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Chinese Physics Letters

Evolution of Spin and Charge in a System with Interacting Impurity and Conducting Electrons

张永梅, 熊诗杰

Published Jan 1, 2003• 0 citations
OpenAlex

Abstract

We investigate the dynamics of spin and charge in an interacting system consisting of impurity and conduct-ing electrons. The time evolution of spin and charge in the impurity is given by solving the time-dependent Schroedinger equations for the many-body states of the interacting system. By switching on the interaction be-tween impurity and conducting electrons, the spin and charge of the impurity begin oscillations with frequencies that reflect the elementary excitations of the interacting system. The dynamics reflects the basic picture of the Kondo effect.

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We investigate the dynamics of spin and charge in an interacting system consisting of impurity and conduct-ing electrons. The time evolution of spin and charge in the impurity is given by solving the time-dependent Schroedinger equations for the many-body states of the interacting system. By switching on the interaction be-tween impurity and conducting electrons, the spin and charge of the impurity begin oscillations with frequencies that reflect the elementary excitations of the interacting system. The dynamics reflects the basic picture of the Kondo effect.
We investigate the dynamics of spin and charge in an interacting system consisting of impurity and conducting electrons. The time evolution of spin and charge in the impurity is given by solving the time-dependent Schrödinger equations for the many-body states of the interacting system. By switching on the interaction between impurity and conducting electrons, the spin and charge of the impurity begin oscillations with frequencies that reflect the elementary excitations of the interacting system. The dynamics reflects the basic picture of the Kondo effect.
We analyze the spin- and charge-density oscillations near impurities in spin chains and quantum wires. These so-called Friedel oscillations give detailed information about the impurity and also about the interactions in the system. The temperature dependence of these oscillations explicitly shows the renormalization of backscattering and conductivity, which we analyze for a number of different impurity models. We are also able to analyze screening effects in one dimension. The relation to the Kondo effect and experimental consequences are discussed.
We study the spin and charge oscillations of a quantum dot by exactly solving the time-dependent many-body Schr\"odinger equation of a system with a dot embedded in a ring. The dot is characterized by the on-site Coulomb interaction and the gate voltage that governs the occupation status. The itinerant electrons are moving in the ring. By switching on the coupling between the dot and the ring the spin and charge on the dot begin to have undamped oscillations. In the regime of single occupation of the dot, there exists a base frequency of the oscillations that is associated with the spin excitations. Some higher frequencies may be associated with both the charge and spin motions. The results reveal the dynamical characteristics of the spin and charge degrees of freedom and the spectrum of low-energy excitations.
We study the real-time dynamics of the Kondo effect after a quantum quench in which a magnetic impurity is coupled to two metallic Hubbard chains. Using an effective field theory approach, we find that for noninteracting electrons the charge current across the impurity is given by a scaling function that involves the Kondo time. In the interacting case, we show that the Kondo time decreases with the strength of the repulsive interaction and the time dependence of the current reveals signatures of the Kondo effect in a Luttinger liquid. In addition, we verify that the relaxation of the impurity magnetization does not exhibit universal scaling behavior in the perturbative regime below the Kondo time. Our results highlight the role of nonequilibrium dynamics as a valuable tool in the study of quantum impurities in interacting systems.
A detailed derivation of the recently proposed time-dependent numerical renormalization-group (TD-NRG) approach to nonequilibrium dynamics in quantum-impurity systems is presented. We demonstrate that the method is suitable for fermionic as well as bosonic baths. Comparisons with exact analytical results for the charge relaxation in the resonant-level model and for dephasing in the spin-boson model establish the accuracy of the method. The real-time dynamics of a single spin coupled to each type of bath is investigated. We use the TD-NRG to calculate the spin relaxation and spin precession of a single Kondo impurity. The short- and long-time dynamics are studied as a function of temperature in the ferromagnetic and antiferromagnetic regimes. The short-time dynamics agrees very well with analytical results obtained at second order in the exchange coupling JJJ. In the ferromagnetic regime, the transient spin decay is described by the scaling variable $x=2{\ensuremath{\rho}}_{F}\ensuremath{\mid}J(T)\ensuremath{\mid}Tt$. In the antiferromagnetic regime, the long-time decay is governed for T<TKT<{T}_{K}T<TK​ by the Kondo time scale 1∕TK1∕{T}_{K}1∕TK​. Here ${\ensuremath{\rho}}_{F}$ is the conduction-electron density of states, TK{T}_{K}TK​ is the Kondo temperature, and J(T)J(T)J(T) is the effective exchange coupling at temperature TTT. Results for spin precession are obtained by rotating the external magnetic field from the xxx axis to the zzz axis.
We investigate the equilibrium and real-time properties of the spin-correlation function $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$ in the two-impurity Kondo model for different distances RRR between the two-impurity spins. It is shown that the competition between the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction and the Kondo effect governs the amplitude of $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$. For distances RRR exceeding the Kondo length scale, the Kondo effect also has a profound effect on the sign of the correlation function. For ferromagnetic Heisenberg couplings JJJ between the impurities and the conduction band, the Kondo effect is absent and the correlation function only decays for distances beyond a certain length scale introduced by finite temperature. The real-time dynamics after a sudden quench of the system reveals that correlations propagate through the conduction band with Fermi velocity. We identify two distinct timescales for the long-time behavior, which reflects that for small JJJ the system is driven by the RKKY interaction while for large JJJ the Kondo effect dominates. Interestingly, we find that at certain distances a one-dimensional dispersion obeying $\ensuremath{\epsilon}(k)=\ensuremath{\epsilon}(\ensuremath{-}k)$ may lead to a local parity conservation of the impurities such that $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$ becomes a conserved quantity for long times and does not decay to its equilibrium value.