Spin coherence excitation and rephasing with optically shelved atoms
Byoung Seung HAM, M. S. Shahriar, M. K. Kim +1 more
We investigate the use of resonant optical Raman pulses to excite and rephase ground state spin coherences via the partial storage or shelving of atoms. Unlike direct-rf-excited spin echoes or off-resonant Raman echoes, the resonant Raman optical field efficiently excites and rephases the spin coherence using \ensuremath{\pi} and 2\ensuremath{\pi} pulses, respectively. In a crystal of ${\mathrm{Pr}}^{3+}$ doped ${\mathrm{Y}}_{2}{\mathrm{SiO}}_{5},$ we experimentally observe spin echo efficiency as high as 46% of the free induction decay signal.
Physical review. B, Condensed matter•Nov 1, 1998•57 citations