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Optical pumping of a dense quantum gas at its limits : continuous Sisyphus cooling and demagnetization cooling towards degeneracy

Valentin Volchkov

Published Jan 1, 2013• 0 citations
Publisher

Abstract

In this thesis, I study optical pumping as a powerful cooling tool for trapped ultra-cold atoms in a highly collisional regime. First application of optical pumping is a continuous loading scheme used to transfer atoms from a guided beam into a hybrid trap. Further, I introduce a Sisyphus cooling scheme based on radio-frequency transitions and optical pumping, operating simultaneously to the accumulation of atoms in the trap. The combined scheme of continuous loading and Sisyphus cooling is demonstrated for a large range of initial conditions of the guided atoms. Thereby, I show that collisional thermalization occurs in a steady-state for almost arbitrary initial conditions, provided that the first dissipative step is able to prevent the atom from leaving the trap during its first passage. On the one hand, this scheme could be applied to a wide range of atomic or molecular beams. On the other hand, phase-space density of 4*10^-4 is reached in a continuous operation mode with chromium atoms. In the second part, I investigate demagnetization cooling based on dipolar relaxation collisions driving the thermalization of the internal (spin) and the external (motional) degrees of freedom. In the case of a gas, one has the advantage that the spin degree of freedom can be cooled very efficiently using optical pumping. It is shown, that demagnetization cooling of a gas is more efficient than evaporation cooling in terms of phase-space density gain versus loss of atoms. This allows reaching a temperature of 6uK at a phase-space density of 0.03. It is observed, that both, continuous Sisyphus cooling and demagnetization cooling are limited by a density dependent loss mechanism. I present circumstantial evidence for excited-state collisions as the dominant limiting process. Finally, I discuss possible extensions to the current experimental procedures, possibly allowing reaching quantum degeneracy by optical means only.

DOI
10.18419/opus-5116

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In the last decades, experimental access to the quantum regime has been gained in a large variety of systems, including dilute ultracold gases, trapped ions, micromechanical oscillators, superconducting circuits, and many more.These systems allow for such exciting applications as quantum computing and communication, quantum metrology and quantum simulation.A physical system's quantum mechanical features can only be revealed by cooling it until the thermal excitations are negligible.To date, the coldest temperatures are reached with ultracold gases by a combination of laser cooling and evaporation, inherently producing individual ensembles.However, many applications can greatly benefit from a continuous source of ultracold atoms, for example sympathetic cooling of molecules or nanoscopic objects.Ideally, this cooling source operates without light, as most molecules have a rich internal structure and can absorb photons of many wavelengths.Another promising application of continuous sources of ultracold matter is atom interferometry.Such interferometers perform measurements of inertial forces, time and gravity.Currently, each cold sample is destroyed by its evaluation and the measurement is interrupted by the preparation of a new samples.Continuous sources can help to eliminate this restriction.So far, no dark and continuous sources exist in the microkelvin regime.This thesis presents the first preparation of such an ultracold atom cloud which is continuously replenished and protected from light.The continuously refilled reservoir is prepared by loading a magnetically guided atom beam into an elongated magnetic trapping potential.This static potential has an entrance barrier which allows atoms from a guided beam to enter the trap.Once in the trap, the atoms undergo collisions and redistribute their kinetic energy.Those gaining energy can escape again, but those losing energy are trapped.A steady state with 3.8 × 10 7 atoms atoms at a temperature of 102 µK is reached and maintained.The setup of the continuous loading scheme is described in this thesis.A key component is a mesoscopic atom chip which produces all magnetic fields for the continuous loading scheme.The initial atom source is a high-flux double magneto-optical trap system.An atomic beam is created out of the precooled atoms and guided to the static trap through a stray light protection allowing for a dark retrapping region.The cooling scheme does not rely on any specific atomic properties of the atoms and can thus be applied to a wide range of particles.The results offer exciting perspectives for an application as a continuous source of ultracold atoms, either as a coolant for sympathetic cooling or as a resource for metrology.

