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Acta Physica Sinica

Study of odd-parity states of Sm atom with two-photon ionization detection method

Ming Li, Dai Chang-Jian, Xie Jun

Published Jan 1, 2010• 2 citations
Publisher

Abstract

摘要 采用两台激光器对Sm原子奇宇称激发态的光谱及其特性进行了系统研究.利用一台波长在585 nm到663 nm之间调谐的染料激光器,将Sm原子从某个4f66s27FJ(J=0—6)态激发到具有奇宇称的4f66s6p或4f55d6s2激发态.然后,采用波长固定在532 nm的强激光束,对处于上述奇宇称激发态的Sm原子进行双光子电离,以实现探测其光谱信息 关键词: 双光子电离 / 奇宇称态 / Sm原子 Abstract In this paper, spectra of odd-parity states of Sm atom are systematically studied with two-photon ionization detection method. The Sm atom is excited by a pulsed dye laser and scanned from 585 nm to 663 nm, so that it is populated in different odd-parity states with 4f66s6p and 4f55d6s2 electronic configurations from one of the 4f66s27FJ(J=0—6) states. Then the Sm atom is further excited and ionized by a two-photon transition with a second laser which has a much higher intensity and a fixed wavelength. The Sm ions emerging from the above processes were detected by an MCP detector. Some of the transitions are reported for the first time together with their resonance wavelengths and relative strengths, while the rest of them which have been reported previously in the litcrature are confirmed by the present work with supplementary information on their relative strengths. Keywords: two-photon ionization / odd-parity states / Sm atom 作者及机构信息 李鸣, 戴长建, 谢军 1. 天津理工大学主校区理学院,天津 300384 基金项目: 国家自然科学基金(批准号:10574098,10674102)、天津市自然科学基金(批准号:05YFJMJC05200)资助的课题. Authors and contacts Li Ming, Dai Chang-Jian, Xie Jun 1. 天津理工大学主校区理学院,天津 300384 参考文献 [1] [1]Li S B, Dai C J, Sun W, Xue P 2001 J. Phys. B 34 2123 [2] [2]Huang W, Xu X Y, Xu C B, Xue P, Xue M, Chen D Y 1996 Phys. Rev. A 54 5423 [3] [3]Quan W, Liu H P, Shen L, Zhan M S 2007 Chin. Phys. 16 3642 [4] [4]Camus P, Gallagher T F, Lecomte J M, Pillet P, Pruvost L 1989 Phys. Rev. Lett. 62 2365 [5] [5]Fedoseev V N, Mishin V I, Vedeneev D S, Zuzikov A D 1991 J. Phys. B 24 1575 [6] [6]Ding X B, Dong C Z, Fumihiro K, Takato K, Stephan F 2008 Chin. Phys. B 17 0592 [7] [7]Vidolova E P, Krustev T B, Angelov D A, Mincheva S 1997 J. Phys. B 30 667 [8] [8]Zhang L J, Feng Z G, Li A L, Zhao J M, Li G Y, Jia S T 2009 Chin. Phys. B 18 1838 [9] [9]Liang L, Wang Y C, Chao Z, Qiang W C 2007 J. Phys. B 75 127 [10] ]Lange V, Aymar M, Eichmann U, Sandner W 1991 J. Phys. B 24 91 [11] ]Raheel A, Yaseen M, Nadeem A, Bhatti S A, Baig M A 1999 J. Phys. B 32 953 [12] ]Raheel A, Nadeem A, Yaseen M, Aslam M, Bhatti S A, Baig M A 1999 J. Phys. B 32 4361 [13] ]Yi J, Park H, Lee J 1998 J. Kore. Phys. Soci. 5 916 [14] ]Hu S F, Zhang S, Mei