Imaging systems play a crucial role in shaping understanding of our surroundings. Modern imaging systems enable the acquisition of images of objects at length-scales and resolutions previously deemed impossible. However, as the drive for better images and novel applications increases, several questions fundamental to our understanding of imaging are being raised. We are familiar with images containing many millions of photons, but how many photons does it take to form an image? In scenarios requiring covert imaging, or where high-light levels damage the sample being imaged, is it possible to image a sample with a very small number of very low-energy photons? This thesis will focus on answering these two questions. In order to answer these questions I developed a heralded quantum imaging system. The strong spatial correlations inherent between down-converted twin photons have been utilised in many quantum imaging techniques for the past 25 years. Thus far, standard quantum imaging techniques have relied on scanning a fibre detector across the field of view in order to measure the spatial information in the image. However, the scanning mechanism fundamentally limits the detection efficiency of the imaging system. Recent years have seen an increased interest in using the latest camera technology within quantum imaging systems. The advent of single-photon-sensitive cameras has opened up new possibilities within the quantum imaging field. It is now possible to obtain images of objects by detecting very low-light illumination across the full scene simultaneously. In the heralded quantum imaging system presented in this thesis, a combination of quantum mechanics and a high-sensitivity camera was employed to obtain high contrast images containing very few photons. This was the first such system built. Using the correlations between the twin photons generated by our down-conversion source, and our development of compressive sampling techniques to post-process the acquired data enabled the acquisition of an image containing an average of only 0.5 photons per pixel. This represents a significant reduction when compared with a conventional image that contains of order 105 photons per pixel. I also developed this imaging system to use twin photons at vastly different wave- lengths. The object was probed with low-energy infrared photons whilst the image was developed on a camera using the correlated visible photon. This disparity in energy between the two photons enabled the acquisition of images using only several thousand photons, corresponding to an energy deposition on the sample of only a few pJ.
Imaging systems play a crucial role in shaping understanding of our surroundings. Modern imaging systems enable the acquisition of images of objects at length-scales and resolutions previously deemed impossible. However, as the drive for better images and novel applications increases, several questions fundamental to our understanding of imaging are being raised. We are familiar with images containing many millions of photons, but how many photons does it take to form an image? In scenarios requiring covert imaging, or where high-light levels damage the sample being imaged, is it possible to image a sample with a very small number of very low-energy photons? This thesis will focus on answering these two questions. In order to answer these questions I developed a heralded quantum imaging system. The strong spatial correlations inherent between down-converted twin photons have been utilised in many quantum imaging techniques for the past 25 years. Thus far, standard quantum imaging techniques have relied on scanning a fibre detector across the field of view in order to measure the spatial information in the image. However, the scanning mechanism fundamentally limits the detection efficiency of the imaging system. Recent years have seen an increased interest in using the latest camera technology within quantum imaging systems. The advent of single-photon-sensitive cameras has opened up new possibilities within the quantum imaging field. It is now possible to obtain images of objects by detecting very low-light illumination across the full scene simultaneously. In the heralded quantum imaging system presented in this thesis, a combination of quantum mechanics and a high-sensitivity camera was employed to obtain high contrast images containing very few photons. This was the first such system built. Using the correlations between the twin photons generated by our down-conversion source, and our development of compressive sampling techniques to post-process the acquired data enabled the acquisition of an image containing an average of only 0.5 photons per pixel. This represents a significant reduction when compared with a conventional image that contains of order 105 photons per pixel. I also developed this imaging system to use twin photons at vastly different wave- lengths. The object was probed with low-energy infrared photons whilst the image was developed on a camera using the correlated visible photon. This disparity in energy between the two photons enabled the acquisition of images using only several thousand photons, corresponding to an energy deposition on the sample of only a few pJ.
