It is conventional to describe the motion of an atom in a laser field (and other D.C fields) by a Fokker-Planck equation which is characterized by a force and a diffusion coefficient. Gordon and Ashkin have obtained a result for the diffusion coefficient in a spherically symmetric approximation. We have recently treated it as a second order tensor and have gotten a different result. The tensor has three terms. The leading term arises from the recoil of the atom during fluorescence, the second comes from gradients of the laser intensity and the D.C. fields and the last comes from a combination of the recoil term and gradients. The trace of our leading term agrees with the result of Gordon and Ashkin but there is no agreement at all with the other terms. The calculation was performed for a traveling wave laser and is being extended now to a standing wave laser by a graduate student. The experiment being undertaken here will use a swept laser frequency to compensate for the change in resonance frequency (due to the Doppler effect) of the atom as it slows down.
It is conventional to describe the motion of an atom in a laser field (and other D.C fields) by a Fokker-Planck equation which is characterized by a force and a diffusion coefficient. Gordon and Ashkin have obtained a result for the diffusion coefficient in a spherically symmetric approximation. We have recently treated it as a second order tensor and have gotten a different result. The tensor has three terms. The leading term arises from the recoil of the atom during fluorescence, the second comes from gradients of the laser intensity and the D.C. fields and the last comes from a combination of the recoil term and gradients. The trace of our leading term agrees with the result of Gordon and Ashkin but there is no agreement at all with the other terms. The calculation was performed for a traveling wave laser and is being extended now to a standing wave laser by a graduate student. The experiment being undertaken here will use a swept laser frequency to compensate for the change in resonance frequency (due to the Doppler effect) of the atom as it slows down.
In the limit of asymptotically small photon momentum, a Fokker–Planck equation for the center-of-mass Wigner function suffices to describe laser cooling of an atom. We have devised a procedure to compute the light pressure force and the diffusion tensor for an atom with an arbitrary level structure, traveling with an arbitrary velocity in any given three-dimensional light field. The scheme is based on solving a set of differential equations closely related to the density matrix equations of motion encountered in conventional recoilless laser spectroscopy. Computer programs have been written that automatically construct and solve the required equations from broad specifications of the problem, such as energies and angular momenta of the atomic levels. A Langevin equation stochastic simulation has been implemented to solve the Fokker-Planck equation of laser cooling using the computed force and diffusion. Comparisons of optical-molasses experiments and simulations carried out for a model sodium atom with a J = 2→J = 3 transition show qualitative similarities such as sub-Doppler limit temperatures, but the quantitative agreement of theory and experiment is not satisfactory.
This work discusses the effect of a high-intensity standing wave laser field on the motion of neutral atoms moving with a relatively high velocity. The analysis involves a detailed calculation of the force acting on the atoms and the calculation of the diffusion tensor associated with the fluctuations of the quantum force operator. The high-intensity laser field limit corresponds to a Rabi frequency much greater than the natural rate of the atom. The general results are valid for any atomic velocity. Results are then specialized to the case of slow and fast atoms where the Doppler shift of the laser frequency due to the atomic motion is either smaller or larger than the natural decay rate of the atom. The results obtained for the force and diffusion tensor are applied to a particular ideal experiment that studies the evolution of a fast atomic beam crossing a high-intensity laser beam. The theories developed previously, for a similar laser configuration, discuss only the low atomic velocities case and not the more realistic case of fast atoms. Here, an approximate solution of the equation for the distribution is obtained. Starting from the approximate distribution function, the deflection angle and dispersion angle for themore » atomic beam with respect to the free motion are calculated.« less
We give a general theoretical description of radiative forces on atoms in a monochromatic radiation field. The driven transition has a lower level consisting of several substates, and we consider the limit of low velocities and weak intensities. This situation comprises the schemes where cooling to temperatures below the Doppler limit is possible. After expressing the atomic dipole in terms of the polarizability tensor, we obtain an expression of the force as the sum of the radiation pressure, the dipole force, and a contribution from the gradient of the polarization. This latter contribution contains a part resulting from redistribution of photons between the plane waves that compose the field, and a part resulting from fluorescence. We express the average force and the momentum-diffusion tensor in terms of a closed evolution equation for the lower-state density matrix. We show by a scaling argument that in any case of cooling, the final temperature goes down linearly with the intensity, until the recoil limit is approached. The description is valid for a weak and monochromatic, but otherwise arbitrary field, and it allows for the presence of an external magnetic field, and of hyperfine splitting. It is applicable to cooling in one, two, or three dimensions. We give numerical results for the average force in a number of specific cases of two counterrunning plane waves.
The momentum diffusion coefficient, as a function of position and velocity, is discussed for two-state atoms travelling through a standing-wave laser field. Equations leading to the force and diffusion coefficient have been obtained by Minogin. The authors present an alternative derivation, based on moments of the Wigner function and give numerical solutions in terms of matrix continued fractions. In strong fields, the discussion is supplemented by a derivation of the diffusion coefficient within the dressed-atom basis, and a picture of the diffusion mechanism emerges which is quite different from the one at low intensities. Calculated forces and diffusion coefficients are used in a Fokker-Planck equation to obtain stationary atomic velocity distributions.
The motion of slow atoms with degenerate energy levels in a resonant, nonuniformly polarized laser field is described by the Fokker-Planck equation for the atomic distribution function in phase space in terms of the semiclassical approach. Field gradient expansions are used for the spatially nonuniform coefficients of the equation. For closed atomic transitions J g =J→J e =J+1 (J g and J e are the total angular momenta of the ground and excited states, respectively), new analytical results are presented for the light pressure force and the friction and diffusion coefficients in momentum space. These results allow the kinetic effects (laser cooling, localization in optical potential wells, etc.) in a field of arbitrary one-, two-, or three-dimensional configuration to be investigated. In several cases, the new contributions to the friction coefficient are interpreted qualitatively.
The present state of research on the cooling of atomic ensembles by means of laser radiation pressure is discussed. First the basic theory of resonance radiation pressure is reviewed. The effect of recoil on the drift and fluctuations of the momentum of an atom interacting with resonance radiation is examined. There is an analysis of the forces acting on an atom in some simple light fields: a traveling plane wave, a Gaussian beam, and counterpropagating Gaussian beams. The review then focuses on the monochromatization of atoms by resonance radiation pressure and related methods for laser cooling of atoms. The roles played by the radiation pressure force and by momentum diffusion in shaping the narrow velocity distributions of the ensemble of atoms are analyzed. The lowest temperature obtainable in the radiation cooling of atoms is estimated. The basic experimental methods for laser cooling of atomic beams are described. Problems of the three-dimensional cooling of atomic ensembles and problems of localizing cold atoms in light fields, steady-state magnetic fields, and electrostatic fields are discussed. The review concludes with a discussion of some applications of cold atoms in high-precision spectroscopy, frequency standards, and atomic physics.