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Spinor Bose Gases in Cubic Optical lattice

Mohamed Mobarak

Published Jan 1, 2014• 1 citation
Publisher

Abstract

In recent years the quantum simulation of condensed-matter physics problems has resulted from ex- citing experimental progress in the realm of ultracold atoms and molecules in optical lattices. In this thesis we analyze theoretically a spinor Bose gas loaded into a three-dimensional cubic optical lattice. In order to account for different superfluid phases of spin-1 bosons with a linear Zeeman effect, we work out a Ginzburg-Landau theory for the underlying spin-1 Bose-Hubbard model. To this end we add artificial symmetry- breaking currents to the spin-1 Bose-Hubbard Hamiltonian in order to break the global U (1) symmetry. With this we determine a diagrammatic expansion of the grand-canonical free energy up to fourth order in the symmetry-breaking currents and up to the leading non-trivial order in the hopping strength which is of first order. As a cross-check we demonstrate that the resulting grand- canonical free energy allows to recover the mean-field theory. Applying a Legendre transfor- mation to the grand-canonical free energy, where the symmetry-breaking currents are transformed to order parameters, we obtain the effective Ginzburg-Landau action. With this we calculate in detail at zero temperature the Mott insulator-superfluid quantum phase boundary as well as condensate and particle number density in the superfluid phase. We find that both mean-field and Ginzburg-Landau theory yield the same quantum phase transition between the Mott insulator and superfluid phases, but the range of validity of the mean-field theory turns out to be smaller than that of the Ginzburg-Landau theory. Due to this finding we expect that the Ginzburg-Landau theory gives better results for the superfluid phase and, thus, we restrict ourselves to extremize only the effective Ginzburg-Landau action with respect to the order parameters. With- out external magnetic field the superfluid phase is a polar (ferromagnetic) state for anti-ferromagnetic (ferromagnetic) interactions, i.e. only the hyperfine spin 0 (1) is macroscopically occupied, in accor- dance with previous mean-field results. On the other hand, in the presence of the external magnetic field for ferromagnetic interaction, the superfluid phase does not change as the minimization of the energy implies the maximal spin value. However, when an anti-ferromagnetic interaction competes with the linear Zeeman effect, we can distinguish various ferromagnetic and anti-ferromagnetic su- perfluid phases within the range of validity of the Ginzburg-Landau theory. Increasing the external magnetic field yields a breaking of spin singlet pairs and a subsequent alignment of spins, thus anti- ferromagnetic phases decrease until only a ferromagnetic superfluid phase prevails. In addition, we find that the superfluid-Mott insulator phase transition is always of second order for both ferromag- netic and anti- ferromagnetic interactions. However, the transitions between different superfluid phases for an anti-ferromagnetic interaction can be both of first and second order depending on whether the respective macroscopic occupation of hyperfine spin states changes discontinuously or continuously. The established Ginzburg-Landau theory for spin-1 bosons in optical lattices will certainly be the basis for many further applications as, for instance, time-of-flight absorption pictures or collective excitations, which are of experimental importance.