S M, Qiu J Z, Chen X 1990 J. Quant. Spectrosc. Radiat. Transfer 1 75 [15] ]Hu S F, Mei S M, Zhang S, Chen X, Xu Y F 1990 Chin. Phys. Lett. 6 64 [16] ]Hu S F, Qiu J Z, Wang G, Liang Y, Chen X 1989 Acta. Phys. Sin. 38 487 (in Chinese) [胡素芬、 邱济真、 张森、 王刚、 梁宜、 陈星 1989 物理学报 38 487] [17] ]Jia L, Jing C Y, Zhou Z Y, Liu F C 1992 J. Opt. Soc. Am. B 10 1317 [18] ]Jayasekharan T, Razvi M A N, Bhale G L 2000 J. Phys. B 33 3123 [19] ]Nakhate S G, Razvi M A N, Connerade J P, Ahmad S A 2000 J. Phys. B 33 5191 [20] ]Pulhani A K, Shah M L, Dev V, Suri B M 2004 J. Opt. Soc. Am. B 22 1117 [21] ]Park H, Kim H, Yi J, Han J, Rhee Y, Lee J 1998 J. Kore. Phys. Soci. 33 288 [22] ]Gononai A I, Plekan O I 2003 J. Phys. B 36 4155 [23] ]Guan F, Dai C J, Zhao H Y 2008 Chin. Phys. B 17 3655 [24] ]Martin W C, Zalubas R, Hagan L 1978 Atomic Energy Levels-The Rare-Earth Elements, NSRDS-NBS60 (U.S. GPO, Washington, D.C.) p162 [25] ]Zhao H Y, Dai C J, Guan F 2009 J. Phys. B 42 065001 [26] ]Zhao H Y, Dai C J, Cuan F 2009 Chin. Phys. B 58 0215 施引文献

DOI
10.7498/aps.59.3154

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摘要 采用两台激光器对Sm原子奇宇称激发态的光谱及其特性进行了系统研究.利用一台波长在585 nm到663 nm之间调谐的染料激光器,将Sm原子从某个4f66s27FJ(J=0—6)态激发到具有奇宇称的4f66s6p或4f55d6s2激发态.然后,采用波长固定在532 nm的强激光束,对处于上述奇宇称激发态的Sm原子进行双光子电离,以实现探测其光谱信息 关键词: 双光子电离 / 奇宇称态 / Sm原子 Abstract In this paper, spectra of odd-parity states of Sm atom are systematically studied with two-photon ionization detection method. The Sm atom is excited by a pulsed dye laser and scanned from 585 nm to 663 nm, so that it is populated in different odd-parity states with 4f66s6p and 4f55d6s2 electronic configurations from one of the 4f66s27FJ(J=0—6) states. Then the Sm atom is further excited and ionized by a two-photon transition with a second laser which has a much higher intensity and a fixed wavelength. The Sm ions emerging from the above processes were detected by an MCP detector. Some of the transitions are reported for the first time together with their resonance wavelengths and relative strengths, while the rest of them which have been reported previously in the litcrature are confirmed by the present work with supplementary information on their relative strengths. Keywords: two-photon ionization / odd-parity states / Sm atom 作者及机构信息 李鸣, 戴长建, 谢军 1. 天津理工大学主校区理学院,天津 300384 基金项目: 国家自然科学基金(批准号:10574098,10674102)、天津市自然科学基金(批准号:05YFJMJC05200)资助的课题. Authors and contacts Li Ming, Dai Chang-Jian, Xie Jun 1. 