•Jan 1, 2015•4 citations
In this thesis, I study optical pumping as a powerful cooling tool for trapped ultra-cold atoms in a highly collisional regime. First application of optical pumping is a continuous loading scheme used to transfer atoms from a guided beam into a hybrid trap. Further, I introduce a Sisyphus cooling scheme based on radio-frequency transitions and optical pumping, operating simultaneously to the accumulation of atoms in the trap. The combined scheme of continuous loading and Sisyphus cooling is demonstrated for a large range of initial conditions of the guided atoms. Thereby, I show that collisional thermalization occurs in a steady-state for almost arbitrary initial conditions, provided that the first dissipative step is able to prevent the atom from leaving the trap during its first passage. On the one hand, this scheme could be applied to a wide range of atomic or molecular beams. On the other hand, phase-space density of 4*10^-4 is reached in a continuous operation mode with chromium atoms. In the second part, I investigate demagnetization cooling based on dipolar relaxation collisions driving the thermalization of the internal (spin) and the external (motional) degrees of freedom. In the case of a gas, one has the advantage that the spin degree of freedom can be cooled very efficiently using optical pumping. It is shown, that demagnetization cooling of a gas is more efficient than evaporation cooling in terms of phase-space density gain versus loss of atoms. This allows reaching a temperature of 6uK at a phase-space density of 0.03. It is observed, that both, continuous Sisyphus cooling and demagnetization cooling are limited by a density dependent loss mechanism. I present circumstantial evidence for excited-state collisions as the dominant limiting process. Finally, I discuss possible extensions to the current experimental procedures, possibly allowing reaching quantum degeneracy by optical means only.
Demagnetization cooling relies on spin-orbit coupling that brings motional and spin degrees of freedom into thermal equilibrium. In the case of a gas, one has the advantage that the spin degree of freedom can be cooled very efficiently using optical pumping. We investigate demagnetization cooling of a chromium gas in a deep optical dipole trap over a large temperature range and reach high densities up to $5\ifmmode\times\else\texttimes\fi{}{10}^{19}$ m${}^{\ensuremath{-}3}$. We study the loss mechanism under such extreme conditions and identify excited-state collisions as the main limiting process. We discuss that in some systems demagnetization cooling has a realistic potential of reaching degeneracy by optical cooling only.
We demonstrate continuous Sisyphus cooling combined with a continuous loading mechanism used to efficiently slow down and accumulate chromium atoms from a guided beam. While the loading itself is based on a single slowing step, applying a radio frequency field forces the atoms to repeat this step many times resulting in a so-called Sisyphus cooling. This extension allows efficient loading and cooling of atoms from a wide range of initial beam conditions. We study the interplay of the continuous loading and simultaneous Sisyphus cooling in different density regimes. In the case of a low density flux we observe a differential gain in phase-space density of nine orders of magnitude. This makes the presented scheme an ideal tool for reaching collisional densities enabling evaporative cooling—in spite of unfavourable initial conditions.
This thesis examines two complimentary methods for the laser cooling of a magnetically guided ultra-cold atom beam. If combined, these methods could serve as a starting point for high-through put and possibly even continuous production of Bose-Einstein condensates. First, a mechanism is outlined to harvest ultra cold atoms from a magnetically guided atom beam into an optical dipole trap. A continuous loading scheme is described that dissipates the directed kinetic energy of a captured atom via deceleration by a magnetic potential barrier followed by optical pumping to the energetically lowest Zeeman sublevel. The application of this scheme to the transfer of ultra cold chromium atoms from a magnetically guided atom beam into a deep optical dipole trap is investigated via numerical simulations of the loading process. Based on the results of the theoretical studies the feasibility and the efficiency of our loading scheme, including the realisation of a suitable magnetic field configuration, are analysed. Second, experiments were conducted on the transverse laser cooling of a magnetically guided beam of ultra cold chromium atoms. Radial compression by a tapering of the guide is employed to adiabatically heat the beam. Inside the tapered section heat is extracted from the atom beam by a two-dimensional optical molasses perpendicular to it, resulting in a significant increase of atomic phase space density. A magnetic offset field is applied to prevent optical pumping to untrapped states. Our results demonstrate that by a suitable choice of the magnetic offset field, the cooling beam intensity and detuning, atom losses and longitudinal heating can be avoided. Final temperatures below 65 µK have been achieved, corresponding to an increase of phase space density in the guided beam by more than a factor of 30.
