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Comparative Study of Forward and Diffusely Scattered Light in a Coherently Prepared Ultracold Rubidium Gas

Olave Gonzalez

Published Oct 21, 2019• 0 citations
Publisher

Abstract

A comparison between forward and diffusely scattered light propagating in a coherently prepared ultracold 87Rb atomic vapor is presented. This research is part of the ongoing effort to characterize the processes, such as diffusion, that contribute to coherence loss in atomic media under conditions of electromagnetically induced transparency, for applications in realistic systems. Toward this end, a magneto optical trap (MOT) of 87Rb has been built, and the atomic vapor sample characterized in terms of atomic density, shape and size, temperature, and optical depth. Next, two co-propagating beams were sent through the sample, to establish an electromagnetically induced transparency in a Λ-type system. In these measurements the two laser fields are not phase-locked, so ground state coherence will be affected by the lasers' phase fluctuations. Observation of the forward and diffusely scattered light were made for different conditions of probe pulse length, control field intensity, and probe field frequency detuning. Storage and retrieval of slow light pulses was achieved for the forward scattering (transmission) channel, but was not observed unambiguously in the diffusely scattered (fluorescence) channel.

DOI
10.25777/309d-2g02

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A comparison between forward and diffusely scattered light propagating in a coherently prepared ultracold 87Rb atomic vapor is presented. This research is part of the ongoing effort to characterize the processes, such as diffusion, that contribute to coherence loss in atomic media under conditions of electromagnetically induced transparency, for applications in realistic systems. Toward this end, a magneto optical trap (MOT) of 87Rb has been built, and the atomic vapor sample characterized in terms of atomic density, shape and size, temperature, and optical depth. Next, two co-propagating beams were sent through the sample, to establish an electromagnetically induced transparency in a Λ-type system. In these measurements the two laser fields are not phase-locked, so ground state coherence will be affected by the lasers' phase fluctuations. Observation of the forward and diffusely scattered light were made for different conditions of probe pulse length, control field intensity, and probe field frequency detuning. Storage and retrieval of slow light pulses was achieved for the forward scattering (transmission) channel, but was not observed unambiguously in the diffusely scattered (fluorescence) channel.
Recent years have observed fast developments in neutral atomic vapor based quantum information storage technology. The technique utilizes light fields in the optical wavelength region as signal carrier and retriever and neutral atomic systems (e.g. single atoms, ensembles of atoms, atom-like defects in solids) as storage media. Photons are robust carriers of information due to their high velocity (c = 2.998 x 108 m/s) and ease of transportation (they propagate rectilinearly with low loss). Their high mobility, however, makes it a challenging task to spatially localize and therefore store them. Atoms (or atom-like systems), on the other hand, can be easily localized in space while providing quantum states accessible to photons and therefore are ideal candidates for storage media. Electromagnetically-induced transparency (EIT) is a light-induced atomic coherence phenomenon that dramatically modifies the optical properties of an atomic medium to a weak probe field by the application of a strong coupling field. As a probe pulse propagates in an EIT medium it experiences ultraslow group velocity and generates a copropagating spin wave. These consequences of EIT can be exploited for light pulse storage and retrieval in an atomic medium.
We show that under conditions typical of electromagnetically induced transparency (EIT) in an ultracold atomic sample in a magneto-optical trap, a significant portion of the incident probe pulse is transferred into Rayleigh and Raman scattering channels. The light scattered into the Rayleigh channel emerges from the sample with an EIT time delay. We show that a proper description of the probe light propagation in the sample should include, in the diffusion dynamics, a spin polariton generated by the two-photon EIT process. The results have important implications for studies of weak light localization and for manipulation of single and few photon states in ultracold atomic gases.
We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic media prepared at ultralow temperatures can be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the media, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We demonstrate how this mechanism, potentially interesting for developing quantum memories, would work for the example of a coherent light pulse propagating through an alkali-metal atomic vapor under typical conditions attainable in experiments with ultracold atoms.
This thesis set out to investigate light storage based on dynamic electromagnetically induced transparency (EIT) in a room-temperature atomic ensemble of rubidium as a means to provide a quantum memory for single-photons created by a single rubidium atom coupled to a high-finesse optical resonator. Setting up the light storage medium presented a new addition to the research group's portfolio of experimental techniques and led to investigations of EIT, slow light and stored light in warm rubidium-87 vapour. Lambda level schemes connecting Zeeman or hyperfine substates on the D1 and D2 lines were addressed in rubidium vapour cells containing different buffer gases and different isotopic fractions of rubidium-87 and rubidium-85. Single beam spectroscopy with a weak probe was used to characterise the vapour cells. A numerical method to fit the D line spectrum to a theoretical model to include isotopic fractions and collisional broadening of a buffer gas has been implemented. Temperature and isotopic fractions could be reliably extracted from the fit parameters. For an offset-stabilisation of two lasers to address a lambda level scheme connecting the two different hyperfine groundstates in rubidium a phase locked loop including a frequency divider has been designed and implemented. Light storage and retrieval has been demonstrated using a Zeeman scheme on the D1 line. Two microsecond long classical light pulses containing one million photons on average were stored and retrieved with an efficiency of 15% after a delay of one microsecond. Several methods of attenuating the strong co-propagating control laser beam to allow for lowering the signal pulse intensity in future experiments are discussed.
Coherent nonlinear effects such as Electromagnetically Induced Transparency\n(EIT), Coherent Population Trapping (CPT), and Slow light are studied in thermal\nRb vapor by both continuous and pulsed laser fields. This work primarily includes\nthree parts: (I) mode-locked rubidium laser and its applications (II) enhanced coupling\nbetween optical and sound waves in the forward direction via ultra-slow light\n(III) optical steering via ultra-slow light in rubidium vapor.\nIn part(I), I describe the construction and study of a mode-locked rubidium laser\noperating at the Rb D1 line using an active mode-locking technique inside the laser\ncavity. The mode-locked laser field is used to observe coherent effects in a dense\nrubidium gas.\nIn part(II), I experimentally demonstrate enhanced acoustic-optic coupling that\noccurs when the velocity of sound is close to the group velocity of light. Dragging of\nthe light by effective motion of the gas in a Rb cell is the origin of enhanced coupling.\nGood agreement between theory and experiment is found.\nIn part(III), I experimentally demonstrate optical beam deflection in coherently\ndriven rubidium vapor due to the steep refraction index profile in the region of EIT.
Over the past half century, atomic ensembles have been used to create sensors, clocks, and quantum information systems. As these devices become more compact, and as the number of atoms increases to improve the sensitivity for detection, the atomic samples are increasing in density and optical depth. As such, the spectroscopic properties of the atomic media are modified due to interactions among the particles in the ensemble. We report investigation of near-resonance light scattering from a cold atomic sample of 87Rb. Initially prepared in a magneto-optical trap, the atoms are loaded into a far-off-resonance optical dipole trap (FORT) in which the ensemble has a temperature near 100 mK and initial Gaussian radii of approximately 3 mm and 280 mm in the transverse and longitudinal directions, respectively. With atomic densities in the range of 1010 - 1013 atoms/cm3, measurements are made on the F=2 -> F'=3 nearly closed hyperfine transition. The experimental geometry consists of projecting a near-resonance collimated laser beam onto the entire volume of the FORT and detecting the diffusely scattered light. The measured scattered light intensity as a function of detuning, atomic number, and sample size suggests that collective light scattering depends on the optical depth of the system.