天津理工大学主校区理学院,天津 300384 参考文献 [1] [1]Li S B, Dai C J, Sun W, Xue P 2001 J. Phys. B 34 2123 [2] [2]Huang W, Xu X Y, Xu C B, Xue P, Xue M, Chen D Y 1996 Phys. Rev. A 54 5423 [3] [3]Quan W, Liu H P, Shen L, Zhan M S 2007 Chin. Phys. 16 3642 [4] [4]Camus P, Gallagher T F, Lecomte J M, Pillet P, Pruvost L 1989 Phys. Rev. Lett. 62 2365 [5] [5]Fedoseev V N, Mishin V I, Vedeneev D S, Zuzikov A D 1991 J. Phys. B 24 1575 [6] [6]Ding X B, Dong C Z, Fumihiro K, Takato K, Stephan F 2008 Chin. Phys. B 17 0592 [7] [7]Vidolova E P, Krustev T B, Angelov D A, Mincheva S 1997 J. Phys. B 30 667 [8] [8]Zhang L J, Feng Z G, Li A L, Zhao J M, Li G Y, Jia S T 2009 Chin. Phys. B 18 1838 [9] [9]Liang L, Wang Y C, Chao Z, Qiang W C 2007 J. Phys. B 75 127 [10] ]Lange V, Aymar M, Eichmann U, Sandner W 1991 J. Phys. B 24 91 [11] ]Raheel A, Yaseen M, Nadeem A, Bhatti S A, Baig M A 1999 J. Phys. B 32 953 [12] ]Raheel A, Nadeem A, Yaseen M, Aslam M, Bhatti S A, Baig M A 1999 J. Phys. B 32 4361 [13] ]Yi J, Park H, Lee J 1998 J. Kore. Phys. Soci. 5 916 [14] ]Hu S F, Zhang S, Mei S M, Qiu J Z, Chen X 1990 J. Quant. Spectrosc. Radiat. Transfer 1 75 [15] ]Hu S F, Mei S M, Zhang S, Chen X, Xu Y F 1990 Chin. Phys. Lett. 6 64 [16] ]Hu S F, Qiu J Z, Wang G, Liang Y, Chen X 1989 Acta. Phys. Sin. 38 487 (in Chinese) [胡素芬、 邱济真、 张森、 王刚、 梁宜、 陈星 1989 物理学报 38 487] [17] ]Jia L, Jing C Y, Zhou Z Y, Liu F C 1992 J. Opt. Soc. Am. B 10 1317 [18] ]Jayasekharan T, Razvi M A N, Bhale G L 2000 J. Phys. B 33 3123 [19] ]Nakhate S G, Razvi M A N, Connerade J P, Ahmad S A 2000 J. Phys. B 33 5191 [20] ]Pulhani A K, Shah M L, Dev V, Suri B M 2004 J. Opt. Soc. Am. B 22 1117 [21] ]Park H, Kim H, Yi J, Han J, Rhee Y, Lee J 1998 J. Kore. Phys. Soci. 33 288 [22] ]Gononai A I, Plekan O I 2003 J. Phys. B 36 4155 [23] ]Guan F, Dai C J, Zhao H Y 2008 Chin. Phys. B 17 3655 [24] ]Martin W C, Zalubas R, Hagan L 1978 Atomic Energy Levels-The Rare-Earth Elements, NSRDS-NBS60 (U.S. GPO, Washington, D.C.) p162 [25] ]Zhao H Y, Dai C J, Guan F 2009 J. Phys. B 42 065001 [26] ]Zhao H Y, Dai C J, Cuan F 2009 Chin. Phys. B 58 0215 施引文献
Two-photon-resonant three-photon ionization of atomic phosphorus is studied in the 298--306-nm wavelength range. P atoms are produced by Ar+{\mathrm{Ar}}^{+}Ar+ ion sputtering of an InP solid sample and the photoions are detected by a quadrupole mass spectrometer. The laser power dependence of the 3p4{\mathit{p}}^{4}p4S3/20{\mathit{S}}_{3/2}^{0}S3/20​--4 4S3/20^{4}\mathrm{S}_{3/2}^{0}4S3/20​ two-photon excitation and one-photon ionization of 4p4{\mathit{p}}^{4}p4S3/20{\mathit{S}}_{3/2}^{0}S3/20​ phosphorus is determined in the 10--200 MW/cm2{\mathrm{cm}}^{2}cm2 range. The cross section for the ionization step is estimated in the frame of the quantum-defect theory: \ensuremath{\sigma}\ensuremath{\sim}3\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}18}$ cm2{\mathrm{cm}}^{2}cm2. The two-photon Rabi frequency ${\mathrm{\ensuremath{\Omega}}}_{\mathit{R}}$ is deduced from the comparison of our experimental results with the extended two-level model developed by Eberly [Phys. Rev. Lett. 42, 1049 (1979)] to describe (m+n) resonant multiphoton ionization processes and with the rate equation approximation analysis. The best fit gives ${\mathrm{\ensuremath{\Omega}}}_{\mathit{R}}$(${\mathrm{s}}^{\mathrm{\ensuremath{-}}1}$)=8IL{\mathit{I}}_{\mathit{L}}IL​(W/cm2{\mathrm{cm}}^{2}cm2). This value compares relatively well with the theoretical estimate ${\mathrm{\ensuremath{\Omega}}}_{\mathit{R}}$=5.5IL{\mathit{I}}_{\mathit{L}}IL​ obtained by limiting the perturbation-theory summation to the dominant intermediate states. The combination of well-characterized Ar+{\mathrm{Ar}}^{+}Ar+ ion sputtering of a solid sample with resonant photoionization is used to perform actual trace analysis of materials. For example, 0.5 ppm of phosphorus in a silicium sample was measured by this method with a lateral resolution of \ensuremath{\sim}300 \ensuremath{\mu}m.
摘要 本文利用全量子理论,在非旋波近似下对单模相干态光场与级联型三能级原子相互作用过程中场熵随时间的演化进行了精确求解.数值计算的结果表明:随着初始时刻平均光子数n以及光场与原子的耦合强度u, v的增大,场熵的平均值先增大后减小,因此纠缠度也同样先增大后减小;随着失谐量Δ的增大,场熵的平均值逐渐减小,因此纠缠度也逐渐减小. 关键词: 相干态正交化展开 / 非旋波近似 / 场熵 Abstract In this paper,the evolution of field entropy in the system of single-mode coherent light field interacting with a three-level cascade type atom is calculated exactly in the frame of complete quantum theory and without rotating wave approximation.The numerical results indicate that with the increases of the initial mean photon number n and the atom-field coupling strengths u and v the mean value of the field entropy increases at first and then decreases.Therefore,the degrees of entanglement also increase at first and then decrease.The mean value of the entropy of the field decreases with the enlarging of the detuning Δ, which leads to the decrease of the degrees of entanglement. Keywords: coherent-state orthogonalization expansion / without rotating wave approximation / field entropy 作者及机构信息 丛红璐, 任学藻, 姜道来, 廖旭 1. 西南科技大学理学院,绵阳 621010 基金项目: 四川省自然科学基金(批准号: 2006C028)资助的课题. Authors and contacts Cong Hong-Lu, Ren Xue-Zao, Jiang Dao-Lai, Liao Xu 1. 西南科技大学理学院,绵阳 621010 参考文献 [1] [1]Phoenix S J D, Knight P L 1988 Ann. Phys. 186 381 [2] [2] Phoenix S J D, Knight P L 1991 Phys. Rev. A 44 6023 [3] [3]Obada A S F, Ahmed M M A, Faramawy F K, Khalil E M 2004 Chin. J. Phys. 42 80 [4] [4]Faisal A A E, Wahiddin M R B, Obada A S F 2008 Opt. Commun. 281 2854 [5] [5]Liu S M 2003 Chin. J. Quantum. Electron. 