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Study of multiple optical transitions in 87Rb using laser diodes

C. L. J. Newton, H. G. Robinson

Published Dec 1, 1982• 1 citation
OpenAlex

Abstract

Recent work with laser diodes has indicated their potential usefulness in optically pumping atomic frequency standards. We consider various optical pumping schemes for 87-Rb incorporating such light sources at two D1 frequencies for experimental situations of either evacuated wall-coated cells or atomic beams. Numerical integration of rate equations governing the level populations with arbitrary pumping light choices of intensity, D1 hyperfine transition(s), and polarization and subsequent calculation of scattered light provide a simplified O-O hyperfine signal analysis.

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The time evolution of populations of the ground state hyperfine Zeeman levels of 87 Rb atoms is analyzed using the Runge—Kutta method for the case that a rubidium beam is optically pumped, under different conditions of polarization, with a weak monochromatic laser and an 87 Rb lamp. On the base of the results above, the least estimated laser and 87 Rb lamp power for the best population inversion is obtained, aiding further investigations.

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On the efficiency of laser pumping of hyperfine structure sublevels of Rubidium-87 and Cesium-133 atoms

A. I. Magunov, Vitalii G Pal'chikov

The evolution of the hyperfine structure magnetic sublevel populations of 87 Rb and 133 Cs atoms in resonant linearly polarized laser fields is theoretically analyzed. Analytical expressions are obtained for stationary populations of the magnetic sublevels of the ground state 5 2 S 1/2 F g = 1, F f = 2 in 87 Rb and 6 2 S 1/2 F g = 3, F f = 4 in 133 Cs under optical pumping at the F g ↔ F e = F g and F f ↔ F e = F f transitions of the D 2 lines ( n 2 S 1/2 n 2 P 3/2 ) versus the initial populations. The characteristic population stabilization time are obtained by numerical solution for the density matrix equations, depending on the intensity of the laser fields and the detuning of the optical resonance. It is shown that the alternation of the polarization direction of the laser field at the transition F f ↔ F e = F f almost completely transfers atoms to the lower sublevel of the "clock" M1 transition F g M = 0 ↔ F f M = 0 in rubidium and cesium frequency standards, which proportionally increases the signal of the recording system.

Journal of Physics Conference Series•Sep 1, 2021•0 citations
Recent work with laser diodes has indicated their potential usefulness in optically pumping atomic frequency standards. We consider various optical pumping schemes for 87-Rb incorporating such light sources at two D1 frequencies for experimental situations of either evacuated wall-coated cells or atomic beams. Numerical integration of rate equations governing the level populations with arbitrary pumping light choices of intensity, D1 hyperfine transition(s), and polarization and subsequent calculation of scattered light provide a simplified O-O hyperfine signal analysis.
In this paper, we present our studies on double resonance using atomic 87Rb in a wall-coated cell, in view of applications in a laser-pumped Rb atomic frequency standard. We study the systematic clock frequency shifts in a wall-coated cell, such as light shift, microwave power shift [11, 12] and shift due to cell temperature [13] (for the cell body, and for the Rb reservoir, also called the cell stem). We also report on our clock stability measurement using the wallcoated cell in DR scheme, and discuss the influence of the shift parameters first on the frequency stability of the clock.
It is experimentally demonstrated that, using diode lasers for optical pumping and RF /spl pi/-pulses for population transfer, nearly all of the ground state Rb atoms in a vapor cell can be concentrated into one of the two M/sub F/ = 0 sublevels. The fractional population difference /spl Delta/ between the two M/sub F/ = 0 levels can be made as high as 1. This should result in a very significant improvement (about a factor of 100) in the S/N over the conventional discharge-lamp-pumped rubidium frequency standards (RFSs). This would lead to a substantial improvement in the short-term stability of the RFS. This is a pulsed population transfer scheme. The microwave interrogation takes place in the absence of strong pumping light. This has the potential for eliminating the light shift and thereby improving the long-term frequency stability of a an RFS.>
The /sup 87/Rb cell frequency standard, optically pumped by a laser diode, is of great interest in the development of high short-term stability oscillators. We report experiments performed on a rubidium cell prototype aiming at evaluate the transfer of the laser noise to the hyperfine clock transition via the light shift effect, which appears to be the main contribution to the observed short term frequency stability in this kind of standard. Pulsed optical pumping will also be examined in order to strongly reduce the light shift effect and to achieve the theoretical limit never approached up to now despite the strong detected microwave signals.
The evolution of the hyperfine structure magnetic sublevel populations of 87 Rb and 133 Cs atoms in resonant linearly polarized laser fields is theoretically analyzed. Analytical expressions are obtained for stationary populations of the magnetic sublevels of the ground state 5 2 S 1/2 F g = 1, F f = 2 in 87 Rb and 6 2 S 1/2 F g = 3, F f = 4 in 133 Cs under optical pumping at the F g ↔ F e = F g and F f ↔ F e = F f transitions of the D 2 lines ( n 2 S 1/2 n 2 P 3/2 ) versus the initial populations. The characteristic population stabilization time are obtained by numerical solution for the density matrix equations, depending on the intensity of the laser fields and the detuning of the optical resonance. It is shown that the alternation of the polarization direction of the laser field at the transition F f ↔ F e = F f almost completely transfers atoms to the lower sublevel of the "clock" M1 transition F g M = 0 ↔ F f M = 0 in rubidium and cesium frequency standards, which proportionally increases the signal of the recording system.