This portfolio of work contributes to the remit of the National Physical Laboratory (NPL) to develop the underpinning expertise and tools for validating nascent and future optical quantum technologies based on the discrete and quantum properties of photons. This requirement overlaps with the requirement to provide validation for devices operating in the photon-counting regime. A common theme running through the portfolio is photon pairs generated through spontaneous parametric downconversion (SPDC). \n \nA Hong-Ou-Mandel (HOM) interferometer sourced with visible wavelength photon pairs from an SPDC process in beta-barium borate (BBO) was designed, built and characterised. The visibility of the HOM interference is dependent on the indistinguishability of the interfering photons, but is also influenced by imperfections of the interferometer; therefore an investigation was carried out to quantify the effects of the interferometer imperfections on the measured visibility so that the true photon indistinguishability could be measured with a quantified uncertainty. \n \nA bright source of correlated pair photons in the telecoms band based upon a pump enhanced SPDC process in periodically-poled potassium titanyl phosphate (PPKTP) was designed, built and characterised. From the characterisation measurements the source brightness was estimated to be 6.2×10⁴ pairs/ s/ mw pump. The photon pairs were further characterised through their incorporation as a source in a HOM interference experiment. \n \nThe developed correlated photon pair source was at the heart of a novel scheme for the generation of polarisation entangled photon pairs, for which the design, build and characterisation work is presented. The source was demonstrated to produce two of the four maximally entangled Bell states with quantum interference visibilities of around 0.95. The generated states were also shown to break a form of Bell’s inequality by around six standard deviations. The polarisation entangled photon pair source was originally built at the University of St Andrews and was later transferred to the NPL where it will extend NPL’s capabilities to this key spectral region. \n \nFinally a study was carried out to investigate the possibility of a wavelength tuneable device for the absolute measurement of single photon detector quantum efficiencies based upon an established SPDC technique.
This portfolio of work contributes to the remit of the National Physical Laboratory (NPL) to develop the underpinning expertise and tools for validating nascent and future optical quantum technologies based on the discrete and quantum properties of photons. This requirement overlaps with the requirement to provide validation for devices operating in the photon-counting regime. A common theme running through the portfolio is photon pairs generated through spontaneous parametric downconversion (SPDC). \n \nA Hong-Ou-Mandel (HOM) interferometer sourced with visible wavelength photon pairs from an SPDC process in beta-barium borate (BBO) was designed, built and characterised. The visibility of the HOM interference is dependent on the indistinguishability of the interfering photons, but is also influenced by imperfections of the interferometer; therefore an investigation was carried out to quantify the effects of the interferometer imperfections on the measured visibility so that the true photon indistinguishability could be measured with a quantified uncertainty. \n \nA bright source of correlated pair photons in the telecoms band based upon a pump enhanced SPDC process in periodically-poled potassium titanyl phosphate (PPKTP) was designed, built and characterised. From the characterisation measurements the source brightness was estimated to be 6.2×10⁴ pairs/ s/ mw pump. The photon pairs were further characterised through their incorporation as a source in a HOM interference experiment. \n \nThe developed correlated photon pair source was at the heart of a novel scheme for the generation of polarisation entangled photon pairs, for which the design, build and characterisation work is presented. The source was demonstrated to produce two of the four maximally entangled Bell states with quantum interference visibilities of around 0.95. The generated states were also shown to break a form of Bell’s inequality by around six standard deviations. The polarisation entangled photon pair source was originally built at the University of St Andrews and was later transferred to the NPL where it will extend NPL’s capabilities to this key spectral region. \n \nFinally a study was carried out to investigate the possibility of a wavelength tuneable device for the absolute measurement of single photon detector quantum efficiencies based upon an established SPDC technique.
Correlated photon pairs generated through spontaneous parametric downconversion have become a key resource for research into enhanced optical measurement and quantum optical information processing. A pump-enhanced χ(2) source of correlated photons in the telecom band is presented. An investigation of the pair photon coincidence detection rate measured from the source, together with the evaluation of system losses, indicated a single spatial fibre-optic mode pair production rate of 6.12 × 104 s−1 mW−1 pump power, an order of magnitude greater than was measured without enhancement. A Hong-Ou-Mandel interference experiment confirmed that the enhancement did not have any adverse effect on the spatial and frequency indistinguishability of the emitted pairs. The source comprises a symmetric and linear enhancement cavity for the pump, making it particularly suitable for generating polarisation entangled photon pairs without the need for compensating crystals 1 Thomas, PJ, Chunnilall, CJ, Stothard, DJM, Walsh, DA and Dunn, MH. 2010. Opt. Express, 18: 26600–26612. [Crossref], [PubMed], [Web of Science ®] , [Google Scholar].
