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Chinese Physics Letters

Control of Polarization Interference in Doppler Broadened Two-Photon Resonant Four-Wave Mixing System

Zuo Zhan-Chun, Xia Liu, Sun Jiang, Ling-An Wu, Panming Fu

Published Feb 24, 2006• 0 citations
Publisher

Abstract

We study two-photon resonant nondegenerate four-wave mixing (NFWM) in a Doppler broadened system. It is found that because the induced polarization is sensitive to the atomic velocity, there exists interference between polarizations of atoms with different velocities, leading to significant modification of the NFWM spectra. This polarization interference can be controlled through applying an additional coupling field.

DOI
10.1088/0256-307x/23/3/028

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We study two-photon resonant nondegenerate four-wave mixing (NFWM) in a Doppler broadened system. It is found that because the induced polarization is sensitive to the atomic velocity, there exists interference between polarizations of atoms with different velocities, leading to significant modification of the NFWM spectra. This polarization interference can be controlled through applying an additional coupling field.
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We study the quantum interference in two-photon resonant nondegenerate four-wave mixing (NFWM) in a dressed cascade four-level system in which the two upper levels are coupled by a strong laser field. We find that in the presence of a strong coupling field, two-photon resonant NFWM spectrum exhibits Autler-Townes splitting, which reflects the levels of the dressed states. It also leads to either suppression or enhancement of the NFWM signal. This scheme involves the resonant three-photon excitation, therefore, provides a new spectroscopic tool for studying highly excited atomic states with high sensitivity.
We study six-wave mixing (SWM) spectroscopy based on electromagnetically induced transparency in a Doppler-broadened cascade four-level system. It is found that the SWM spectra are extremely sensitive to the configuration of the incident beams, where the linewidth can be either Doppler-free or very broad, due to the polarization interference of atoms of different velocities. This polarization interference can be controlled in the presence of a strong coupling field. Moreover, SWM can be employed as a new type of Doppler-free Autler–Townes (AT) spectroscopy, which has better spectral resolution than conventional AT spectroscopy. Finally, we also reveal the intrinsic connection between frequency-domain SWM spectroscopy and time-domain photon echoes through studying the time-domain correspondence of SWM.
In nonlinear atomic gaseous media the interference between independent macroscopic polarizations of different ensembles within the atomic velocity distribution can lead to anomalous behavior of the multiwave mixing spectra. For phase-conjugate six-wave mixing (SWM) in a Doppler-broadened N-type four-level system, it is found that the SWM spectrum can be either Doppler-free or very broad, depending on the directions of the incident beams and the ratios between the magnitudes of the wave vectors. This polarization interference can be controlled by the strong coupling field which, on the other hand, can induce Autler-Townes (AT) splitting when the SWM spectrum is Doppler-free. This technique may find special applications as an improved form of AT spectroscopy with higher resolution.