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Bulletin of the American Physical Society

Decoherence-Free Control of Large Spin-Atomic Systems with Coherent Electromagnetic Fields

Seth Merkel, Souma Chaudhury, Poul Jessen, Ivan Deutsch

Published May 30, 2008• 0 citations
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The control of light-matter interaction at the quantum level usually requires coherent laser fields. But already an exchange of virtual photons with the electromagnetic vacuum field alone can lead to quantum coherences, which subsequently suppress spontaneous emission. We demonstrate such spontaneously generated coherences (SGC) in a large ensemble of nuclei operating in the x-ray regime, resonantly coupled to a common cavity environment. The observed SGC originates from two fundamentally different mechanisms related to cooperative emission and magnetically controlled anisotropy of the cavity vacuum. This approach opens new perspectives for quantum control, quantum state engineering and simulation of quantum many-body physics in an essentially decoherence-free setting.
We perform a first-principles derivation of the general master equation to study the non-Markovian dynamics of a two-level atom (2LA) interacting with an electromagnetic field (EMF). We use the influence functional method, which can incorporate the full back reaction of the field on the atom, while adopting Grassmannian variables for the 2LA and the coherent-state representation for the EMF. We find exact master equations for the cases of a free quantum field and a cavity field in the vacuum. In response to the search for mechanisms to preserve maximal coherence in quantum computations in ion trap prototypes, we apply these equations to analyze the decoherence of a 2LA in an EMF, and find that decoherence time is close to relaxation time. This is at variance with the claims by authors who studied the same system but used a different coupling model. We explain the source of difference and argue that, contrary to common belief, the EMF, when resonantly coupled to an atom, does not decohere it as efficiently as a bath does on a quantum Brownian particle. The master equations for non-Markovian dynamics derived here are expected to be useful for exploring new regimes of 2LAEMF interaction, which is becoming physically important experimentally.