Entangled photon pairs play a crucial role in emerging quantum technologies, acting as tamper-proof padlocks in secure quantum communication, ultra-precise probes in quantum metrology and high-fidelity information carriers in photonic quantum computing. Amongst the many technological possibilities for generating photon pairs, sources based on spontaneous parametric down-conversion (SPDC) in second-order nonlinear crystals are still the workhorse tool in quantum optics laboratories, and more recently even in long-distance quantum communication with satellites. SPDC is a widely used method to create entangled photon pairs. The number of photon pairs that can be detected in a particular choice of collection modes, typically being optical single-mode fibers, depends critically on the spatial characteristics of the multi-mode SPDC emission as well as the particular beam waist of the collection modes. While several studies have already addressed the issue of optimal fiber coupling of SPDC photons in theory and experiment, the results of these studies arrive at different conclusions. Here, we present the results of a comprehensive experimental study on the optimal collection of photon pairs into single-mode optical fibers. Our approach is based on quasi-phase-matched type II SPDC from a periodically poled KTiOPO4 (ppKTP) crystal. We discuss the influence of pump and collection focal parameters on the spectral brightness and heralding efficiency, as well as practical issues of alignment tolerances into an optical single mode fiber. Further, Using two-photon interference (Hong-Ou-Mandel interference), we assess the spectral bandwidth of the photon pairs for variable crystal lengths. The results are in good agreement with our theoretical model, thus providing the recipe of building ultra bright and stable entangled photon sources.
Quantum information protocols tend to involve more and more entangled photon pairs, for enabling advanced quantum tasks. To compensate for the low success efficiency of these protocols, one can increase the repetition rate of the emitted pairs, up to current telecom standard (40 GHz). In this context, we propose a realization of ultra-fast photon pair sources, intended for either heralded quantum state engineering or entanglement swapping at telecom wave- length. In this paper, we present preliminary results consisting of a two-photon interference experiment using four photons where the achieved raw visibility of the Hong-Ou-Mandel (HOM) dip exceeds 98.6 %. The interfering photons are generated through spontaneous parametric down conversion process (SPDC) in two independent, separate, periodically poled lithium niobate (PPLN) waveguides.
Spontaneous parametric down-conversion (SPDC) is a reliable and robust source of photons for quantum information applications. For applications that involve operations such as entanglement swapping or single-photon heralding, two-photon states are required to be factorable (uncorrelated) in their spectral and spatial degrees of freedom. We report the design and experimental characterization of an SPDC source that has been optimized for high spectral and spatial purity. The source is pumped by the 776 nm output of a mode-locked Ti:Sapphire laser and consists of a periodically-poled Potassium Titanyl Phosphate (PPKTP) crystal phase-matched for collinear type-II SPDC. The dispersive properties of PPKTP at these wavelengths is such that it is possible to minimize the spectral entanglement by matching the widths of the pump to the spectral phase-matching function. The spatial entanglement is minimized through careful control of the pump focus, yielding nearly single-mode emission. An advantage of this approach is that the emission rate into the collection modes is very high, resulting in a very bright SPDC source. We also report a scheme that employs the output of collinear sources such as these to produce polarization-entangled photon pairs. The scheme, which requires only simple polarization elements, can be scaled to N-photon GHZ states.
This thesis deals with the production of entangled photons using spontaneous parametric down-conversion (SPDC). We start with a short overview of some important theoretical concepts. First we provide a brief reminder of the theory of entanglement. We then discuss how the state of quantum systems can be determined using quantum state tomography. We also explain SPDC, the physical process which we use to produce entangled photons. Finally, we give an overview of the methods which have been used to produce entangled photons in the past, both for two- and three-photon entanglement. \n \nThe first experiment is the design of an efficient source of entangled photon pairs based on a polarizing Sagnac interferometer configuration. With this configuration, we can use quasi-phasematched materials which allow for higher efficiencies than standard bulk nonlinear materials. The source is pumped by a low-power continuous-wave laser diode, and produces degenerate photon pairs at 809nm. It has a spectral brightness of 87,500 pairs/(s mW nm), and the fidelity of the produced quantum states with a Bell state is 98.9%. The source is used for experiments in quantum key distribution, cluster state quantum computing, remote state preparation, state discrimination, and entanglement-enhanced classical communication. \n \nThe second experiment discussed in this thesis is the generation of photon triplets using cascaded SPDC. In this experiment, a primary SPDC source is pumped with a low-power, continuous-wave laser diode, producing photon pairs. Single photons from these pairs serve as the pump for a second down-conversion, resulting in photon triplets. This is the first demonstration of the direct production of photon triplets, and the first observation of SPDC at the single photon level. This method could potentially be used to produce entangled photon triplets without post-selection, and as a source of triggered Bell pairs.
Hong-Ou-Mandel (HOM) interference is a cornerstone of many quantum information processing tasks. It relies on the destructive interference between Feynman paths and provides a measure of photon indistinguishability. For certain applications, e.g. in some quantum secure authentication schemes, the HOM readout needs to be performed remotely, i.e. far away from where the photons were originally created. It is therefore important to understand the effect of dispersion on the two-photon state and consequently its effect on the coincidence probability. Our work focuses on providing measurement data of the effect of polarization mode dispersion (PMD) on the HOM interference for photon pairs produced by spontaneous parametric down conversion (SPDC).