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arXiv:1007.2682 · Journal of the Optical Society of America B

Optical control of diffuse light storage in an ultracold atomic gas

L. V. Gerasimov, Igor M. Sokolov, Dmitriy V. Kupriyanov, R. G. Olave, Mark D. Havey

Published May 18, 2011• 8 citations
arXivHTMLPDF

Abstract

We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic media prepared at ultralow temperatures can be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the media, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We demonstrate how this mechanism, potentially interesting for developing quantum memories, would work for the example of a coherent light pulse propagating through an alkali-metal atomic vapor under typical conditions attainable in experiments with ultracold atoms.

DOI
10.1364/josab.28.001459

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We show that coherent multiple light scattering, or diffuse light propagation, in a disordered atomic media prepared at ultralow temperatures can be effectively delayed in the presence of a strong control field initiating a stimulated Raman process. On a relatively short time scale, when the atomic system can preserve its configuration and effects of atomic motion can be ignored, the scattered signal pulse, diffusely propagating via multiple coherent scattering through the media, can be stored in the spin subsystem through its stimulated Raman-type conversion into spin coherence. We demonstrate how this mechanism, potentially interesting for developing quantum memories, would work for the example of a coherent light pulse propagating through an alkali-metal atomic vapor under typical conditions attainable in experiments with ultracold atoms.
In this paper, we consider a quantum memory scheme for light diffusely propagating through a spatially disordered atomic gas. A unique characteristic is enhanced trapping of the signal light pulse by quantum multiple scattering, which can be naturally integrated with the mechanism of stimulated Raman conversion into a long-lived spin coherence. Then, the quantum state of the light can be mapped onto the disordered atomic spin subsystem and can be stored in it for a relatively long time. The proposed memory scheme can be applicable for storage of the macroscopic analogue of the Ψ ( − ) Bell state and the prepared entangled atomic state performs its quantum hologram, which suggests the possibility of further quantum information processing.
A comparison between forward and diffusely scattered light propagating in a coherently prepared ultracold 87Rb atomic vapor is presented. This research is part of the ongoing effort to characterize the processes, such as diffusion, that contribute to coherence loss in atomic media under conditions of electromagnetically induced transparency, for applications in realistic systems. Toward this end, a magneto optical trap (MOT) of 87Rb has been built, and the atomic vapor sample characterized in terms of atomic density, shape and size, temperature, and optical depth. Next, two co-propagating beams were sent through the sample, to establish an electromagnetically induced transparency in a Λ-type system. In these measurements the two laser fields are not phase-locked, so ground state coherence will be affected by the lasers' phase fluctuations. Observation of the forward and diffusely scattered light were made for different conditions of probe pulse length, control field intensity, and probe field frequency detuning. Storage and retrieval of slow light pulses was achieved for the forward scattering (transmission) channel, but was not observed unambiguously in the diffusely scattered (fluorescence) channel.
We experimentally demonstrate emission of two quantum-mechanically correlated light pulses with a time delay that is coherently controlled via temporal storage of photonic states in an ensemble of rubidium atoms. The experiment is based on Raman scattering, which produces correlated pairs of spin-flipped atoms and photons, followed by coherent conversion of the atomic states into a different photon beam after a controllable delay. This resonant nonlinear optical process is a promising technique for potential applications in quantum communication.
We apply collective Raman scattering to create, store and retrieve spatially multimode light in warm rubidium-87 vapors. The light is created in a spontaneous Stokes scattering process. This is accompanied by the creation of counterpart collective excitations in the atomic ensemble - the spin waves. After a certain storage time we coherently convert the spin waves into the light in deterministic anti-Stokes scattering. The whole process can be regarded as a delayed four-wave mixing which produces pairs of correlated, delayed random images. Storage of higher order spatial modes up to microseconds is possible owing to usage of a buffer gas. We study the performance of the Raman scattering, storage and retrieval of collective excitations focusing on spatial effects and the influence of decoherence caused by diffusion of rubidium atoms in different buffer gases. We quantify the number of modes created and retrieved by analyzing statistical correlations of intensity fluctuations between portions of the light scattered in the far field.
We propose a scheme to realize the storage and retrieval of light pulses in a fast-light medium via a mechanism of active Raman gain (ARG). The system under consideration is a four-level atomic gas interacting with three (pump, signal, and control) laser fields. We show that a stable propagation of signal light pulses with superluminal velocity (i.e., fast-light pulses) is possible in such a system through the ARG contributed by the pump field and the quantum interference effect induced by the control field. We further show that a robust storage and retrieval of light pulses in such a fast-light medium can be implemented by switching on and off the pump and the control fields simultaneously. The results reported here may have potential applications for light information processing and transmission using fast-light media.
We show that under conditions typical of electromagnetically induced transparency (EIT) in an ultracold atomic sample in a magneto-optical trap, a significant portion of the incident probe pulse is transferred into Rayleigh and Raman scattering channels. The light scattered into the Rayleigh channel emerges from the sample with an EIT time delay. We show that a proper description of the probe light propagation in the sample should include, in the diffusion dynamics, a spin polariton generated by the two-photon EIT process. The results have important implications for studies of weak light localization and for manipulation of single and few photon states in ultracold atomic gases.