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Advances in electronics and electron physics

Magnetic Coherence Resonances and Transitions at Zero Frequency

Edmond Geneux, Georges J. Béné, J. Perrenoud

Published Jan 1, 1970• 0 citations
Publisher
DOI
10.1016/s0065-2539(08)60037-2

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It has been shown analytically and numerically that the effect of magnetic coherence (interference) of levels in L- and V-type transitions, induced by the field of a traveling linearly polarized electromagnetic (EM) wave of arbitrary intensity, can make a significant contribution both to the populations of transition levels (more ~50% than of the field contribution) and to the absorption resonance spectra during frequency and magnetic scanning. Differences in the manifestation of the magnetic coherence effect in level populations for open and closed types of transitions have been identified. It has been established that narrow coherent electromagnetically induced transparency (EIT) resonances are formed in the absorption resonance spectra during magnetic scanning near zero magnetic field. The dependencies of EIT resonance parameters on the characteristics of atomic transitions and EM wave intensity have been investigated. The contribution of the magnetic coherence effect of transition levels to the shape of these resonances has been revealed.
The Lamb theory of the optical maser is applied to circularly polarized atomic transitions, and used to consider the beat frequencies and the coherence properties of such orthogonal fields when axial magnetic fields are applied to the gaseous laser. The beat frequency approaches zero in near-zero magnetic fields and synchronization can then occur between the right- and left-handed circularly polarized oscillations. For a resonator with no undue polarization constraint, such a strong coupling gives rise to a linearly polarized output, and to a rotation of the plane of polarization with increasing magnetic field. A self-consistent expression is derived for this rotation under steady-state conditions, and a maximum rotation of $\ifmmode\pm\else\textpm\fi{}\frac{1}{4}\ensuremath{\pi}$ with magnetic field is indicated before the synchronization breaks down and circularly polarized beat phenomena appear. The rotation with magnetic field depends on the laser intensity, on the anisotropy in the cavity losses, and on the position of the cavity resonance within the Doppler linewidth. Also, the angle of rotation is indeterminate unless such anisotropy is present. Other regions of such coherence can occur at higher magnetic fields, where the beat frequency again approaches zero. These depend on the detailed shape of the various dispersion curves of the laser medium. The results derived from the theory used are in general agreement with experimental observations on the 1.153-\ensuremath{\mu} He-Ne laser transition.
A signal related to the spin level crossing in a zero magnetic field—the Hanle effect—has been registered for the first time in the EPR spectrum. It has been shown that, in the general case, the shape of the signal is determined by two qualitatively different mechanisms: (i) the interference of unsteady-state contributions to the dynamics of atomic coherences (electric or magnetic quantum transition moments with certain phases) with close frequencies (“beats at a zero frequency”) and (ii) the summation of resonant signals determined by the steady-state dynamics of the same atomic coherences. The relaxation time of spin coherences has been determined for the EPR transition of Tm 3+ ions in synthetic forsterite.