This program explores fundamental interactions in multi-component Fermi gases. Since single component Fermi gases do not interact at low temperatures as a consequence of the Pauli exclusion principle, it is necessary to trap and cool more than one fermionic species in order to study interactions. In current experiments, 40K and 6Li are considered particularly promising for observation of superfluidity in a Fermi gases, because these atoms exhibit magnetically tunable Feshbach resonances in their scattering interactions. The predicted superfluidity is an atomic gas analog of a superconducting transition. For systems with resonant interactions, transition temperatures of up to half the Fermi temperature are predicted. This would make these atomic systems the highest temperature superconductors ever studied, in units of the Fermi temperature. However, the most interesting mixtures of these Fermi gases must be confined in an all-optical trap, because the states of interest are repelled from magnetic traps.
This program explores fundamental interactions in multi-component Fermi gases. Since single component Fermi gases do not interact at low temperatures as a consequence of the Pauli exclusion principle, it is necessary to trap and cool more than one fermionic species in order to study interactions. In current experiments, 40K and 6Li are considered particularly promising for observation of superfluidity in a Fermi gases, because these atoms exhibit magnetically tunable Feshbach resonances in their scattering interactions. The predicted superfluidity is an atomic gas analog of a superconducting transition. For systems with resonant interactions, transition temperatures of up to half the Fermi temperature are predicted. This would make these atomic systems the highest temperature superconductors ever studied, in units of the Fermi temperature. However, the most interesting mixtures of these Fermi gases must be confined in an all-optical trap, because the states of interest are repelled from magnetic traps.
Optical traps provide tight confinement and very long storage times for atomic gases. Using a single focused beam from a CO2 laser, we confine a mixture of spin-up and spin-down fermionic 6Li atoms, achieving storage times of ten minutes, and evaporative cooling to quantum degeneracy in seconds. A bias magnetic field tunes the gas to a collisional (Feshbach) resonance, producing extremely strong spin-pairing. This system now tests current many-body predictions for high-temperature superconductors, universal interactions in neutron stars, and hydrodynamic flow of quark-gluon plasmas, a state of matter that existed microseconds after the Big Bang.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
The work described in this thesis can be divided into two parts. The first part is concerned with the production of degenerate Fermi gases and Bose-Fermi mixtures. The second part of the thesis describes studies of strongly interacting spin-mixtures of ultracold fermions. We have cooled a magnetically trapped spin-polarized 6Li Fermi gas into quantum degeneracy by sympathetic cooling with bosonic 23Na. In order to do this, we have converted our previously developed apparatus for Bose-Einstein condensation of 23Na into a two-species cooling facility. We have produced 6Li samples with up to 7 × 107 atoms at temperatures below 0.5TF , and up to 3× 107 atoms at temperatures as low as 0.05TF . Further, we have also produced stable quantum degenerate mixtures of 23Na and 6Li, with several million atoms of each species. In a second set of experiments, we have studied strongly interacting spin-mixtures of 6Li. The strength of interactions was resonantly controlled by applying a magnetic field and tuning to “Feshbach resonances”, which occur when the total energy of the colliding particles coincides with the energy of a bound molecular state. These studies are relevant for the continuing quest for a superfluid transition in a Fermi gas. By studying the inelastic decay of the cloud, we have experimentally identified two Feshbach resonances for the inter-state interactions of the two lowest ground states of 6Li. Most importantly, we found that the lifetime of the strongly interacting system is long enough to observe a superfluid transition in the future. The effects of the coherent collisions in 6Li spin-mixtures were studied using radiofrequency (RF) spectroscopy. We demonstrated the absence of mean field “clock shifts” in a two-state mixture of fermions, and have introduced a three-level method to observe the interaction energy shifts. In the strongly interacting regime, near a Feshbach resonance, we have observed universal behavior of the interaction energy, independent of the value of the scattering length. Finally, we have theoretically studied the effects of Pauli blocking during a free expansion of a degenerate Fermi gas. We have concluded that a strongly interacting normal gas will undergo a hydrodynamic expansion even at zero temperature, due to inefficiency of the Pauli suppression of collisions. Therefore, the already observed hydrodynamic expansion cannot be conclusively interpreted as a signature of superfluidity. Thesis Supervisor: Wolfgang Ketterle Title: John D. MacArthur Professor of Physics
An apparatus has been developed to create spin mixtures of ultracold fermionic 6Li in order to investigate the behavior of strongly interacting Fermi gases, and in particular, search for a superconducting phase transition. 6Li atoms are initially confined in a dual species magneto-optical trap (MOT) along with bosonic 7Li. Due to an overlap between spectral features of the two species, a D2/D1 trap/repump scheme is used for the 6Li. The atoms are subsequently cooled to quantum degeneracy in a magnetic trap through optimized dual forced evaporation and transferred to an all optical trap where spin mixtures are created with RF sweeps and pulses. The atomic interactions are controlled through the use of magnetic Feshbach resonances and an externally applied bias magnetic field of up to 1000 G. This thesis details the construction, operation, and performance of the 6Li portion of the apparatus, as well as current results.
Laser cooling and atom trapping techniques have enabled atomic physicists to attain temperatures on the order of 100 nK. In this regime, a trapped gas must be described within the framework of quantum statistical mechanics. In 1995, Bose-Einstein condensation (BEC) was achieved for the first time in such a system by three independent groups. The success of attaining BEC has encouraged research in quantum degenerate Fermi gases (DFG). One of the most exciting opportunities for a DFG is the prospect for Cooper pairing in a two-component gas. The experimental techniques for obtaining degenerate gases, as well as the mechanism for Cooper pairing, hinges on understanding and characterizing ultracold collisional interactions.\nThis thesis is a twofold study in this exciting field. The first section is an in-depth treatment of collisions in atomic lithium. Lithium has two isotopes, 6Li which is a fermion and 7Li which is a boson. This makes it an ideal candidate for studying quantum degenerate gases. In a series of experiments using a magneto-optical trap, we have spectroscopically measured the ground and excited state molecular potentials for both isotopes. From this work we have been able to obtain the most accurate potentials for lithium to date. These precise measurements have enabled us to extract the most accurate value to date for the 2P atomic radiative lifetime of lithium. Furthermore, we have developed a coupled-channel treatment of two-body collisions which has enabled us to calculate the scattering amplitude, elastic cross section, and rate of spin-exchange decay for any ground state collision in lithium as a function of temperature and magnetic field.\nArmed with this knowledge, we have made progress on the design and construction of an electromagnetic trap for lithium. This trap will enable the study of a degenerate Fermi gas of 6Li as well as the possibility of observing a Cooper pairing transition. The trap performance has been characterized for each isotope and current work is focussed on cooling lithium down to degeneracy. Measurements of spin-exchange decay have been made and compare well with the collisional theory that has been developed.
Experimental methods of laser and evaporative cooling, used in the production of atomic Bose-Einstein condensates have recently been extended to realize quantum degeneracy in trapped Fermi gases. Fermi gases are a new rich system to explore the implications of Pauli exclusion on scattering properties of the system, and ultimately fermionic superfluidity. We have produced a new macroscopic quantum system, in which a degenerate Li-6 Fermi gas coexists with a large and stable Na-23 BEC. This was accomplished using inter-species sympathetic cooling of fermionic 6Li in a thermal bath of bosonic Na-23. We have achieved high numbers of both fermions (less than 10(exp 5) and bosons (less than 10(exp 6), and Li-6 quantum degeneracy corresponding to one half of the Fermi temperature. This is the first time that a Fermi sea was produced with a condensate as a "refrigerator".