Nanoscale control over the second-order photon correlation function ${g}^{(2)}(\ensuremath{\tau})$ is critical to emerging research in nonlinear nanophotonics and integrated quantum information science. Here we report on quasiparticle control of photon bunching with
g(2)(0)>45 in the cathodoluminescence of nanodiamond nitrogen vacancy (
NV0) centers excited by a converged electron beam in an aberration-corrected scanning transmission electron microscope. Plasmon-mediated
NV0 cathodoluminescence exhibits a 16-fold increase in luminescence intensity correlated with a threefold reduction in photon bunching compared with that of uncoupled
NV0 centers. This effect is ascribed to the excitation of single temporally uncorrelated
NV0 centers by single surface plasmon polaritons. Spectrally resolved Hanbury Brown--Twiss interferometry is employed to demonstrate that the bunching is mediated by the
NV0 phonon sidebands, while no observable bunching is detected at the zero-phonon line. The data are consistent with fast phonon-mediated recombination dynamics, a conclusion substantiated by agreement between Bayesian regression and Monte Carlo models of superthermal
NV0 luminescence.
Abstract For the first time, the Autler Townes‐splitting dependency on parity‐time symmetry breaking is investigated. The first‐, second‐, and third‐order splitting in spectral domain outputs obtained through different phase transitions of Eu 3+ : BiPO 4 are explored. First‐order splitting corresponds to pure crystal field splitting attributed to the shifting of energy levels and the inherent effect of the crystal field. Second/third‐order splitting results from the coexistence of crystal field and non‐Hermitian spectral Autler Townes (SAT)‐splitting caused by single‐photon dressing coupled with the interaction of phonon and double photon–phonon dressing. It is further explored the relationship between spectral and temporal‐domain splitting obtained through the different phases of Eu 3+ : BiPO 4 by changing the laser detuning. It is authenticated that the contributions of crystal field, photon, and phonon dressing interactions can only be individually distinguished in the spectral domain. Moreover, the experiment results suggest the analogy of an optical 4 × 1 multiplexer with a channel spacing contrast of ≈91% and an optical router with a channel equalization ratio of ≈93%.