Laser systems and a linear radiofrequency (rf) Paul trap with an integrated co-axial cavity have been developed for experiments in cavity QED and probabilistic entanglement. Single 40Ca+ ions and large Coulomb crystals have been trapped routinely and laser cooled with long trapping lifetimes. A technique to achieve precise overlap of the pseudopotential minimum of the rf-field with the cavity mode has been implemented through variable capacitors in the resonant rf-circuit used to drive the trap. Three-dimensional micromotion compensation has been implemented. An 894 nm laser has been frequency stabilised to a Pound-Drever-Hall cavity which is in turn stabilised to atomic Cs using polarisation spectroscopy. The Allan variance of the error signal has been reduced to less than a kilohertz on timescales greater than a second. A novel implementation of the scanning cavity transfer lock has been developed to transfer the stability of the 894 nm laser to the 397 nm ion cooling and 866 nm repumping lasers. The bandwidth of the system has been increased to 380 Hz and the Allan variance of the error signal has been reduced to less than ten kilohertz on timescales of greater than a second. The pseudopotential minimum of the rf field has been overlapped optimally with the optical cavity mode through mapping of the fluorescence from cavity-field repumped ions as a function of their displacement. Coupling to the cavity mode has been confirmed by observation of resonant fluorescence into the cavity mode using the cavity-assisted Raman transition process. The thesis demonstrates that the setup is ready for the controlled production of single photons with pre-determined polarisation states, and progression onto new schemes to entangle multiple ions that are coupled to the optical cavity mode.
Laser systems and a linear radiofrequency (rf) Paul trap with an integrated co-axial cavity have been developed for experiments in cavity QED and probabilistic entanglement. Single 40Ca+ ions and large Coulomb crystals have been trapped routinely and laser cooled with long trapping lifetimes. A technique to achieve precise overlap of the pseudopotential minimum of the rf-field with the cavity mode has been implemented through variable capacitors in the resonant rf-circuit used to drive the trap. Three-dimensional micromotion compensation has been implemented. An 894 nm laser has been frequency stabilised to a Pound-Drever-Hall cavity which is in turn stabilised to atomic Cs using polarisation spectroscopy. The Allan variance of the error signal has been reduced to less than a kilohertz on timescales greater than a second. A novel implementation of the scanning cavity transfer lock has been developed to transfer the stability of the 894 nm laser to the 397 nm ion cooling and 866 nm repumping lasers. The bandwidth of the system has been increased to 380 Hz and the Allan variance of the error signal has been reduced to less than ten kilohertz on timescales of greater than a second. The pseudopotential minimum of the rf field has been overlapped optimally with the optical cavity mode through mapping of the fluorescence from cavity-field repumped ions as a function of their displacement. Coupling to the cavity mode has been confirmed by observation of resonant fluorescence into the cavity mode using the cavity-assisted Raman transition process. The thesis demonstrates that the setup is ready for the controlled production of single photons with pre-determined polarisation states, and progression onto new schemes to entangle multiple ions that are coupled to the optical cavity mode.
The combination of an ion trap with a high finesse optical cavity is an ideal system for the investigation of strong coupling cavity quantum electrodynamics, and allows the observation of a number of interesting quantum phenomena. To achieve the small mode volumes required without impairing the ion trapping small traps with a short ion electrode distance are needed. Two microscopic linear rf ion traps have been developed and built to accommodate experimental cavities of lengths of several 100 microns. The first trap design, the 'sandwich' trap, was successfully used to trap 40Ca+ - ions for several hours. It was characterised extensively including a measurement of the heating rates of the ions in the trap. Spectroscopy measurements of the cooling transition, as well as the two repumping transitions were carried out. The second trap design, the 'alumina' trap, also successfully trapped 40Ca+ - ions, and a full characterisation of this trap was made. The experimental cavity was installed at a preliminary cavity length distance of 3.7 mm. The cavity characteristics were examined. Finally the trapped ions were overlapped with the cavity mode by adjusting the trap minimum position along the trap axis via dc voltages and the vertical position of the cavity. To progress further a locking scheme for the cavity length as well as a single - photon detection setup are necessary. To achieve strong coupling a reduction of the cavity length will have to be made.
In this work, I detail the reconstruction and upgrades performed on the axial cavity ion trap in the ITCM group at the university of Sussex, and the measurement of the coupling of multiple ions to the cavity mode. This enables the optimal coupling between the ions and the cavity by adjusting the ions position in the radial and axial positions. This covers new ground in extending the optimal coupling beyond two ions which is of great importance for experiments with several ions in an optical cavity. The thesis outlines the background theory of light-matter interaction and cavity QED, before describing the physical ion trap hardware and its assembly. A description of the laser and cavity systems is provided, including techniques for locking both to stable references. A number of novel measurement techniques for measuring and maximising the stability of the ions and cavities are presented, including micromotion minimisation, spectroscopy, magnetic field compensation using the ground state Hanle effect, and Raman spectroscopy. These techniques enable the measurement of crucial parameters of the atomic transitions and the cavity. The work culminates in a description of the optimisation of the coupling between ion strings and the cavity first by adjusting the radial trap position by means of variable capacitors attached to RF electrodes, and then axially by means of adjusting the endcap potentials and therefore the spacing between ions to obtain the greatest localisation while still positioning the ions close to the antinodes of the cavity field.