The process of image recording is arguably one of the most prevalent technology in modern society and continues to inspire vast swathes of research due to its widespread applications spanning military, medical and consumer spheres. The danger present in a field so broad is that separate niches of research can become isolated with critical advancements struggling to traverse the gulfs between. Unifying the field is the omnipresent drive to acquire an ever increasing quality of images at the lowest possible cost, a goal which warrants continual fundamental research. Quantum entanglement exhibits many intriguing characteristics which make it a suitable tool for such fundamental investigations. The process of spontaneous parametric down- conversion has offered a yet unbeaten strength of photon correlations with the quantum nature of their production providing a reliable and controllable source of single-photons. Arising from these attributes is the technique known as ghost imaging. Though now known to be classically possible, the strength of entanglement generated correlations is yet to be surpassed. This thesis implemented this technique in tandem with the cutting edge detector technology in order to probe the fundamentals of image formation. This form of imaging allowed us to subject an object to a known number of photons whilst acquiring structural information from spatially separate, correlated photons which never interact with the object. The strength of the produced correlations allow us to acquire low background, high resolution images with far less light than traditional techniques and affords many novel benefits. The possibility of incorporating this technique with pre-existent regimes allowed me to draw from advancements made across the landscape of imaging research. Although referred to as “quantum ghost imaging” throughout this work, it should be noted that the intrinsic quantum nature of the correlations was not directly relied upon but provided an ideal source of strongly correlated photons. In order to determine the limits of a traditional imaging system this thesis first sought to answer the question: “can an image of an object be reconstructed from fewer photons than ii pixels in the image?” In chapter 3 I approached this from the perspective of compression, which minimises redundant information within a signal. This lead to the development of an imaging regime capable of imaging with far fewer photons than pixels in the image. By employing assumptions about the sparsity of natural images I was able to reconstruct an image of a biological sample containing an average of less than one photon per image pixel. Having reduced the number of photons necessary to form an image I then considered alternative methods for reducing the optical energy impinging on a sample. I sought to answer the question: “can non-degenerate ghost imaging reduce the optical energy impinged upon an object during imaging”. The photons produced in SPDC need not be of similar wavelengths, however may be chosen far from degeneracy, i.e. non-degenerate. In Chapter 4 I presented a ghost imaging system which illuminated the object with infrared light whilst recording the structural information via entangled visible photons. This allowed for objects opaque to visible light to be imaged in high quality without the need for a spatially resolving infrared detector, the state of the art of which lags behind their silicon based visible counterparts. I presented the systems capabilities by imaging objects which were etched into a gold substrate layered on to silicon, both of which are opaque to visible light. Not only did a reduction in energy deposition arise from the lower energy probe wavelength but applying the reconstruction techniques from the previous chapter brought that down to as low as ≈16 nJcm−2s−1. Seeking to expand the repertoire of applications, the low-light capabilities of my ghost imaging were applied to the technique of phase-contrast microscopy in chapter 5. Typically applied to translucent objects, phase-contrast imaging transfers phase information, i.e. the refractive index changed within the object, into an intensity distribution through the use of a phase-filter. In many of these applications the objects tend to be biological in nature, where high optical exposure can result in bleaching or damage. By applying the phase-filter non- locally, i.e. to the photons correlated to those probing the object, I acquired edge-enhanced images of a phase object whilst illuminating with significantly fewer photons than standard phase-contrast techniques. Having displayed the broad applicability of our low-light ghost imaging system, I then sought to determine the optical resolution in chapter 6. The resolution limits of ghost imaging are not clear at first glance owing to the resolutions dependence upon the strength of spatial correlations. As the length over which the spatial correlations are produced can be brought below the standard diffraction limit, it would seem the resolution of the system could be brought similarly low. To clarify this I artificially restricted the number of spatial modes in each of the correlated beams to uncover the physically realisable resolution. I show that although the resolution of a ghost imaging system to be fundamentally determined by the strength of the correlations, this can never be reached due to the inherent limitations of the intervening imaging system.
Correlated-photon imaging, popularly known as ghost imaging, is a technique whereby an image is formed from light that has never interacted with the object. In ghost imaging experiments two correlated light fields are produced. One of these fields illuminates the object, and the other field is measured by a spatially resolving detector. In the quantum regime, these correlated light fields are produced by entangled photons created by spontaneous parametric down-conversion. To date, all correlated-photon ghost-imaging experiments have scanned a single-pixel detector through the field of view to obtain the spatial information. However, scanning leads to a poor sampling efficiency, which scales inversely with the number of pixels, N, in the image. In this work we overcome this limitation by using a time-gated camera to record the single-photon events across the full scene. We obtain high-contrast images, 90%, in either the image plane or the far-field of the photon pair source, taking advantage of the EPR-like correlations in position and momentum of the photon pairs. Our images contain a large number of modes, >500, creating opportunities in low-light-level imaging and in quantum information processing.
