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Applied Physics Letters

Enhanced four-wave mixing by atomic coherence in a Pr3+:Y2SiO5 crystal

Hai-Hua Wang, Dun-Mao Du, Yun-Fei Fan, Aijun Li, Lei Wang, Xiaogang Wei, Zhi‐Hui Kang, Yun Jiang, Jin‐Hui Wu, Jin-Yue Gao

Published Dec 8, 2008• 22 citations
Publisher

Abstract

We experimentally demonstrate an enhanced four-wave mixing (FWM) based on atomic coherence in a Pr3+:Y2SiO5 crystal. By employing coherent population return and fractional stimulated Raman adiabatic passage to prepare maximum atomic coherence in the crystal, an efficient FWM signal can be generated. By measuring the generated FWM signal, the time-dependent atomic coherence is monitored. Such an enhanced FWM in solids may have practical applications in nonlinear optics and laser spectroscopy.

DOI
10.1063/1.3043683

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We experimentally demonstrate an enhanced four-wave mixing (FWM) based on atomic coherence in a Pr3+:Y2SiO5 crystal. By employing coherent population return and fractional stimulated Raman adiabatic passage to prepare maximum atomic coherence in the crystal, an efficient FWM signal can be generated. By measuring the generated FWM signal, the time-dependent atomic coherence is monitored. Such an enhanced FWM in solids may have practical applications in nonlinear optics and laser spectroscopy.
We report on the experimental implementation of stimulated Raman adiabatic passage (STIRAP) in a Pr3+:Y2SiO5 crystal. Our data provide clear and striking proof for nearly complete population inversion between hyperfine levels in the Pr3+ ions. The transfer efficiency was monitored by absorption spectroscopy. Time-resolved absorption measurements serve to monitor the adiabatic population dynamics during the STIRAP process. Efficient transfer is observed for negative pulse delays (STIRAP), as well as for positive delays. We identify the latter by an alternative adiabatic passage process.
Atomic coherence is the interaction process between light and atoms, that is one or more coherent fields couple the different atomic states and cause the quantum interference between the different transition channels. Atomic coherence has led to many interesting and unexpected consequences, such as the Hanle effects, electromagnetically induced transparency (EIT), coherence population trapping (CPT), stimulated Raman adiabatic passage (STIRAP), spontaneous emission control, resonant enhancement of optical nonlinearity, slow and superluminal light propagation, quantum light storage, etc. In which, light storage based on atomic coherence plays an important role in the coherent control of light pulse information. In this chapter, we present some previous works on atomic coherence and optical storage. Firstly, we present the storage and recovery of light pulse based on F-STIRAP, which is fundamentally different from the conventional EIT-based process. Secondly, we present the applications of light storage based on EIT in a Pr3+:Y2SiO5 crystal, which includes the erasure of stored optical information, all-optical routing by light storage, and the coherent control of double light pulses. At last, we propose theoretically and demonstrate experimentally a method to control the atomic coherence by a STIRAP or F-STIRAP process.
We demonstrate coupling of light resonant to transition between two excited states of rubidium and long-lived ground-state atomic coherence. In our proof-of-principle experiment a nonlinear process of four-wave mixing is used to achieve light emission proportional to independently prepared ground-state atomic coherence. Strong correlations between stimulated Raman-scattering light heralding the generation of ground-state coherence and the four-wave mixing signal are measured and shown to survive the storage period, which is promising in terms of quantum memory applications. The process is characterized as a function of laser detunings.
We have experimentally demonstrated the enhancement of coherent Raman scattering in Rb\mathrm{Rb}Rb atomic vapor by exciting maximal atomic coherence with fractional stimulated Raman adiabatic passage. Experimental results are in good agreement with numerical simulations. The results support the possibility of increasing the sensitivity of coherent anti-Stokes Raman spectroscopy by preparing maximal atomic or molecular coherence using short pulses.
We observe experimentally huge enhanced four-wave mixing based on Raman resonance in an 85Rb atomic vapor system. With the decrease of coupling field power or the increase of experimental temperature, the signal tends to be narrowed down in linewidth, and be basically the same spectrum as the stimulated Raman spectroscopy. It is found that the macroscopic polarization interference effect plays a crucial role in determining the nonlinear spectra. Further more, in the Doppler-broadened Λ-type energy level system, there is a strong relationship among electromagnetically induced transparency, four-wave mixing and stimulated Raman spectroscopy. The sharp transparent window in electromagnetically induced transparency can be interpreted as the suppression of Raman gain on the linear absorption of the probe field. However, the four-wave mixing signal is a new field generated by the atomic vapor system, and it comes from the Raman gain which is affected and modified by the absorption and dispersion of the nonlinear optical medium. It shows that in a Λ-type Doppler-broadened system, in essence, both the electromagnetically induced transparency and enhanced four-wave mixing stem from stimulated Raman scattering based on the third-order nonlinear processes, just the spectra of which are from different ways and objects of detection.