We study a system of neutral atoms trapped in a three-dimensional optical lattice suitable for the encoding, initialization and manipulation of atomic qubits. The qubits are manipulated by applied electromagnetic fields interacting with dipole moments of the atoms via light shifts, Raman transitions, Zeeman shifts, and microwave transitions. Our lattice is formed by three orthogonal one-dimensional lattices, which have different frequencies so that interference terms average to zero. This geometry allows considerable freedom in designing the component one-dimensional lattices, so that they provide not only confinement but also independent control in each dimension. Our atomic qubits are initialized from a laser-cooled atomic sample by Raman sideband cooling in individual lattice potential wells. We have demonstrated accurate and robust one-qubit manipulation using resonant microwave fields. In practice such control operations are always subject to errors, in our case spatial inhomogeneities in the microwave Rabi frequency and the light shifted qubit transition frequency. Observation of qubit dynamics in near real time allows us to minimize these inhomogeneities, and therefore optimize qubit logic gates. For qubits in the lattice, we infer a fidelity of 0.990(3) for a single pi-pulse. We have also explored the use of NMR-type pulse techniques in order to further reduce the effect of errors and thus improve gate robustness in the atom/lattice system. Our schemes for two-qubit quantum logic operations are based on controlled collisional interactions. We have experimented with two schemes in order to probe these collisions. The first involves manipulation of the center-of-mass wavepackets of two qubits in a geometry corresponding to two partially overlapping Mach-Zender interferometers. Unfortunately, this scheme has proven extremely sensitive to phase errors, as the wavepackets are moved by the optical lattice. The other scheme starts with two qubits in spatially separated traps, and utilizes microwaves to drive one or both qubits into a third trap in-between the two qubits. Once the wavepackets overlap, the collisions create a large energy shift which can be probed spectroscopically.
We study a system of neutral atoms trapped in a three-dimensional optical lattice suitable for the encoding, initialization and manipulation of atomic qubits. The qubits are manipulated by applied electromagnetic fields interacting with dipole moments of the atoms via light shifts, Raman transitions, Zeeman shifts, and microwave transitions. Our lattice is formed by three orthogonal one-dimensional lattices, which have different frequencies so that interference terms average to zero. This geometry allows considerable freedom in designing the component one-dimensional lattices, so that they provide not only confinement but also independent control in each dimension. Our atomic qubits are initialized from a laser-cooled atomic sample by Raman sideband cooling in individual lattice potential wells. We have demonstrated accurate and robust one-qubit manipulation using resonant microwave fields. In practice such control operations are always subject to errors, in our case spatial inhomogeneities in the microwave Rabi frequency and the light shifted qubit transition frequency. Observation of qubit dynamics in near real time allows us to minimize these inhomogeneities, and therefore optimize qubit logic gates. For qubits in the lattice, we infer a fidelity of 0.990(3) for a single pi-pulse. We have also explored the use of NMR-type pulse techniques in order to further reduce the effect of errors and thus improve gate robustness in the atom/lattice system. Our schemes for two-qubit quantum logic operations are based on controlled collisional interactions. We have experimented with two schemes in order to probe these collisions. The first involves manipulation of the center-of-mass wavepackets of two qubits in a geometry corresponding to two partially overlapping Mach-Zender interferometers. Unfortunately, this scheme has proven extremely sensitive to phase errors, as the wavepackets are moved by the optical lattice. The other scheme starts with two qubits in spatially separated traps, and utilizes microwaves to drive one or both qubits into a third trap in-between the two qubits. Once the wavepackets overlap, the collisions create a large energy shift which can be probed spectroscopically.