DOI
10.17169/refubium-9705

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In recent years the quantum simulation of condensed-matter physics problems has resulted from ex- citing experimental progress in the realm of ultracold atoms and molecules in optical lattices. In this thesis we analyze theoretically a spinor Bose gas loaded into a three-dimensional cubic optical lattice. In order to account for different superfluid phases of spin-1 bosons with a linear Zeeman effect, we work out a Ginzburg-Landau theory for the underlying spin-1 Bose-Hubbard model. To this end we add artificial symmetry- breaking currents to the spin-1 Bose-Hubbard Hamiltonian in order to break the global U (1) symmetry. With this we determine a diagrammatic expansion of the grand-canonical free energy up to fourth order in the symmetry-breaking currents and up to the leading non-trivial order in the hopping strength which is of first order. As a cross-check we demonstrate that the resulting grand- canonical free energy allows to recover the mean-field theory. Applying a Legendre transfor- mation to the grand-canonical free energy, where the symmetry-breaking currents are transformed to order parameters, we obtain the effective Ginzburg-Landau action. With this we calculate in detail at zero temperature the Mott insulator-superfluid quantum phase boundary as well as condensate and particle number density in the superfluid phase. We find that both mean-field and Ginzburg-Landau theory yield the same quantum phase transition between the Mott insulator and superfluid phases, but the range of validity of the mean-field theory turns out to be smaller than that of the Ginzburg-Landau theory. Due to this finding we expect that the Ginzburg-Landau theory gives better results for the superfluid phase and, thus, we restrict ourselves to extremize only the effective Ginzburg-Landau action with respect to the order parameters. With- out external magnetic field the superfluid phase is a polar (ferromagnetic) state for anti-ferromagnetic (ferromagnetic) interactions, i.e. only the hyperfine spin 0 (1) is macroscopically occupied, in accor- dance with previous mean-field results. On the other hand, in the presence of the external magnetic field for ferromagnetic interaction, the superfluid phase does not change as the minimization of the energy implies the maximal spin value. However, when an anti-ferromagnetic interaction competes with the linear Zeeman effect, we can distinguish various ferromagnetic and anti-ferromagnetic su- perfluid phases within the range of validity of the Ginzburg-Landau theory. Increasing the external magnetic field yields a breaking of spin singlet pairs and a subsequent alignment of spins, thus anti- ferromagnetic phases decrease until only a ferromagnetic superfluid phase prevails. In addition, we find that the superfluid-Mott insulator phase transition is always of second order for both ferromag- netic and anti- ferromagnetic interactions. However, the transitions between different superfluid phases for an anti-ferromagnetic interaction can be both of first and second order depending on whether the respective macroscopic occupation of hyperfine spin states changes discontinuously or continuously. The established Ginzburg-Landau theory for spin-1 bosons in optical lattices will certainly be the basis for many further applications as, for instance, time-of-flight absorption pictures or collective excitations, which are of experimental importance.
We analyze theoretically a spinor Bose gas loaded into a three-dimensional cubic optical lattice. In order to account for different superfluid phases of spin-1 bosons in the presence of an external magnetic field, we work out a Ginzburg-Landau theory for the underlying spin-1 Bose-Hubbard model. In particular at zero temperature, we determine both the Mott and the superfluid phases for the competition between the anti-ferromagnetic interaction and the linear Zeeman effect within the validity range of the Ginzburg-Landau theory. Moreover, we find that the phase transition between the superfluid and Mott insulator phases is of second order and that the transitions between the respective superfluid phases for anti-ferromagnetic interaction can be both of first and second order.
We analyze theoretically the emergence of different superfluid phases of spin-1 bosons in a three-dimensional cubic optical lattice by generalizing the recently developed Ginzburg–Landau theory for the Bose–Hubbard model to a spinor Bose gas. In particular at zero temperature, our theory distinguishes within its validity range between various superfluid phases for an anti-ferromagnetic interaction with an external magnetic field. In addition, we determine that the superfluid–Mott insulator phase transition is of second order and that the transitions between the respective superfluid phases with anti-ferromagnetic interaction can be both of first and second order.
Since the experimental realization of Bose-Einstein condensation in 1995, the field of ultracold atoms has expanded rapidly, and has become an important arena for exploring diverse quantum many-body physics, as highlighted by the experimental observation of quantum phase transitions in the system of bosons in a periodic potential, which is described by the Bose-Hubbard model.Recently, ultracold atoms with spin degrees of freedom are actively studied because the coupling between the internal spin degrees of freedom and the spatial degrees of freedom can give rise to novel and interesting physics.A minimal model for studying such physics is the spin-1 Bose-Hubbard model, which describes spin-1 bosons in a periodic potential.The model has a spin-dependent interaction, which can be ferromagnetic or antiferromagnetic, and it is known that although the ferromagnetic model resembles the spinless counterpart, the antiferromagnetic model exhibits totally different features, which make the model much more intensively studied compared with the ferromagnetic one.However, the presence of an external magnetic field can change the situation, because the positive quadratic Zeeman energy competes with the ferromagnetic interaction, which can give rise to rich phases.In this thesis, we explore the ground-state and nonzero-temperature phase diagrams of the spin-1 Bose-Hubbard model under an external magnetic field.To analyze the model, we use an approximation method called the decoupling approximation, or equivalently, the Gutzwiller variational ansatz.It is shown that, in addition to the Mott insulator phase, the model possesses two superfluid phases.Moreover, for large values of a spin-dependent interaction, the phase transitions between the two superfluid phases can be discontinuous.Such discontinuous phase transitions are shown to survive at nonzero but sufficiently low temperature.The discontinuous phase transitions are in clear contrast to the mean-field theory of weakly interacting spin-1 bosons without a lattice, which predicts that the corresponding phase transition is continuous, signifying the importance of the effect of strong interactions on the interplay between the spatial and spinor degrees of freedom. 4.1.2The grand Hamiltonian . . . . . . . . .
