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Chinese Physics Letters

Experimental Observation of Autler-Townes Splitting in Sub-Doppler Selective Reflection Spectroscopy

赵延霆, Jianming Zhao, Tao Huang, Liantuan Xiao, 贾锁堂

Published Jan 1, 2005• 0 citations
OpenAlex

Abstract

We present an experimental study of Autler-Townes splitting of non-linear selective reflection spectroscopy in a A-type driven three-level system. The sub-Doppler reflection spectroscopy is observed and the Autler-Townes splitting is measured as functions of the different coupling laser intensity and detuning. The coherent drive splits the excited state into two dressed states and an Autler-Townes splitting emerges in the probe reflection. The experimental results are in good agreement with theoretical fit.

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We have investigated the effects of inhomogeneous Doppler line broadening on the Autler-Townes (AT) splitting in a three-level open molecular cascade system. For moderate Rabi frequencies in the range of $300--600\phantom{\rule{0.3em}{0ex}}\mathrm{MHz}$, the fluorescence line shape from the uppermost level \ensuremath{\mid}3⟩ in this system depends strongly on the wave-number ratio of the two laser fields. However, the fluorescence spectrum of the intermediate level \ensuremath{\mid}2⟩ appears as expected. We provide a description of the conditions for optimally resolved AT splitting in terms of the ratio of the probe and coupling laser wave numbers, and the laser propagation geometry based on our theoretical analysis of the Doppler integral. The low threshold Rabi frequency region for Autler-Townes splitting is important for high-resolution Autler-Townes spectroscopy since the laser E-field amplitudes are modest in continuous-wave laser experiments.

Physical Review A•Oct 7, 2008•19 citations
We present an experimental study of Autler-Townes splitting of non-linear selective reflection spectroscopy in a A-type driven three-level system. The sub-Doppler reflection spectroscopy is observed and the Autler-Townes splitting is measured as functions of the different coupling laser intensity and detuning. The coherent drive splits the excited state into two dressed states and an Autler-Townes splitting emerges in the probe reflection. The experimental results are in good agreement with theoretical fit.
We present an experimental study of Autler–Townes splitting of non-linear selective reflection spectroscopy in a Λ-type driven three-level system. The sub-Doppler reflection spectroscopy is observed and the Autler–Townes splitting is measured as functions of the different coupling laser intensity and detuning. The coherent drive splits the excited state into two dressed states and an Autler–Townes splitting emerges in the probe reflection. The experimental results are in good agreement with theoretical fit.
With a coupling laser locked to caesium 6S 1/2 F g =4–6P 3/2 F e =5 cycling transition and a co-propagating probe laser scanned across 6S 1/2 F g =4–6P 3/2 F e =3, 4 and 5 transitions, a novel scheme for sub-Doppler spectra in Doppler-broadened V-type three-level system is demonstrated by detecting the transmission of the coupling laser through a caesium vapour cell. The Autler–Townes doublet in the sub-Doppler spectra of the coupling laser is clearly observed. The effects of coupling laser intensity on the splitting and linewidth of the Autler–Townes doublet are experimentally investigated and the results agree well with theoretical predictions. Taking the multiple hyperfine levels of caesium atom into account, a brief analysis is presented.
Some features of the optical Autler-Townes effect as observed in Doppler-broadened three-level systems, including the physical significance of the observed line splitting, the conditions for the observation of the doublet, the doublet separation and the detuning effects, are discussed in this paper. A graphical illustration of the phenomenon, based on a search for on-resonance velocity groups, is proposed which allows a complete qualitative discussion of the effect and shows that the observed doublet is not really a splitting of the resonance as for the atom at rest but rather corresponds to a frequency hole where the laser probe does not see any resonant velocity group. The method is applied to real three-level systems of neon as typical cases. A semi-classical density-matrix calculation is performed numerically and definitely confirms the results of the qualitative graphical discussion ; furthermore it shows that, for many experimental situations, the first order approximation is inadequate. The observation of the Autler-Townes doublet in a new experiment using two dye lasers is reported. The experimental results and that of one of our previous experiments are compared with the theoretical predictions ; the agreement is quite satisfactory.
We report an experimental observation of Autler-Townes doublet splitting in electromagnetically induced transparency (EIT) resonance. The splitting is introduced by a coherent microwave field, which perturbs a three-level A-type EIT system through an auxiliary level. The doublet splitting of EIT resonance is demonstrated in two cases, where the microwave field shares a common lower level with coupled or probe transition, respectively. The dependence of doublet splitting on microwave field intensity and detuning is measured. This may provide a feasible way of manipulating the atomic states with both laser and microwave field.
Theoretical analysis of the Autler-Townes splitting pattern in a three-level cascade excitation of a Doppler-broadened sample reveals that the observed Autler-Townes splitting is not only a function of the coupling-laser Rabi frequency, as in the homogeneously broadened case, but can also strongly depend on the wavenumber ratio of the coupling and probe lasers. Utilizing a steady-state density matrix formalism, we derive exact expressions for the populations of the intermediate and upper levels for a homogeneously broadened system. In the limit of a weak probe field, analytical expressions for Doppler-broadened excitation spectra from the intermediate and upper levels are derived. Using these expressions, we investigate the critical role of Doppler broadening on the observation of Autler-Townes splitting and its asymptotic behavior as a function of the coupling Rabi frequency for counterpropagating and copropagating configurations for different wavenumber ratios of the lasers.
We have investigated the effects of inhomogeneous Doppler line broadening on the Autler-Townes (AT) splitting in a three-level open molecular cascade system. For moderate Rabi frequencies in the range of 300−−600MHz300--600\phantom{\rule{0.3em}{0ex}}\mathrm{MHz}300−−600MHz, the fluorescence line shape from the uppermost level \ensuremath{\mid}3⟩ in this system depends strongly on the wave-number ratio of the two laser fields. However, the fluorescence spectrum of the intermediate level \ensuremath{\mid}2⟩ appears as expected. We provide a description of the conditions for optimally resolved AT splitting in terms of the ratio of the probe and coupling laser wave numbers, and the laser propagation geometry based on our theoretical analysis of the Doppler integral. The low threshold Rabi frequency region for Autler-Townes splitting is important for high-resolution Autler-Townes spectroscopy since the laser E-field amplitudes are modest in continuous-wave laser experiments.