Classical light sources emit a randomly-timed stream of individual photons, the spatial distribution of which can be detected with a camera to form an image. Quantum light sources, based on parametric down conversion, emit photons as correlated photon-pairs. The spatial correlations between the photons enables imaging systems where the preferential selection of photon-pairs allows for enhancements in the noise performance over what is possible using classical light sources. However, until now the technical challenge of measuring, and correlating both photons has led to system complexity. Here we show that a camera capable of resolving the number of individual photons in each pixel of the detector array can be used to record an image formed from these photon-pair events and hence achieve a greater contrast than possible using a classical light source. We achieve an enhancement in the ratio of two-photon events compared to one-photon events using spatially correlated SPDC light compared to uncorrelated illumination by a LED. These results indicate the potential advantages of using photon counting cameras in quantum imaging schemes and these advantages will further increase as the technology is developed. Operating in photon sparse regimes such systems have potential applications in low-light microscopy and covert imaging.
Correlated photon imaging, popularly known as ghost imaging, is a technique whereby an image is formed from light that has never interacted with the object. In ghost imaging experiments, two correlated light fields are produced. One of these fields illuminates the object, and the other field is measured by a spatially resolving detector. In the quantum regime, these correlated light fields are produced by entangled photons created by spontaneous parametric down-conversion. To date, all correlated photon ghost imaging experiments have scanned a single-pixel detector through the field of view to obtain spatial information. However, scanning leads to poor sampling efficiency, which scales inversely with the number of pixels, N , in the image. In this work, we overcome this limitation by using a time-gated camera to record the single-photon events across the full scene. We obtain high-contrast images, 90%, in either the image plane or the far field of the photon pair source, taking advantage of the Einstein–Podolsky–Rosen-like correlations in position and momentum of the photon pairs. Our images contain a large number of modes, >500, creating opportunities in low-light-level imaging and in quantum information processing.
Extracting as much information as possible about an object when probing with a limited number of photons is an important goal with applications from biology and security to metrology. Imaging with a few photons is a challenging task as the detector noise and stray light are then predominant, which precludes the use of conventional imaging methods. Quantum correlations between photon pairs has been exploited in a so called 'heralded imaging scheme' to eliminate this problem. However these implementations have so-far been limited to intensity imaging and the crucial phase information is lost in these methods. In this work, we propose a novel quantum-correlation enabled Fourier Ptychography technique, to capture high-resolution amplitude and phase images with a few photons. This is enabled by the heralding of single photons combined with Fourier ptychographic reconstruction. We provide experimental validation and discuss the advantages of our technique that include the possibility of reaching a higher signal to noise ratio and non-scanning Fourier Ptychographic acquisition.
Quantum imaging encompasses a broad range of methods that exploit the quantum properties of light to capture information about an object. One such approach involves using a two-photon quantum state, where only one photon interacts with the object being imaged while its entangled partner carries spatial or temporal information. To implement this technique, it is necessary to generate specific quantum states of light and detect photons at the single-photon level. While this method has been successfully demonstrated in the visible electromagnetic spectrum, extending it to X-rays has faced significant challenges due to the difficulties in producing a sufficient rate of X-ray photon pairs and detecting them with adequate resolution. Here, we demonstrate record high rates of correlated X-ray photon pairs produced via a spontaneous parametric down-conversion process and we employ these photons to perform quantum correlation imaging of several objects, including a biological sample (E. cardamomum seedpod). Notably, we report an unprecedented detection rate of about 6,300 pairs per hour and the observation of energy anti-correlation for the X-ray photon pairs. We also present a detailed analysis of the properties of the down-converted X-ray photons, as well as a comprehensive study of the correlation imaging formation, including a study of distortions and corrections. These results mark a substantial advancement in X-ray quantum imaging, expanding the possibilities of X-ray quantum optical technologies, and illustrating the pathway towards enhancing biological imaging with reduced radiation doses.