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Acta Physica Polonica A

Zeeman Coherences Narrowing due to Ramsey Effects Induced by Thermal Motion of Rubidium Atoms

Z. D. Grujić, Marina M. Mijailović, Bratimir M. Panic, Milan Minic, A. Kovačević, M. Obradović, B. M. Jelenković, S. Cartaleva

Published Nov 1, 2007• 1 citation
Publisher

Abstract

We investigated effects of spatially separated laser fields on amplitudes and widths of electromagnetically induced transparency in M-type atomic system.We have shown narrowing of the electromagnetically induced transmission resonance and therefore enhancement of medium non-linearities that can be explained by diffusion-induced Ramsey narrowing.Depending on the polarization of two laser beams, narrow probe Hanle transmission resonance changes its sign in respect of the profile obtained when the pump laser beam is off.

DOI
10.12693/aphyspola.112.799

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Physica Scripta•Sep 1, 2014•1 citation
We investigated effects of spatially separated laser fields on amplitudes and widths of electromagnetically induced transparency in M-type atomic system.We have shown narrowing of the electromagnetically induced transmission resonance and therefore enhancement of medium non-linearities that can be explained by diffusion-induced Ramsey narrowing.Depending on the polarization of two laser beams, narrow probe Hanle transmission resonance changes its sign in respect of the profile obtained when the pump laser beam is off.
Experimental and theoretical investigations show the strong effect of the pump beam, spatially separated from the probe beam, on the probe's electromagnetically induced absorption (EIA) and nonlinear magneto-optical rotation (NMOR). Linearly polarized pump and probe laser beams are locked to the Fg = 2 → Fe = 3 transition of the 87Rb D2 line and pass a vacuum Rb gas cell coaxially. We show that the observed narrowing of EIA and NMOR resonances is due to the Ramsey effect. Linewidths of the resonances decrease when the size of the dark region between pump and probe lasers increases. Variation of the angle between pump and probe linear polarizations strongly influences the phases of atomic coherences generated by the pump beam and consequently the line-shapes of the probe EIA and NMOR resonances. Complete change of the resonance sign is possible if the phases of the ground state coherences, Δmg = 2, are altered by π. The central EIA fringe becomes less pronounced if the probe intensity increases, due to the larger probe contribution to atomic evolution. Ramsey-like interference is a manifestation of the evolution of ground state Zeeman coherences, required for EIA, in the dark region in the presence of a small magnetic field.
Nonlinear magneto-optical rotation (NMOR) of linearly polarized light, resonant to the Fg = 2 → Fe = 1 atomic transition of D1 line of 87Rb is investigated experimentally, by applying spatially separated laser fields in the Rb vacuum cell. In our experiment, the probe laser beam propagates through the center of the pump laser beam, which has the shape of a hollow cylinder. We have measured the rotation of the probe laser beam polarization with respect to the incident polarization, as a function of the external magnetic field, parallel to the laser beam propagation. We show substantial narrowing of the resonance if the pump beam, with the same linear polarization, is present. The opposite direction of the probe rotation was obtained when the pump laser beam polarization is orthogonal to the probe laser beam polarization.
We investigate the evolution of the atomic coherence between Zeeman sublevels with $\ensuremath{\Delta}{m}_{F}=2$ in the region between pump and probe laser beams, in a Rb vapor cell using the Hanle configuration. The transmission of the probe beam, placed inside the hollow pump beam, shows the narrowing of the Hanle resonance (at external magnetic field B=0B=0B=0) by Ramsey fringes whose separation from the central peak depends on the distance between the beams. The temporal evolution of the pump induced alignment is evident from the changes of the probe transmission spectra with increasing the angle between linear polarizations of each beam. Experimental results are in agreement with the results of the model which calculates probe fluorescence by solving time-dependent optical Bloch equations, from the time when atom enters the pump beam to the time when it leaves the probe beam. The results for total excited state populations were averaged over atomic velocities distribution.
In this paper, we present a theoretical model for studying the interaction between linearly polarized laser light and near-degenerated Zeeman sublevels for a multiple V-type atomic system of $^{2}S_{1∕2}{F}_{g}=2\ensuremath{\rightarrow}^{2}P_{3∕2}{F}_{e}=3$ transition in 87Rb^{87}\mathrm{Rb}87Rb. We have calculated the laser absorption in a Hanle configuration, as well as the amplitudes and the widths of electromagnetically induced absorption (EIA) in the range of laser intensities from 0.01to40mW∕cm20.01\phantom{\rule{0.3em}{0ex}}\text{to}\phantom{\rule{0.3em}{0ex}}40\phantom{\rule{0.3em}{0ex}}\mathrm{mW}∕{\mathrm{cm}}^{2}0.01to40mW∕cm2. Our results, showing nonvanishing EIA amplitude, a nonmonotonic increase of the EIA width for the increase of laser intensity, and pronounced shape differences of the Hanle EIA curves at different laser intensities, are in good agreement with recent experimental results. We have found that the EIA behaves differently than the electromagnetically induced transparency (EIT) as a function of the laser intensity. Both the amplitude and width of the EIA have narrow maximums at 1to2mW∕cm21\phantom{\rule{0.3em}{0ex}}\text{to}\phantom{\rule{0.3em}{0ex}}2\phantom{\rule{0.3em}{0ex}}\mathrm{mW}∕{\mathrm{cm}}^{2}1to2mW∕cm2. We have shown the strong influence of Doppler broadening of atomic transition on Hanle resonances and have suggested the explanation of it.
We present a theoretical model for electromagnetically induced transparency (EIT) in vapor that incorporates atomic motion and velocity-changing collisions into the dynamics of the density-matrix distribution. Within a unified formalism, we demonstrate various motional effects, known for EIT in vapor: Doppler broadening of the absorption spectrum; Dicke narrowing and time-of-flight broadening of the transmission window for a finite-sized probe; diffusion of atomic coherence during storage of light and diffusion of the light-matter excitation during slow-light propagation; and Ramsey narrowing of the spectrum for a probe and pump beams of finite size.
We experimentally studied the temporal evolution of Zeeman electromagnetically induced transparency (EIT) resonances induced by the laser resonant to hyperfine transition of 87Rb in a rubidium buffer gas cell. We simultaneously modulated the laser beam intensity and polarization to achieve the repeated interaction of the laser beam with coherently prepared atoms. Our cell was placed in a homogenous magnetic field to obtain the Larmor precession of the phase of coherences. The weak laser beam was used to probe the atoms at the end of the Ramsey sequence. We measured the transparency of the probe pulse at different magnetic fields for a given excitation pulse and the period of free evolution of Zeeman coherences in the dark. From these data, we reconstructed the temporal evolution of EIT resonances. The Ramsey fringes that appeared on the EIT curves at the beginning of the second probing pulse disappeared at later moments due to various decay processes.