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Conference on Lasers and Electro-Optics

Precision measurements with coherent dark resonances

R. Wynands, A. Nagel, L. Graf, Sebastián Brandt, Dieter Meschede, A. Naumov

Published Nov 27, 2002• 0 citations
Publisher

Abstract

Summary form only given.We consider coherent dark resonances in Cs vapor cells where the effective interaction time between atoms and light is increased through the addition of a buffer gas or through a coating of the cell walls with siloxane. The light sources are two diode lasers phase locked at 9.2 GHz frequency difference, corresponding to the hyperfine splitting of cesium. The phase-locked loop eliminates difference frequency jitter and leads to resonances narrower than 50 Hz, which can be applied to various precision experiments.

DOI
10.1109/iqec.1998.680298

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Chinese Physics B•Apr 1, 2013•3 citations
Summary form only given.We consider coherent dark resonances in Cs vapor cells where the effective interaction time between atoms and light is increased through the addition of a buffer gas or through a coating of the cell walls with siloxane. The light sources are two diode lasers phase locked at 9.2 GHz frequency difference, corresponding to the hyperfine splitting of cesium. The phase-locked loop eliminates difference frequency jitter and leads to resonances narrower than 50 Hz, which can be applied to various precision experiments.
When neon is introduced as a buffer gas the interaction time of cesium atoms in a vapor cell with resonant laser beams is drastically increased. Using a pair of phase-locked lasers we have observed linewidths as narrow as $42 $Hz for coherent dark resonances in a cesium vapor cell. We study the influence of power and pressure broadening and systematic shifts of the resonance frequency. Our experiments demonstrate that coherent dark resonances could rival direct radio-frequency precision measurements, which have a wide range of applications in physics.
Summary form only given, as follows.The 30 kHz linewidth and extremely steep dispersion of a coherent dark resonance in a caesium vapor cell allows measurements of magnetic fields to about 10 nT in 0.1 s integration time, limited by stray fields. The narrow resonance should make possible a compact frequency standard. In a preliminary experiment the authors used a coherent dark resonance in a 2 cm long caesium vapor cell to measure magnetic fields with about 10-5 uncertainty. Two diode lasers (852 nm wavelength) were phase-locked onto each other with a 9.2 GHz frequency offset, corresponding to the frequency ground state separation of the two caesium levels. The difference frequency is derived from a stable tunable rf source. Absorption spectrum of the caesium coherent population trapping resonance for linear laser polarizations is illustrated; it is split into seven components by a magnetic field parallel to the laser polarization direction. The width of the individual lines is only 130 kHz due to power broadening. The steep slope of the resonance could be used to lock the frequency of the 9.2 GHz rf source. This would provide a compact frequency reference.
Summary form only given. We report on recent experiments to use dark line coherent population trapping (CPT) resonances in cesium vapor as the basis for a compact frequency reference. The resonance is excited by directly modulating the injection current of a VCSEL at one-half the ground state hyperfine transition of Cs (4.6 GHz) to produce RF sidebands on the optical carrier. The laser output is then passed through a room-temperature cell containing Cs at its vapor pressure together with 8.7 kPa of Neon buffer gas and the transmitted optical power is detected in a photodiode. When the laser carrier is tuned half way between the two hyperfine components of the D/sub 2/ line at 852 nm, and the RF modulation frequency is adjusted to be equal to one-half the hyperfine splitting, the absorption of the sidebands through the cell is slightly reduced due to the CPT effect. As the RF frequency is scanned over the resonance, lock-in detection is used to produce a /spl sim/1 kHz wide dispersive error signal which is in turn used to stabilize the modulation frequency. The narrow signal is the result of the buffer gas, which reduces the time-of-flight broadening of the transition.
The coherent dark resonance between the hyperfine levels F=1, m F =0 and F=2, m F =0 of the rubidium ground state has been observed experimentally with the light of a pulsed mode-locked diode laser operating at the D1 transition frequency. The resonance occurs whenever the pulse repetition frequency matches an integer fraction of the rubidium 87 ground state hyperfine splitting of 6.8 GHz. Spectra have been taken by varying the pulse repetition frequency. Using cells with argon as a buffer gas a linewidth as narrow as 149 Hz was obtained. The rubidium ground state decoherence cross section for collisions with xenon atoms has been measured for the first time with this method using a pure isotope rubidium vapor cell and xenon as a buffer gas.
Summary form only given. We have experimentally investigated the potential of narrow coherent population trapping resonances for precision applications like magnetometry or atomic frequency standards. CPT can be observed in /spl Lambda/ systems where two ground states are coupled to a common excited state by two near-resonant light fields. Effective formation of ground state coherences takes place when the frequency difference of the light fields precisely matches the ground state splitting. This process leads to reduced absorption in the medium (electromagnetically induced transparency) and thus reduced fluorescence intensity (dark resonance) at the optical resonance frequency. Extremely narrow dark resonances can be observed when the two light fields have fixed phase and frequency difference and time-of-flight broadening is suppressed by the use of a buffer gas, making this type of system a promising candidate for precision applications. The /spl Lambda/ systems under study here are the D/sub 2/ lines of Cs, /sup 87/Rb and /sup 85/Rb where the ground state hyperfine splittings are 9.2 GHz, 6.8 GHz, and 3.0 GHz, respectively. Thus in a magnetic field the CPT resonance splits into several Zeeman components whose frequency positions are determined by the Breit-Rabi formula.
We present a pair of phase-locked lasers with a 9.2-GHz frequency difference through the injection locking of a master laser to the RF-modulation sideband of a slave diode laser. Using this laser system, a coherent population trapping (CPT) signal with a typical linewidth of ∼ 182 Hz is obtained in a cesium vapor cell filled with 30 Torr (4 kPa) of neon as the buffer gas. We investigate the influence of the partial pressure of the neon buffer gas on the CPT linewidth, amplitude, and frequency shift. The results may offer some references for CPT atomic clocks and CPT atomic magnetometers.