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Bulletin of the American Physical Society

Observation of long range Rydberg blockade

Mark E. Saffman

Published May 22, 2009• 0 citations
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Observation of ultralong range Rydberg molecules

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Bulletin of the American Physical Society•May 21, 2009•0 citations
We study the long-range interaction of a single ion with a highly excited ultracold Rydberg atom and report on the direct observation of an ion-induced Rydberg excitation blockade mediated over tens of micrometer distances. Our hybrid ion-atom system is directly produced from an ultracold atomic ensemble via near-threshold photoionization of a single Rydberg excitation, employing a two-photon scheme that is specifically suited for generating a very low-energy ion. The ion's motion is precisely controlled by small electric fields, which allows us to analyze the blockade mechanism for a range of principal quantum numbers. Finally, we explore the capability of the ion as a high-sensitivity, single-atom-based electric field sensor. The observed ion-Rydberg-atom interaction is of current interest for entanglement generation or studies of ultracold chemistry in hybrid ion-atom systems.
The Rydberg blockade is a key ingredient for entangling atoms in arrays. However, it requires atoms to be spaced well within the blockade radius, which limits the range of local quantum gates. Here we break this constraint using Floquet frequency modulation, with which we demonstrate Rydberg-blockade entanglement beyond the traditional blockade radius and show how the enlarged entanglement range improves qubit connectivity in a neutral atom array. Further, we find that the coherence of entangled states can be extended under Floquet frequency modulation. Finally, we realize Rydberg anti-blockade states for two sodium Rydberg atoms within the blockade radius. Such Rydberg anti-blockade states for atoms at close range enables the robust preparation of strongly-interacting, long-lived Rydberg states, yet their steady-state population cannot be achieved with only the conventional static drive. Our work transforms between the paradigmatic regimes of Rydberg blockade versus anti-blockade and paves the way for realizing more connected, coherent, and tunable neutral atom quantum processors with a single approach.
We propose an experiment to demonstrate a blockade mechanism caused by long-range anisotropic interactions in an ultracold dipolar gas composed of the recently observed ``butterfly'' Rydberg molecules. At the blockade radius, the strong intermolecular interaction between two adjacent molecules shifts their molecular states out of resonance with the photoassociation laser, preventing their simultaneous excitation. When the molecules are prepared in a quasi-one-dimensional (Q1D) trap, the interaction's strength can be tuned via a weak external field. The molecular density thus depends strongly on the angle between the trap axis and the field. The available Rydberg and internal molecular states provide a wide range of tunability.