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Quantum Electronics and Laser Science Conference

Spectroscopy with squeezed fields

Z. Ficek

Published Jun 7, 1996• 0 citations
OpenAlex

Abstract

Summary form only given. We extend the analytical technique to the case of a fully quantized dressed-atom model with a detuned driving laser field and incorporate the cavity effect on the fluorescence spectrum. We find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth squeezed vacuum only if there is nonzero squeezing at the Rabi sidebands. We show that this condition is readily achieved with a squeezed vacuum that is the output from a nondegenerate parametric oscillator, whereas for a squeezed vacuum that is the output from a degenerate parametric oscillator a squeezing bandwidth comparable to the Rabi frequency is required.

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Spectral linewidth narrowing by a narrow bandwidth squeezed vacuum in a cavity

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The fluorescence spectrum of a strongly driven two-level atom located inside an optical cavity damped by a narrow-bandwidth squeezed vacuum is studied. We use a dressed atom model approach, first applied to squeezed vacuum problems by Yeoman and Barnett, to derive the master equation of the system and discuss the role of the cavity and the squeezed vacuum in the narrowing of the spectral lines and the population trapping effect. We find that in the presence of a single-mode cavity the effect of squeezing on the fluorescence spectrum is more evident in the linewidths of the Rabi sidebands rather than in the linewidth of the central component. Even in the absence of squeezing, the cavity can reduce the linewidth of the central component almost to zero, whereas the Rabi sidebands can be narrowed only to some finite value. In the presence of a two-mode cavity and a two-mode squeezed vacuum the signature of squeezing is evident in the linewidths of all spectral lines. We also establish that the narrowing of the spectral lines is very sensitive to the detuning of the driving field from the atomic resonance. Moreover, we find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth case only if the input squeezed modes are perfectly matched to the cavity modes and if there is non-zero squeezing at the Rabi sidebands.

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Two-level atom in a squeezed vacuum with finite bandwidth

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The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.

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Resonance fluorescence spectra of three-level atoms in a squeezed vacuum

M. R. Ferguson, Z. Ficek, Bryan J. Dalton

The fluorescence field from one of the two allowed transitions in a three-level atom can sense squeezed fluctuations of a vacuum field coupled to the other transition. We examine the fluorescence spectra of strongly driven three-level atoms in \ensuremath{\Lambda}, V, and cascade configurations in which one of the two one-photon transitions is coupled to a finite-bandwidth squeezed vacuum field, when the bandwidth is much smaller than the difference in the atomic transition frequencies, though much larger than atomic decay rates and Rabi frequencies of the driving fields. The driving fields are on one-photon resonance, and the squeezed vacuum field is generated by a degenerate parameter oscillator. Details are only given for the \ensuremath{\Lambda} configuration. The extension to the V and cascade configurations is straightforward. We find that in all configurations the fluorescence spectra of the transition not coupled to the squeezed vacuum field are composed of five lines, one central and two pairs of sidebands, with intensities and widths strongly influenced by the squeezed vacuum field. However, only the central component and the outer sidebands exhibit a dependence on the squeezing phase. We also examine the fluorescence spectrum for the cascade configuration with a squeezed vacuum field on resonance with the two-photon transition between the ground and the most excited states and now generated by a nondegenerate parametric oscillator. In this case, where the squeezed vacuum field can be made coupled to both transitions, all spectral lines depend on the squeezing phase. The spectral features are explained in terms of the dressed-atom model of the system. We show that the coherent mixing of the atomic states by the strong driving fields modifies transition rates between the dressed states, which results in the selective phase dependence of the spectral features. \textcopyright{} 1996 The American Physical Society.