20 725 (in Chinese) [刘素梅 2003 量子电子学报 20 725] [6] [6]Zou Y, Li Y P 2009 Chin. Phys. B 18 2794 [7] [7]Zhang J F, Tan L, Liu L W, Ding C Y 2008 Acta Phys. Sin. 57 2205 (in Chinese) [张金芳、谭磊、刘利伟、丁彩英 2008 物理学报 57 2205] [8] [8]Hu X P, Guo H 2009 Acta Phys. Sin. 58 272 (in Chinese) [胡孝平、郭红 2009 物理学报 58 272] [9] [9]Liu T, Feng M,Wang K L 2007 Commun. Theor. Phys. 47 561 [10] ]Zhang Z J, Wang K L,Qin G 2005 Chin. Phys. 14 1317 [11] ]T Liu, K L Wang, M Feng 2007 J. Phys. B:At. Mol. Opt.2 Phys. 40 1967 [12] ]Fan Y X, Liu T, Feng M, Wang K L 2007 Commun. Theor. Phys. 47 781 [13] ]Liu T, Fan Y X, Huang S W, Wang K L, Wang Y 2007 Commun. Theor. Phys. 47 791 [14] ]Ren X Z, Jiang D L, Cong H L, Liao X 2009 Acta Phys. Sin. 58 5394 (in Chinese) [任学藻、姜道来、丛红璐、廖旭 2009 物理学报 58 5394] [15] ]Ren X Z, Liao X, Huang S W, Wang K L 2009 Acta Phys. Sin. 58 2680 (in Chinese) [任学藻、廖旭、黄书文、汪克林 2009 物理学报 58 2680] [16] ]Ren X Z, Liao X, Liu T, Wang K L 2006 Acta Phys. Sin. 55 2865 (in Chinese) [任学藻、廖旭、刘涛、汪克林 2006 物理学报 55 2865] [17] ]Chen Q H,Zhang Y Y, Liu T, Wang K L 2008 Phys. Rev. A 78 1050 施引文献
摘要 提出了一种基于多阶量子隐形传态的量子路由方案, 在量子移动终端之间没有共享纠缠对的情况下, 仍然可以完成量子态的无线传输. 该量子路由方案可以用来构建量子无线广域网, 其传输时延与所经过的链路距离和基站数目无关, 传输一个量子态所需的时间与采用量子隐形传态所需的时间相同. 因此, 从数据传输速率的观点来看, 该方案优于基于纠缠交换的量子路由方案. 关键词: 量子通信 / 多阶量子隐形传态 / 量子路由 / 量子无线广域网 Abstract According to multistage quantum teleportation, we here propose a quantum routing scheme which teleports a quantum state from one quantum device to another wirelessly even though the two devices which do not share entangled photon pairs mutually. By the quantum routing scheme, the model of quantum wireless wide-area networks is presented. In terms of time complexity, the proposed scheme transports a quantum bit in the time almost the same as the quantum teleportation regardless of the number of hops between the source and destination node. From this point of view, the quantum routing scheme is close to optimal scheme in data transmission time. The correlative routing process is proposed under different conditions. The quantum state is transferred by multistage quantum teleportation, therefore, the information transfer between any two nodes in quantum wireless wide-area networks is realized. Keywords: quantum communication / multistage quantum teleportation / quantum routing / quantum wireless wide-area networks 作者及机构信息 刘晓慧1 2, 聂敏1, 裴昌幸2 1. 西安邮电大学通信与信息工程学院, 西安 710061; 2. 