Demagnetization cooling utilizes dipolar relaxations that couple the internal degree of freedom (spin) to the external (angular momentum) in order to cool an atomic cloud efficiently. Optical pumping into a dark state constantly recycles the atoms that were thermally excited to higher spin states. The net energy taken away by a single photon is very favorable since the lost energy per atom is the Zeeman energy rather than the recoil energy. As the density of the atomic sample rises the presence of the photons leads to limiting processes. In our previous publication [Volchkov et al. (2014)] we have shown that light-assisted collisions are such an important limiting process. In this paper we suppress light-assisted collisions by detuning the optical pumping light such that the Condon point coincides with the first node of the ground state wave function of two colliding atoms. This leads to an increased cooling efficiency χ ≥ 17 as well as to increased maximum densities of n ≈ 1 · 10(20) m(-3). However, due to the high number of involved molecular states the net suppression is not strong enough to reach quantum degeneracy.
In this thesis I describe two non-evaporative cooling schemes for cooling Rb atoms. The first is a Sisyphus-like ultracold gas cooling scheme called Spatially-selecTive Optical Pumping (STOP) cooling. In principle, STOP cooling has wide applicability to both atoms and molecules. STOP cooling works by exploiting the fact that atoms or molecules in a confining potential can be optically pumped out of an otherwise dark state in a spatially-selective way. Selecting atoms or molecules for optical pumping out of a dark state in a region of high potential energy and then waiting a fixed time after the optical pumping allows for the creation of a group of high kinetic energy atoms or molecules moving in a known direction. These can then be slowed using external fields (such as the scattering force from a resonant laser beam) and optically pumped back into the dark state, cooling the gas and closing the cooling cycle. I present theoretical modeling of the STOP cooling technique, including predictions of achievable cooling rates. I have conducted an experimental study of the cooling technique for a single cooling cycle, observing one dimensional cooling rates in excess of 100 micro-K per second in an ultracold gas of 87Rb atoms. I will also comment on the prospects for improving the cooling performance beyond that presented in this work. The second cooling scheme I investigated is called Two-Isotope Collision Assisted Zeeman (2-CAZ) cooling. Through a combination of spin-exchange collisions in a magnetic field and optical pumping, it is possible to cool a gas of atoms without requiring the loss of atoms from the gas. I investigated 2-CAZ cooling using 85Rb and 87Rb. I was able to experimentally confirm that the measured 2-CAZ cooling rate agreed with a cooling rate predicted though a simple analytic model. As part of the measured cooling rate, I quantitatively characterized the heating rates associated with our actual implementation of this cooling technique and found hyperfine-changing collisions to be a significant limitation for the 85/87Rb gas mixture. Possible improvements to this experiment will be discussed as well as the prospects for improved cooling performance using an atom without hyperfine structure as the optically pumped atom.
In the last decades, experimental access to the quantum regime has been gained in a large variety of systems, including dilute ultracold gases, trapped ions, micromechanical oscillators, superconducting circuits, and many more.These systems allow for such exciting applications as quantum computing and communication, quantum metrology and quantum simulation.A physical system's quantum mechanical features can only be revealed by cooling it until the thermal excitations are negligible.To date, the coldest temperatures are reached with ultracold gases by a combination of laser cooling and evaporation, inherently producing individual ensembles.However, many applications can greatly benefit from a continuous source of ultracold atoms, for example sympathetic cooling of molecules or nanoscopic objects.Ideally, this cooling source operates without light, as most molecules have a rich internal structure and can absorb photons of many wavelengths.Another promising application of continuous sources of ultracold matter is atom interferometry.Such interferometers perform measurements of inertial forces, time and gravity.Currently, each cold sample is destroyed by its evaluation and the measurement is interrupted by the preparation of a new samples.Continuous sources can help to eliminate this restriction.So far, no dark and continuous sources exist in the microkelvin regime.This thesis presents the first preparation of such an ultracold atom cloud which is continuously replenished and protected from light.The continuously refilled reservoir is prepared by loading a magnetically guided atom beam into an elongated magnetic trapping potential.This static potential has an entrance barrier which allows atoms from a guided beam to enter the trap.Once in the trap, the atoms undergo collisions and redistribute their kinetic energy.Those gaining energy can escape again, but those losing energy are trapped.A steady state with 3.8 × 10 7 atoms atoms at a temperature of 102 µK is reached and maintained.The setup of the continuous loading scheme is described in this thesis.A key component is a mesoscopic atom chip which produces all magnetic fields for the continuous loading scheme.The initial atom source is a high-flux double magneto-optical trap system.An atomic beam is created out of the precooled atoms and guided to the static trap through a stray light protection allowing for a dark retrapping region.The cooling scheme does not rely on any specific atomic properties of the atoms and can thus be applied to a wide range of particles.The results offer exciting perspectives for an application as a continuous source of ultracold atoms, either as a coolant for sympathetic cooling or as a resource for metrology.