In this thesis, we investigate strongly correlated phenomena in quantum spin systems. In the first part of this work, we study geometrically frustrated antiferromagnets (AFMs). Generalizing the SU(2) Heisenberg Hamiltonian to Sp(N) symmetry, we obtain, in the large-N limit, the mean-field phase diagrams for the planar pyrochlore and cubic AFMs. We then use gauge theories to consider fluctuation effects about their respective mean-field configurations. We find, in addition to conventional Neel states, a plethora of novel magnetically disordered phases: two kinds of spin liquids, Z2 in 2+1D and U(1)in 3+1D, and several valence bond solids such as two and three-dimensional plaquette and columnar singlet states. We use the same approach to study the diamond lattice AFM which possesses extended classical ground state degeneracy. We demonstrate that quantum and entropic fluctuations lift this degeneracy in different ways. In the second part of the thesis, we study ultracold spinor atoms confined in optical lattices. We first demonstrate the feasibility of experimental realization of rotor models using ultracold spin-one Bose atoms in a spin-dependent and disordered optical lattice. We show that the ground state of such disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense, and suggest an imaging experiment to detect the biaxial nematicity in such systems. Finally, using variational wavefunction methods, we study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two dimensional optical trap. We chart out the phase diagrams for Mott states with n = 1 and n = 2 atoms per lattice site. We show that the long-range dipolar interaction stabilizes a state characterized by antiferromagnetic chains made of ferromagnetically aligned spins. We also obtain the mean-field phase boundary for the superfluid-insulator transition, and show that inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first order antiferromagnetic-ferromagnetic spin ordering transition.
In this thesis we study various aspects of spinor Bose-Einstein condensates in optical superlattices using a Bose-Hubbard Hamiltonian that takes spin effects into account. We decouple the unit cells of the superlattice via a mean-field approach and take into account the dynamics within the unit cell exactly. In this way we derive the ground-state phase diagram of spinor bosons in superlattices. The system supports Mott-insulating as well as superfluid phases. The transitions between these phases are second-order for spinless bosons and second- or first-order for spin-1 bosons. Antiferromagnetic interactions energetically penalize high-spin configurations and elongate all Mott lobes, especially the ones corresponding to an even atom number on each lattice site. We find that the quadratic Zeeman effect lifts the degeneracy between different polar superfluid phases leading to additional metastable phases and first-order phase transitions. A change of magnetic fields can drive quantum phase transitions in the same way as a change in the tunneling amplitude does. Furthermore we study the physics of spin-1 atoms in superlattices deep in the Mott insulating phase when the superlattice decomposes into isolated double-well potentials. Assuming that a small number of spin-1 bosons is loaded in an optical double-well potential, we study single-particle tunneling that occurs when one lattice site is ramped up relative to a neighboring site. Spin-dependent effects modify the tunneling events in a qualitative and quantitative way. Depending on the asymmetry of the double well different types of magnetic order occur, making the system of spin-1 bosons in an optical superlattice a model for mesoscopic magnetism with an unprecedented control of the parameters. Homogeneous and inhomogeneous magnetic fields are applied and the effects of the linear and the quadratic Zeeman shifts are examined. We generalize the concept of bosonic staircases to connected double-well potentials. We show that an energy offset between the two sites of the unit cell in an extended superlattice induces a staircase of single-atom resonances in \nthe same way as in isolated double well. We also examine single-atom resonances in the superfluid regime and find clear fingerprints of them in the superfluid density. We also investigate the bipartite entanglement between the sites and construct states of maximal entanglement. The entanglement in our system is due to both orbital and spin degrees of freedom. We calculate the contribution of orbital and \nspin entanglement and show that the sum of these two terms gives a lower bound for the total entanglement.
The Bose–Hubbard model describing interacting bosons in an optical lattice is reduced to a simple spin-1 XY model with single-ion anisotropy in the vicinity of the Mott phase. We propose a mean-field theory based on a constraint SU(3) pseudo-boson representation on the effective model to study the properties of the superfluid-Mott-insulator phase transition. By calculating the elementary excitation spectra and the average particle number fluctuation in the Brillouin zone center, we find that the energy gaps vanish continuously around ( J XY / J z ) c ≈0.175 and ( J XY / J z ) c ≈0.094 for 2D and 3D cubic lattices respectively, where the superfluid order parameters come up from zero and the Mott insulator state changes into a superfluid state.