Controlling quantum states of light is of central importance to many fields of modern physics. The technology to do so underpins the only feasible means for long-distance quantum communication using quantum-key-distribution, and plays a pivotal role in the application of quantum computing, quantum metrology and investigations of fundamental physics. Motivated by these applications, in this thesis we present a number of experimental results that demonstrate an enhanced level of control over photonic states. First, we tackle one of the most important technological issues currently facing the field, namely the creation of pure multi-photon Fock states from pulsed parametric downconversion. Our technique shows a marked improvement over previous photon sources when employed for quantum information tasks. At a more foundational level, we experimentally examine the properties of quantum correlations in the temporal domain, where our results highlight surprising differences between its spatial-domain counterpart of multipartite entanglement. Finally, we experimentally implement single- and multi-photon quantum walks in the discrete- and continuous-time regimes respectively. Quantum walks have received much attention in recent years due to their vast applicability in quantum information science, especially for quantum simulation and emulation. On this front we use the quantum walk formalism to perform a full experimental simulation of topological phases in a 1-dimensional configuration. Aside from being the first demonstration of topological phases in this regime, our system exhibits unprecedented control over the topological properties in a quantum system. As such we are able to observe the exotic behaviour of trapped bound states, and discover the new phenomenon of paired bound states—a feature unique to periodically driven systems.
Controlling quantum states of light is of central importance to many fields of modern physics. The technology to do so underpins the only feasible means for long-distance quantum communication using quantum-key-distribution, and plays a pivotal role in the application of quantum computing, quantum metrology and investigations of fundamental physics. Motivated by these applications, in this thesis we present a number of experimental results that demonstrate an enhanced level of control over photonic states. First, we tackle one of the most important technological issues currently facing the field, namely the creation of pure multi-photon Fock states from pulsed parametric downconversion. Our technique shows a marked improvement over previous photon sources when employed for quantum information tasks. At a more foundational level, we experimentally examine the properties of quantum correlations in the temporal domain, where our results highlight surprising differences between its spatial-domain counterpart of multipartite entanglement. Finally, we experimentally implement single- and multi-photon quantum walks in the discrete- and continuous-time regimes respectively. Quantum walks have received much attention in recent years due to their vast applicability in quantum information science, especially for quantum simulation and emulation. On this front we use the quantum walk formalism to perform a full experimental simulation of topological phases in a 1-dimensional configuration. Aside from being the first demonstration of topological phases in this regime, our system exhibits unprecedented control over the topological properties in a quantum system. As such we are able to observe the exotic behaviour of trapped bound states, and discover the new phenomenon of paired bound states—a feature unique to periodically driven systems.
Discrete-time quantum walks are among the branches of quantum information and computation. They are platforms for developing quantum algorithms for quantum computers. In addition, due to their universal primitive nature, discrete-time quantum walks have been used to simulate other quantum systems and phenomena that are observed in physics and chemistry. To fully utilize the potentials that the discrete-time quantum walks hold in their applications, control over the discrete-time quantum walks and their properties becomes essential. In this dissertation, we propose two models for attaining a high level of control over the discrete-time quantum walks. In the first one, we incorporate a dynamical nature for the unitary operator performing the quantum walks. This enables us to readily control the properties of the walker and produce diverse behaviors for it. We show that with our proposal, the important properties of the discrete-time quantum walks such as variance would indeed improve. To explore the potential of this proposal, we apply it in the simulations of topological phases in condensed matter physics. With our proposal, we can control the simulations and determine the type of topological phenomena that should be simulated. In addition, we confirm simulations of topological phases and boundary states that can be observed in one-, two- and three-dimensional systems. Finally, we report the emergence of exotic phase structures in form of cell-like structures that contain all types of topological phases and boundary states of certain classes. In our second proposal, we take advantage of resources available in quantum mechanics, namely quantum entanglement and entangled qubits. In this proposal, we use entangled qubits in the structure of a quantum walk and show that by tuning the initial entanglement between these qubits and how these qubits are modified through the walk, one is able to produce diverse behaviors for the quantum walk and control its behavior.