西安电子科技大学, 综合业务网理论及关键技术国家重点实验室, 西安 710071 基金项目: 国家自然科学基金(批准号: 61072067, 61172071)、国家重点实验室专项基金(批准号: ISN1001004) 和陕西省教育厅专项科研计划(批准号: 2011JK1017)资助的课题. Authors and contacts Liu Xiao-Hui1 2, Nie Min1, Pei Chang-Xing2 1. School of Communication and Information Engineering, Xi’an University of Post and Telecommunication, Xi’an 710061, China; 2. State Key Laboratory of Integrated Service Networks, Xidian University, Xi’an 710071, China Funds: Project supported by the National Natural Science Foundation of China (Grant Nos. 61072067, 61172071), the State Key Laboratory of Integrated Services Networks, China (Grant No. ISN1001004), and the Scientific Research Project of the Education Department of Shaanxi Province, China (Grant No. 2011JK1017). 参考文献 [1] Li S, Ma H Q, Wu L A, Zhai G J 2013 Acta Phys. Sin. 62 084214 (in Chinese) [李申, 马海强, 吴令安, 翟光杰 2013 物理学报 62 084214] [2] Guo B H, Yang L, Xiang C, Guan C, Wu L A, Liu S H 2013 Acta Phys. Sin. 62 130303 (in Chinese) [郭邦红, 杨理, 向憧, 关翀, 吴令安, 刘颂豪 2013 物理学报 62 130303] [3] Bouwmeester D, Pan J W, Mattle K, Manfred E, Weinfurter H, Zeilinger A 1997 Nature 390 575 [4] Chen P, Deng F G, Long G L 2006 Chin. Phys. 15 2228 [5] Pan J W, Simon C, Brukner C, Zellinger A 2001 Nature 410 1067 [6] Jin X M, Ren J G, Yang B, Yi Z H, Zhou F, Xu X F, Wang S K, Yang D, Hu Y F, Jiang S, Yang T, Yin H, Chen K, Peng C Z, Pan J W 2010 Nature Photon. 4 376 [7] Yin J, Ren J G, Lu H, Cao Y, Yong H L, Wu Y P, Liu C, Liao S K, Zhou F, Jiang Y, Cai X D, Xu P, Pan G S, Jia J J, Huang Y M, Yin H, Wang J Y, Chen Y A, Peng C Z, Pan J W 2012 Nature 488 185 [8] Kwait P G, Waks E, White A G, Appelbaum I, Eberhard P H 1999 Phys. Rev. A 60 R773 [9] Raimond J M, Brune M, Haroche S 2001 Rev. Mod. Phys. 73 565 [10] Sun B, Chapman M S, You L 2004 Phys. Rev. A 69 042316 [11] Artur S, Regina B H, Barry C S, Wolfgang T 2009 Phys. Rev. A 80 062310 [12] Dousse A, Suffczyński J, Beveratos A, Krebs O, Lemaître A, Sagnes I, Bloch J, Voisin P, Senellart P 2010 Nature 466 217 [13] Guo Z, Yan L S, Pan W, Luo B, Xu M F 2011 Acta Phys. Sin. 60 060301 (in Chinese) [郭振, 闫连山, 潘炜, 罗斌, 徐明峰 2011 物理学报 60 060301] [14] Song K H, Zhang W J, Guo G C 2002 Chin. Phys. 11 218 [15] Peng C Z, Yang T, Bao X H, Zhang J, Jin X M, Feng F Y, Yang B, Yang J, Yin J, Zhang Q, Li N, Tian B L, Pan J W 2005 Phys. Rev. Lett. 94 150501 [16] Bourgoin J P, Meyer-Scott E, Higgins B L, Helou B, Erven C, Hbel H, Kumar B, Hudson D, D’Souza I, Girard R, Laflamme R, Jennewein T 2013 New J. Phys. 15 023006 [17] Liu X H, Pei C X, Nie M 2010 Chin. Phys. Lett. 27 120303 [18] Zhu C H, Pei C X, Ma H X, Yu X F 2006 J. Xidian Univ. 33 839 (in Chinese) [朱畅华, 裴昌幸, 马怀新, 于晓飞 2006 西安电子科技大学学报 33 839] [19] Zhou X Q, Wu Y W, Zhao H 2011 Acta Phys. Sin. 60 040304 (in Chinese) [周小清, 邬云文, 赵晗 2011 物理学报 60 040304] [20] Yu X T, Xu J, Zhang Z C 2012 Acta Phys. Sin. 61 220303 (in Chinese) [余旭涛, 徐进, 张在琛 2012 物理学报 61 220303] 施引文献