadratic band-crossing point in two-dimensional fermionic systems that provide an explicit example, within well controlled approximations, for the nematic ordering discussed in Chapter 2 and spontaneous anomalous Hall effect discussed in Chapter 4. At the non-interacting level, we show that a quadratic band-crossing point exists and is topologically stable when the Berry flux of this crossing point is ±27r and the point symmetry group at this point has either fourfold or sixfold rotational symmetries. Strikingly, we find that this would-be topologically stable quadratic band-crossing is marginally unstable against short-range interactions: a quadratic band-crossing point in two dimensions is unstable against shortrange repulsion, no matter how weak! Four ordered phases are found in this system, the quantum anomalous Hall state, the quantum spin Hall phase, the nematic phase, and the nematic-spin-nematic phase."
This thesis is devoted to the study of strongly correlated phases of quantum matter in two spatial dimensions. In presence of strong interactions, the electron can split up into separate spin and charge degrees of freedom. The diagnosis of such fractionalized excitations in recent experiments, as well as finding new probes for their detection, comprise the two major themes of this thesis.\nThe first part of the thesis, comprising chapters 2-6, discusses the relevance of fractionalization to the pseudogap phase of the underdoped high Tc cuprate superconductors. This is motivated by transport experiments that show a violation of Luttinger's theorem, possible only in the presence of topological order that can arise naturally as a consequence of fractionalization. Chapters 2 and 3 focus on phenomenological models with bosonic charge carriers and fermionic spin carriers, and investigate transport properties as well as various confinement transitions to symmetry broken phases. Chapters 4, 5 and 6 deal with a different framework of electron fractionalization, where the charge carriers are fermionic and spin carriers are bosonic. We find that these models can better explain the thermal and electrical transport properties in chapter 5. In chapters 6 and 7, we show how such models arise naturally from quantum fluctuations of antiferromagnetism, and can simultaneously intertwine the anti-nodal spectral gap with the discrete broken symmetries that are observed in the cuprates. \nThe second part of the thesis, comprising chapters 7 and 8, proposes new experimental probes to study the behavior of insulating two dimensional quantum magnets. Aided by geometric frustration and strong quantum fluctuations, they may realize a spin liquid ground state which can be extremely difficult to detect via conventional probes. Chapter 7 discusses how novel spin-transport probes from the spintronics community can be used to detect fractionalized excitations in a quantum spin liquid. Chapter 8 studies how the temperature dependent anisotropy of in-plane versus out-of-plane thermal conductivities can serve as an explicit signature of fractionalization in layered two-dimensional materials.
Abstract In recent experiments, external anisotropy has been a useful tool to tune different phases and study their competitions. In this paper, we look at the quantum Hall charge density wave states in the N = 2 Landau level. Without anisotropy, there are two first-order phase transitions between the Wigner crystal, the 2-electron bubble phase, and the stripe phase. By adding mass anisotropy, our analytical and numerical studies show that the 2-electron bubble phase disappears and the stripe phase significantly enlarges its domain in the phase diagram. Meanwhile, a regime of stripe crystals that may be observed experimentally is unveiled after the bubble phase gets out. Upon increase of the anisotropy, the energy of the phases at the transitions becomes progressively smooth as a function of the filling. We conclude that all first-order phase transitions are replaced by continuous phase transitions, providing a possible realisation of continuous quantum crystalline phase transitions.
A low-disorder, two-dimensional electron system (2DES) subjected to a large perpendicular magnetic field and cooled to very low temperatures provides a rich platform for studies of many-body quantum phases. The magnetic field quenches the electrons' kinetic energy and quantizes the energy into a set of Landau levels, allowing the Coulomb interaction to dominate. In excited Landau levels, the fine interplay between short- and long-range interactions stabilizes bubble phases, Wigner crystals with more than one electron per unit cell. Here, we present the screening properties of bubble phases, probed via a simple capacitance technique where the 2DES is placed between a top and a bottom gate and the electric field penetrating through the 2DES is measured. The bubbles formed at very low temperatures screen the electric field poorly as they are pinned by the residual disorder potential, allowing a large electric field to reach the top gate. As the temperature is increased, the penetrating electric field decreases and, surprisingly, exhibits a pronounced minimum at a temperature that appears to coincide with the melting temperature of the bubble phase. We deduce a quantitative phase diagram, as a function of Landau level filling factor (\ensuremath{\nu}) and temperature, for the transition from the bubble to liquid phases for $4\ensuremath{\le}\ensuremath{\nu}\ensuremath{\le}5$.