Advances in photonics will lead to breakthroughs in technology with a similar impact to that resulted from the development of electronics. At the quantum level, photons exhibit some unique features, such as non-classical correlations and bosonic bunching. The manipulation of these quanta of light foresee the construction of quantum devices capable of outperforming their classical counterparts in the purposes for which they are built. Despite a significant progress in developing quantum technologies, several unsolved issues certainly remain: Efficient quantification of quantum correlations in a system, and manipulation of multiple photons at once, are two of such hurdles to be overcome. In this thesis, we tackle these two issues and present experimental progress towards their solution. We first explore quantum entanglement between two single-photons and its effect on phases appearing on the system's wavefunction. The observed phases revealed an intimate connection between entanglement––a purely quantum phenomena––and geometric and topological structures of abstract manifolds: A special case of geometric phases was found to increase monotonically with the amount of entanglement in the system, thus serving as an alternative measure of quantum correlations. We then employed a system of three single-photons, and two concatenated entangling gates, as the basis of a quantum simulation protocol: A three-particle quantum simulator, mimicking the entangling evolution of two particles, is used to experimentally demonstrate that the overhead in measuring concurrence––a measure of two-particle entanglement––can be significantly reduced down to measuring only two observables. At this point, increasing the number of photons being handled proved extremely difficult; the low efficiency of photon sources based on parametric downconversion––the gold-standard and only source at-the-time used for multi-photon experiments––imposed a hard limit on countrates and hence the number of photons to be manipulated. We thus then focused on overcoming this obstacle: We studied a solid-state emitter and its performance as a multi-photon source. We employed a quantum dot-cavity system to show that streams of tens of indistinguishable single-photons are produced, whose temporal-to-spatial demultiplexing serves as a novel kind of multi-photon source. A three-photon source was then built and employed in the first demonstration of multi-photon interference from a solid-state source: We implemented a BosonSampling device with a source that is between one and two orders-of-magnitude more efficient than its downconversion counterpart. The main limiting factors for scaling to higher photon numbers were identified to be not intrinsic to the solid-state emitter, but determined by low detector efficiencies and the probabilistic nature of the demultiplexing scheme. Future improvements on these limitations are expected to allow the generation of sources with a higher number of single-photons, a task that has to date remained otherwise impossible.
Since the awareness of entanglement was raised by Einstein, Podolski, Rosen and Schrödinger in the beginning of the last century, it took almost 55 years until entanglement entered the laboratories as a new resource. Meanwhile, entangled states of various quantum systems have been investigated. Sofar, their biggest variety was observed in photonic qubit systems. Thereby, the setups of today's experiments on multi-photon entanglement can all be structured in the following way: They consist of a photon source, a linear optics network by which the photons are processed and the conditional detection of the photons at the output of the network. In this thesis, two new linear optics networks are introduced and their application for several quantum information tasks is presented. The workhorse of multi-photon quantum information, spontaneous parametric down conversion, is used in different configurations to provide the input states for the networks. The first network is a new design of a controlled phase gate which is particularly interesting for applications in multi-photon experiments as it constitutes an improvement of former realizations with respect to stability and reliability. This is explicitly demonstrated by employing the gate in four-photon experiments. In this context, a teleportation and entanglement swapping protocol is performed in which all four Bell states are distinguished by means of the phase gate. A similar type of measurement applied to the subsystem parts of two copies of a quantum state, allows further the direct estimation of the state's entanglement in terms of its concurrence. Finally, starting from two Bell states, the controlled phase gate is applied for the observation of a four photon cluster state. The analysis of the results focuses on measurement based quantum computation, the main usage of cluster states. The second network, fed with the second order emission of non-collinear type II spontaneous parametric down conversion, constitutes a tunable source of a whole family of states. Up to now the observation of one particular state required one individually tailored setup. With the network introduced here many different states can be obtained within the same arrangement by tuning a single, easily accessible experimental parameter. These states exhibit many useful properties and play a central role in several applications of quantum information. Here, they are used for the solution of a four-player quantum Minority game. It is shown that, by employing four-qubit entanglement, the quantum version of the game clearly outperforms its classical counterpart. Experimental data obtained with both networks are utilized to demonstrate a new method for the experimental discrimination of different multi-partite entangled states. Although theoretical classifications of four-qubit entangled states exist, sofar there was no experimental tool to easily assign an observed state to the one or the other class. The new tool presented here is based on operators which are formed by the correlations between local measurement settings that are typical for the respective quantum state.
Light, which is composed of discrete quanta, or photons, is one of the most fundamental concepts in physics. Being an elementary entity, the behaviour of photons is governed by the rules of quantum mechanics. The ability to create, manipulate and measure quantum states of light is not only useful in foundational tests of quantum theory, but also in a wide range of quantum technologies – which aim to utilize non-classical properties of quantum systems to perform tasks not possible with classical resources. Only recently has it been possible to control the properties of number states of light, which have a fixed photon-number. Two-photon states are central to testing fundamental physical theories (such as locality and reality) and the implementation of quantum information technologies. The versatility of photon-pair states is en- abled by the potential entanglement properties it can posses. Thus controlling the correlations between photons is crucial to both pure and applied physics. To produce a single photon, a photon-pair state can be used. Detection of one photon indicates its twin’s existence. Many applications, such as optical quantum computation, require pure indistinguishable single photons. Heralding single pho- tons from a photon-pair will, in general, produce single photons in a mixed quantum state due to correlations within the pair. A common approach to creating photon-pairs is through the nonlinear sponta- neous four-wave mixing interaction in optical fibres. This thesis presents a theoreti- cal and experimental implementation of a scheme to tailor the spectral correlations within the pairs. Emphasis is placed on engineering the two-photon state such that they are completely uncorrelated. Spatial entanglement is naturally avoided due to the discrete nature of the optical fibre modes. Spectral correlations are eliminated by careful choice of dispersion characteristics and conditions. The purity of the photons generated by this scheme is demonstrated by means of two-photon inter- ference from independent sources. We measure a purity of (85.9 ± 1.6)% with no spectral filtering, exhibiting the usefulness of this source for quantum technologies and applications.
