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Optics and Spectroscopy

The effect of hyperfine level structure on the process of light scattering by polarized atoms

M. Ya. Agre, Л. П. Рапопорт

Published Mar 1, 1994• 0 citations
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We report on the observation of a new magic frequency within the hyperfine structure of the D2 line of 87{}^{87}87Rb atoms at which the scattering of light into a high-finesse cavity is suppressed by an interplay between quantum interference and the strong collective coupling of atoms to the cavity. Scattering from a cloud of laser-driven cold atoms into the cavity was measured in a polarization sensitive way. We have found that both the Rayleigh and Raman scattering processes into the near-resonant cavity modes are extinguished at 185 MHz below the F=2↔\leftrightarrow↔F'=3 transition frequency. This coincidence together with the shape of the observed spectral dip imply that the effect relies on a quantum interference in the polariton excitations of the strongly coupled combined atom-photon system. We have also demonstrated the existence of a magic frequency around -506 MHz, where only the Raman scattering is suppressed due to a quantum interference effect at the single-atom level.
A combined experimental and theoretical investigation of time- and alignment-dependent propagation of light in an ultracold atomic gas of atomic 85Rb^{85}\mathrm{Rb}85Rb is reported. Coherences among the scattering amplitudes for light scattering off excited hyperfine levels produce strong variations of the light polarization in the vicinity of atomic resonance. Measurements are in excellent agreement with Monte Carlo simulations of the multiple scattering process.