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Bulletin of the American Physical Society

Large fractional delay for slow and stored light in atomic vapor

Irina V. Novikova, David Phillips, Ronald Lee Walsworth

Published Jun 7, 2007• 0 citations
OpenAlex

Abstract

Conclusions • Control and signal fields have orthogonal linear polarizations. • Two AOMs allow independent control of Probe and Control field intensities. • PZT allows adjustment of phase difference, , between control and probe fields. • Use gain and pulse recompression to localize pulse in medium • Turn off control field to store pulse as atomic coherence. • After storage interval, retrieve using constant control field. Fractional delay > 20

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Conclusions • Control and signal fields have orthogonal linear polarizations. • Two AOMs allow independent control of Probe and Control field intensities. • PZT allows adjustment of phase difference, , between control and probe fields. • Use gain and pulse recompression to localize pulse in medium • Turn off control field to store pulse as atomic coherence. • After storage interval, retrieve using constant control field. Fractional delay > 20
This thesis deals with the study of propagation effects experienced by weak light pulses as they propagate in atomic media driven by strong pulses. We explore both the ultra-short and long pulse regime and investigate the phenomena that arise at these different time scales. In the short pulse regime, a strongly driven two level atomic system presents transient light shifts, and non-adiabatic transitions occur between these adiabatic levels. We have studied a method to probe these light shifts in real time by propagating a weak probe through the medium. The light shifts enrich the spectrum of the probe and the probe gets shaped as a result. In this way a strongly driven two-level system can act as an active pulse shaper, and can introduce oscillations in the temporal profile of an ultra-short pulse at a time scale shorter than the pulse duration. We also show that by driving the system with two time delayed non-resonant strong fields, the non-adiabatic effects can be rendered phase dependent. This gives very sensitive phase control of the excited state population and can be used to formulate new techniques in interferometry. In the long pulse regime we present a new method of slowing light that can be realized in a double two-level system interacting with two orthogonally polarized light pulses that propagate along different axis. Spatio-temporal dependence of the total polarization induces a grating in the ground Zeeman coherence. The stronger of the two fields (the control field) is diffracted from this grating into the direction of the weak probe field compensating for the absorption of this latter field. A transparency window is thus created in the absorption spectrum of the probe leading to the slowing down of light. The transparency window exhibits characteristics similar to the one obtained by EIT (electromagnetic induced transparency) method. However, the important difference between our method and the traditional EIT method, is that ours doesn't rely on realizing dark state in the system. This may open the possibility of slowing down light in more complex atomic media. Moreover, when the linear absorptive response of the medium is cancelled in this manner, the nonlinear response becomes more important. In the situation where fields propagate in the same direction and have same frequency, two regimes have been investigated. For small optical depths, the effective susceptibility behaves as chi_lin exp[2 i phi] (with phi the phase difference between two fields). This renders phase control of the medium response, and the medium can be changed from an absorber to an amplifier, with normal or anomalous dispersion, by adjusting the relative phase phi.  In the regime of large optical thickness, phase saturation takes place and the effective susceptibility turns into chi_lin*, changing an absorber into an amplifier without effecting the dispersive response (chi_lin is linear susceptibility).
Electromagnetically-induced transparency (EIT) of atomic medium interacting with two laser beams can exhibit effects of reciprocal influence of both beams on optical properties of the medium. If the probe beam reaches instantaneous intensity comparable to that of the control beam, considerable energy is transferred to the latter. Resulting increase in the control-beam intensity temporarily modifies EIT conditions and consequently affects propagation of probe-beam pulses. The effect is particularly strong in atomic media exhibiting significant dissipation of radiation energy due to relaxation processes efficiently counteracting the optical pumping. Coherent interaction of atoms with both beams causes reduction of dissipation of the control beam (reciprocal EIT conditions). Our experiments with hot rubidium vapor demonstrate the possibility of dual control over slow propagation of light pulses in such media. Besides the well-known dependence on input control-beam intensity, the delays of output probe pulses depended significantly also on the energy of input probe pulses. Moreover, for relatively short input pulses, very specific shape of output pulses was observed, invariant in wide ranges of input probe pulse energies and control-beam intensities. The shapes of the output pulses were also the same for short input pulses of different shapes as well as for pulses temporarily stored in the medium by switching off the control beam during their propagation.