The photon is a quantum system that is by nature robust against noise, and fast travelling, providing an ideal information carrier for quantum information science. The field of quantum information science has generated a great deal of interest for both researchers and the public due to the advantages it can have over classical technologies in areas including communication, computing and cryptography. In this thesis, I explore several different ways that photons can be used to realize quantum information advantages and enable quantum technologies, information tasks and fundamental studies of physics. A strong emphasis is placed on their practical implementation in optical experiments, where the challenges of noise, loss and device imperfections must be considered and combated. I utilize spontaneous parametric downconversion-based sources of high-quality single photons, and their polarization, path, and temporal degrees of freedom for encoding quantum information. In my first experimental project, I demonstrate the first violation of noncontextuality with time-polarization intraparticle entangled states encoded in a single photon by implementing a powerful interference-based measurement technique for photonic states. I perform a test of noncontextuality, acquiring a parameter |SCHSH| = 2.744 ± 0.006, which violates the classical bound of 2 by over 110 standard deviations, rigorously certifying both entanglement and contextuality of the system. We propose a new approach for preparing and measuring high-dimensional time-bin states, that overcomes many of the limitations of previous techniques, and demonstrate it for time-bin qubits and qutrits. In the next experimental project, I investigate the topic of universal cloning in quantum steering-with cloning and steering being two fundamental aspects of quantum physics deeply involved in the security of quantum protocols. I report the first experimental demonstration of cloned quantum steering, showing a simultaneous violation in a steering test by two clones made from one part of an entangled pair of photons. This provides a conclusive result on the question of whether the cloning of quantum steering is possible. We also present theoretical results that clarify our understanding of cloned steering for qubits: we find a no-go theorem where quantum steering can only be copied by a qubit universal cloning machine for 2 and 3 clones, and a monogamy relation where for N clones, steering is only possible if a minimum of N + 1 measurements are performed on each clone. I discuss the field of random number generation, and study how quantum physics allows for certifiably unpredictable random sequences, without needing complete trust in all of the physical devices, offering high levels of security over classical approaches. I report the first discrete-variable detection-loophole-free implementation of one-sided device-independent randomness expansion of certified random bits, based on the quantum steering task. These results illustrate an approach to secure randomness with greater tolerance to noise and loss compared to Bell test-based protocols. The final experimental project looks at quantum autoencoders, which are a quantum machine learning tool that we investigate for the purpose of denoising quantum states. I model and simulate a denoising quantum autoencoder which compresses ququarts into a qubit space and reconstructs noise-reduced ququart states. I construct an experimental apparatus that implements this device, and demonstrate quantum state tomography of ququart states, and the training of the autoencoder.
The quantum description of light offers a unique set of optical effects that has led to promising applications beyond those described by classical physics. Although well-defined quantum states of light do not persist in typical classical environments, phenomena such as entanglement often enhance optical approaches to communication, measurement, and sensing. With the emergence of new tasks in classical and quantum optical technology, new tools are required that must be specifically engineered including the generation of quantum states. This thesis is concerned with three principle tasks in engineering and implementing entangled photonic states. First, the use of frequency anti-correlated and polarization entangled two-photon states generated during spontaneous parametric down conversion (SPDC) to precisely evaluate optical delays with quantum interferometry is demonstrated in a realistic commercially available optical telecommunication device. Second, the study of correlated orbital angular momentum (OAM) states for efficient object identification is presented. Finally, experimental efforts towards the development of sources for entangled weak coherent states are discussed. The generation of broadband entangled states leading to well-defined second order interference patterns is a necessary step for the application of low coherence quantum interferometry as a metrological device. The flexibility of non-uniformly chirped periodically poled nonlinear crystals offers a rich set of tools for precise state engineering. The experimental evaluation of a broadband source of polarization entanglement is presented. In addition, design considerations for applications that require optimized quantum interference features are discussed along with a numerical investigation of the limits of quantum interferometry with even order dispersion cancellation. We present an experimental demonstration of correlated OAM sensing exploiting the two-dimensional and correlated nature of states produced during SPDC projected onto the OAM basis. Efficient object recognition through the identification of azimuthal symmetries of arbitrary objects is achieved by observing the full two-photon joint OAM spectrum and focusing on non-conserved OAM components not found in the natural OAM spectrum of SPDC. Finally, quantum key distribution (QKD) is currently the most successful quantum optical application; however, a limiting trade off between the achievable rates and distances confines the approach to niche applications. The generation of entangled coherent states has been proposed to transition QKD into a new regime that would set aside single photons and two-photon entangled states for higher intensity coherent pulses. The key technical limitation that has prohibited the demonstration of such states is a reliable source of single-photon cross phase modulation. The plausibility and experimental efforts towards creating such an environment in a solid state device is presented.