Neutral atoms are promising candidates to store and manipulate quantum information. In this thesis we examine several problems related to the control of neutral atoms for quantum computation and simulation. In the first problem we show how the transport of atoms in an optical lattice can be controlled through variation of the polarization of the optical lattice and the application of global microwave pulses. This type of control control is a first step in many of the schemes for quantum computation and quantum simulation. We show that with the available tools for global control, the synthesis of any unitary transformation, consistent with translational invariance, may be performed and provide an explicit method for carrying this out. In the second problem, we study a spectroscopic method for probing atomic interactions that may form the basis for two-qudit quantum logic gates. The confinement of atoms required to perform quantum computation can strongly affect how they interact. Probing the nature of those confinement-induced effects is a first step towards quantum computing with neutral atoms. Transport of the atoms to overlapping wells is achieved through microwave pulses that drive population between hyperfine levels in a lin-perp-lin polarization-gradient lattice. By measuring the amount of population transferred into certain excited states, we can detect changes in the spectrum of the two-atom system induced by the interaction. In the third problem, we consider a cloud of cold atoms driven by both microwave and radio-frequency magnetic fields. The large number of spin sublevels available in individual atoms makes them candidates for a qudit-based quantum computer. Because the applied fields that drive the system may be inhomogeneous, the collection of atoms forms an ensemble of different qudits. Borrowing ideas developed for NMR control, we show how to drive the ensemble through a given evolution. We show that even in the presence of large experimental errors, state preparation may be achieved with high fidelities. We also show that intentionally applied variations in spatial magnetic fields can be used to synthesize different states in different regions of space.
The present work investigates the state-selective transport of single neutral cesium atoms in a one-dimensional optical lattice. It demonstrates experimental applications of this transport, including a single atom interferometer, a quantum walk and controlled two-atom collisions. The atoms are stored one by one in an optical lattice formed by a standing wave dipole trap. Their positions are determined with sub-micrometer precision, while atom pair separations are reliably inferred down to neighboring lattice sites using real-time numerical processing. Using microwave pulses in the presence of a magnetic field gradient, the internal qubit states, encoded in the hyperfine levels of the atoms, can be separately initialized and manipulated. This allows us to perform arbitrary single-qubit operations and prepare arbitrary patterns of atoms in the lattice with single-site precision. Chapter 1 presents the experimental setup for trapping a small number of cesium atoms in a one-dimensional optical lattice. Chapter 2 is devoted to fluorescence imaging of atoms, discussing the imaging setup, numeric methods and their performance in detail. Chapter 3 focuses on engineering of internal states of trapped atoms in the lattice using optical methods and microwave radiation. It provides a detailed investigation of coherence properties of our experimental system. Finally manipulation of individual atoms with almost single-site resolution and preparation of regular strings of atoms with predefined distances are presented. In Chapter 4, basic concepts, the experimental realization and the performance of the state-selective transport of neutral atoms over several lattice sites are presented and discussed in detail. Coherence properties of this transport are investigated in Chapter 5, using various two-arms single atom interferometer sequences in which atomic matter waves are split, delocalized, merged and recombined on the initial lattice site, while the interference contrast and the accumulated phase difference are measured. By delocalizing a single atom over several lattice sites, possible spatial inhomogeneities of fields along the lattice axis in the trapping region are probed. In Chapter 6, experimental realization of a discrete time quantum walk on a line with single optically trapped atoms is presented as an advanced application of multiple path quantum interference in the context of quantum information processing. Using this simple example of a quantum walk, fundamental properties of and differences between the quantum and classical regimes are investigated and discussed in detail. Finally, by combining preparation of atom strings, position-dependent manipulation of qubit states and state-selective transport, in Chapter 7, two atoms are deterministically brought together into contact, forming a starting point for investigating two-atom interactions on the most fundamental level. Future prospects and suggestions are finally presented in Chapter 8.