Physical Review A•Sep 1, 1996•48 citations
Summary form only given. We extend the analytical technique to the case of a fully quantized dressed-atom model with a detuned driving laser field and incorporate the cavity effect on the fluorescence spectrum. We find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth squeezed vacuum only if there is nonzero squeezing at the Rabi sidebands. We show that this condition is readily achieved with a squeezed vacuum that is the output from a nondegenerate parametric oscillator, whereas for a squeezed vacuum that is the output from a degenerate parametric oscillator a squeezing bandwidth comparable to the Rabi frequency is required.
The fluorescence spectrum of a strongly driven two-level atom located inside an optical cavity damped by a narrow-bandwidth squeezed vacuum is studied. We use a dressed atom model approach, first applied to squeezed vacuum problems by Yeoman and Barnett, to derive the master equation of the system and discuss the role of the cavity and the squeezed vacuum in the narrowing of the spectral lines and the population trapping effect. We find that in the presence of a single-mode cavity the effect of squeezing on the fluorescence spectrum is more evident in the linewidths of the Rabi sidebands rather than in the linewidth of the central component. Even in the absence of squeezing, the cavity can reduce the linewidth of the central component almost to zero, whereas the Rabi sidebands can be narrowed only to some finite value. In the presence of a two-mode cavity and a two-mode squeezed vacuum the signature of squeezing is evident in the linewidths of all spectral lines. We also establish that the narrowing of the spectral lines is very sensitive to the detuning of the driving field from the atomic resonance. Moreover, we find that the population trapping effect, predicted for the broadband squeezed vacuum case, may appear in a narrow-bandwidth case only if the input squeezed modes are perfectly matched to the cavity modes and if there is non-zero squeezing at the Rabi sidebands.
The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.
The dynamics of a strongly driven two-level atom are examined for the case that the atom is coupled to a ``two-mode'' squeezed vacuum. The source of squeezed light is taken to be a (frequency) nondegenerate parametric oscillator. We consider the situation in which the Rabi sidebands produced by the coherent driving field coincide with the spectral peaks of the parametric oscillator. Approximate analytical results are presented and checked against numerical simulations of the exact equations. For a suitable choice of relative phase, all three spectral lines in the fluorescence triplet are found to exhibit subnatural linewidths. Significant modifications to the fluorescence spectrum are also possible with a nonzero laser-atom detuning.
We examine resonance fluorescence of a two-level atom in a squeezed vacuum, under the condition that the squeezing bandwidth is much narrower than the Rabi splitting of the Mollow triplet. For a suitable choice of the relative phase between the squeezed vacuum and coherent driving field, we find significant narrowing of the Rabi peaks and inhibited population decay. These results are in marked contrast to previous broadband squeezing analyses, which predict strong broadening of the Rabi peaks and enhanced population decay. We explore the connection between our work and that on the dynamical suppression of spontaneous emission via strongly driven resonance fluorescence in a cavity [Lewenstein, Mossberg, and Glauber, Phys. Rev. Lett. 59, 775 (1987)]. By modifying this work to incorporate squeezing of the cavity modes, we are able to combine the features of both systems, and thereby predict strong inhibition of the decay of all three components of the Bloch vector in a possible experimental configuration.
The authors present analytical and numerical results for resonance fluorescence produced by a two-level atom damped by a broad-band squeezed vacuum. Previous theoretical analyses of this model have assumed that the laser frequency and the carrier frequency of the squeezed vacuum are equal. The authors introduce a non-zero detuning between the laser frequency and the carrier frequency while maintaining resonance between the laser frequency and atomic resonance. In the absence of the driving field there is a squeezing threshold: above threshold the decay rate of the atomic polarization can be reduced, and below threshold a squeezing-induced two peak spectrum and frequency shift, which is analogous to the Bloch-Siegert shift, are predicted. In the presence of the driving field, the spectrum is asymmetric for Rabi frequencies smaller or comparable to the detuning of the squeezed vacuum. A symmetric spectrum is obtained for large Rabi frequencies. An interpretation is predicted by means of a dressed-state analysis. The authors find that for not too large Rabi frequencies a remarkably large population inversion can be induced in the dressed states, even at exact resonance of the driving field, provided that the laser frequency and carrier frequency are detuned. Moreover, for detection times larger than the inverse detuning, the spectrum is insensitive to the phase between the driving field and the squeezed vacuum, in marked contrast to the case of no detuning.
The fluorescence field from one of the two allowed transitions in a three-level atom can sense squeezed fluctuations of a vacuum field coupled to the other transition. We examine the fluorescence spectra of strongly driven three-level atoms in \ensuremath{\Lambda}, V, and cascade configurations in which one of the two one-photon transitions is coupled to a finite-bandwidth squeezed vacuum field, when the bandwidth is much smaller than the difference in the atomic transition frequencies, though much larger than atomic decay rates and Rabi frequencies of the driving fields. The driving fields are on one-photon resonance, and the squeezed vacuum field is generated by a degenerate parameter oscillator. Details are only given for the \ensuremath{\Lambda} configuration. The extension to the V and cascade configurations is straightforward. We find that in all configurations the fluorescence spectra of the transition not coupled to the squeezed vacuum field are composed of five lines, one central and two pairs of sidebands, with intensities and widths strongly influenced by the squeezed vacuum field. However, only the central component and the outer sidebands exhibit a dependence on the squeezing phase. We also examine the fluorescence spectrum for the cascade configuration with a squeezed vacuum field on resonance with the two-photon transition between the ground and the most excited states and now generated by a nondegenerate parametric oscillator. In this case, where the squeezed vacuum field can be made coupled to both transitions, all spectral lines depend on the squeezing phase. The spectral features are explained in terms of the dressed-atom model of the system. We show that the coherent mixing of the atomic states by the strong driving fields modifies transition rates between the dressed states, which results in the selective phase dependence of the spectral features. \textcopyright{} 1996 The American Physical Society.