We have employed radio-frequency trapping to localize a single 40 Ca + -ion in a high-finesse optical cavity. By means of laser Doppler cooling, the position spread of the ion's wavefunction along the cavity axis was reduced to 42 nm, a fraction of the resonance wavelength of ionized calcium (λ = 397 nm). By controlling the position of the ion in the optical field, continuous and completely deterministic coupling of ion and field was realized. The precise three-dimensional location of the ion in the cavity was measured by observing the fluorescent light emitted upon excitation in the cavity field. The single-ion system is ideally suited to implement cavity quantum electrodynamics under cw conditions. To this end we operate the cavity on the D 3/2 –P 1/2 transition of 40 Ca + (λ = 866 nm). Applications include the controlled generation of single-photon pulses with high efficiency and two-ion quantum gates.
Precise control over internal states of atomic ions in ion traps has been possible for many years enabling high precision spectroscopy of atomic transitions. Trapped ions are suitable candidates for quantum information processing due to their long storage times, low decoherence rates and high readout efficiency. Recent advances in micro-machining fibre optic mirrors and integrated fibre optic-ion trap systems for cavity QED allows one to realise strong coupling between an ion and a cavity mode by reducing the mode volume. For strong ion-cavity coupling, deterministic transfer of quantum states between ions and photons is possible. We have designed and constructed a miniaturised linear Paul trap with an integrated optical cavity, intended for coupling multiple ions to the cavity mode. The RF-electrode separation is 50μm, while the endcap separation is 350μm. The endcap electrodes are narrow tubes of inner diameter 300μm allowing optical fibers through the tubes to form the cavity. The trap depth we calculate to be 650meV for a 10V applied potential at 20MHz. The 4P1⁄2→ 3D3⁄2 transition of the atomic ion 40Ca+ with Γ = 24π × 22MHz can be coupled to an optical fibre Fabry-Perot cavity with length of 380µm, finesse of 33,000 and cavity linewidth k = 2π ×11MHz.The ion-cavity coherent coupling g = 2π × 19:5MHz of this system will put it in single-ion strong coupling regime with cooperativity, C=1.5.
This thesis describes experimental work towards developing a trapped ion quantum information processor. An existing ion trap apparatus was capable of trapping and laser-cooling single ions or small ion strings of 40 Ca+, and had been used for studies of quantum jumps and natural lifetime measurements in Ca. This thesis describes improvements in this apparatus, which have allowed the stability and the flexibility of experimental control of the ions to be greatly increased. This enabled experiments to read out the spin state of a single trapped ion, and to load ions with isotope selectivity through photoionization. The optical systems were improved by installation of new lasers, optical reference cavities, and a system of acousto-optic modulators for laser intensity switching and frequency control. The photon counting for fluorescence detection was improved, and a new photon time-of-arrival correlation circuit developed. This has permitted rapid and more sensitive detection of micromotion, and hence cancellation of stray fields in the trap. A study of resonant circuits in the low RF, high voltage (10 MHz, 1 kV) regime was carried out with a view to developing a new RF supply for the Paul trap with reduced noise and increased power. A new supply based on a helical resonator was built and used to trap ions. This technique has reduced noise and will permit higher secular frequencies to be attained in the future. A magnetic field B in the ion trap is used to define a quantization axis, and in one series of experiments was required to be of order 100 G to provide a substantial Zeeman splitting. A set of magnetic field coils to control the size and direction of B is described. The design of these posed some problems owing to an unforseen issue with the vacuum chamber. In short, it is magnetizable and acts to first approximation like a magnetic shield. The field coils had to be sufficiently substantial to produce the desired field at the ion even in the presence of this shielding effect, and dark resonance (and other) spectra with Zeeman splitting were obtained to calibrate the field using the ion as a probe. Finally, the thesis describes the successful loading of the ion trap by laser photoionization from a weak atomic beam. This involved two new lasers at 423 nm and 389 nm. Saturated absorption spectroscopy of neutral calcium is first described, then transverse excitation of an atomic beam in our vacuum chamber is used to identify all the main isotopes of calcium and confirm their abundances in our source (a heated sample of natural calcium). Finally, photoionization is used to load the trap. This has three advantages over electron-impact ionization. By avoiding an electron gun, we avoid charging of insulating patches and subsequent electric field drift as they discharge; the flux in the atomic beam and hence calcium (and other) deposits on the electrodes can be greatly reduced; and most importantly, the photoionization is isotope selective. Evidence is presented which suggests that even with an non-enriched source, the rare isotope 43 Ca can be loaded with reasonable efficiency. This isotope is advantageous for quantum information experiments for several reasons, but chiefly because its ground state hyperfine structure can act as a stable qubit.
Trapped cold ions are tools which we used to approach two very disparate areas of physics, strong coupling between Ba+ ions and optical resonators, and investigations of a low-energy nuclear isomer of 229-Th. The first part of this thesis describes our progress towards the integration of a miniature Paul (rf) ion trap with a high finesse (F=30000) optical cavity. Ba+ ions were trapped and cooled for long periods and a new scheme for isotope selective photoionization was developed. The second part of this thesis describes our progress towards controlled excitation of the low energy nuclear isomer of 229-Th, which may provide a bridge between the techniques of cold atomic and nuclear physics. As a step towards this goal, 232-Th3+ ions were confined in rf ions traps and cooled via collisions with a buffer gas of helium. A sophisticated scanning program was developed for controlling ion trap loading, tuning lasers, and running a CCD camera to look for fluorescence. The low-lying electronic transitions of Th3+ at 984 nm, 690 nm and 1087 nm were observed via laser fluorescence.