Ultracold neutral atoms confined in optical dipole traps have important applications in quantum computation and information processing, quantum simulators of interacting-many-body systems and atomic frequency metrology. While optical dipole traps are powerful tools for cold atom experiments, the energy level structures of the trapped atoms are shifted by the trapping field, and it is important to characterize these shifts in order to accurately manipulate and control the quantum state of the system.\n\nIn order to measure the light shifts, we have designed a system that allows us to reliably trap individual 87Rb atoms. A non-destructive detection technique is employed so that the trapped atoms can be continuously observed for over 100 seconds. Single atom spectroscopy, trap frequency measurements, and temperature measurements are performed on single atoms in a single focus trap and small number of atoms in a 1D optical lattice in order to characterize the trapping environment, the perturbed energy level structures, and the probe-induced heating.\n\nIn the second part of the thesis, we demonstrate deterministic delivery of an array of individual atoms to an optical cavity and selective addressability of individual atoms in a 1D optical conveyor, which serves as a potential candidate for scalable quantum information processing. The experiment is extended to a dual lattice system coupled to a single cavity with the capability of independent lattice control and addressability. The mutual interactions of atoms in different lattices mediated by a common cavity field are demonstrated. A semi-classical model in the many-atom regime based on the Jaynes-Cummings model is developed to describe the system that is in good qualitative agreement with the data. This work provides a foundation for developing multi-qubit quantum information experiments with a dual lattice cavity system.
We demonstrate accurate single-qubit control in an ensemble of atomic qubits trapped in an optical lattice. The qubits are driven with microwave radiation, and their dynamics tracked by optical probe polarimetry. Real-time diagnostics is crucial to minimize systematic errors and optimize the performance of single-qubit gates, leading to fidelities of 0.99 for single-qubit $\ensuremath{\pi}$ rotations. We show that increased robustness to large, deliberately introduced errors can be achieved through the use of composite rotations. However, during normal operation the combination of very small intrinsic errors and additional decoherence during the longer pulse sequences precludes any significant performance gain in our current experiment.
With the advent of laser cooling and trapping, neutral atoms have become a foundational source of accuracy for applications in metrology and are showing great potential for their use as qubits in quantum information. In metrology, neutral atoms provide the most accurate references for the measurement of time and acceleration. The unsurpassed stability provided by these systems make neutral atoms an attractive avenue to explore applications in quantum information and computing. However, to fully investigate the field of quantum information, we require a method to generate entangling interactions between neutral-atom qubits. Recent progress in the use of highly-excited Rydberg states for strong dipolar interactions has shown great promise for controlled entanglement using the Rydberg blockade phenomenon. I report the use of singly-trapped cesium atoms as qubits for applications in metrology and quantum information. Each atom provides a physical basis for a single qubit by encoding the required information into the ground-state hyperfine structure of cesium. Through the manipulation of these qubits with microwave and optical frequency sources, we demonstrate the capacity for arbitrary single-qubit control by driving qubit rotations in three orthogonal directions on the Bloch sphere. With this control, we develop an atom interferometer that far surpasses the force sensitivity of other approaches by applying the well-established technique of light-pulsed atom-matterwave interferometry to single atoms. Following this, we focus on two-qubit interactions using highly-excited Rydberg states. Through the development of a unique single-photon approach to Rydberg excitation using an ultraviolet laser at 319 nm, we observe the Rydberg blockade interaction between atoms separated by 6.6(3) microns. Motivated by the observation of Rydberg blockade, we study the application of Rydberg-dressed states for a quantum controlled-phase gate. Using a realistic simulation of the dressed-state dynamics, we calculate a controlled-phase gate fidelity of 94% that is primarily limited by Doppler frequency shifts. Finally, we employ our single-photon excitation laser to measure the Rydberg-dressed interaction, thus demonstrating the viability of this approach.
We present a proposal for quantum information processing with neutral atoms trapped in optical lattices as qubits. Initialization and coherent control of single qubits can be achieved with standard laser cooling and spectroscopic techniques. We consider entangling two-qubit logic gates based on optically induced dipole-dipole interactions, calculating a figure-of-merit for various protocols. Massive parallelism intrinsic to the lattice geometry makes this an intriguing system for scalable, fault-tolerant quantum computation.