This thesis is a collection of three separate projects ordered according to the historical development of atomic physics, covering first spectroscopy, then laser cooling, and finally the exploration of quantum dynamics of many-particle states of ultra-cold atoms in optical lattices. We begin with a description of the theory of atomic line shapes with unresolvable hyperfine structure. We apply this theory to experimentally measured spectra of the Lithium D lines and report improved determination of the absolute transition frequencies and an improved bound of the difference in 6Li-7Li nuclear charge radius. We then discuss multi-photon processes in laser cooling and report experimental implementation of multi-photon laser cooling and magneto optical trapping using short lived excited to excited transitions in 133Cs. We present a theoretical proposal to laser cool (Anti-) Hydrogen using a Doppler selective 1S-2S excitation and the Sisyphus effect on the 2S-3P transition. Finally, we detail the construction and operation of an ultracold 87Rb apparatus with a double well optical lattice. We use this lattice to prepare excited many-body states with N´eel antiferromagnetic order and to study the resulting non-equilibrium magnetization dynamics. We observe regimes where the dynamics is dominated by superexchange mediated magnetic interactions.
This thesis is a collection of three separate projects ordered according to the historical development of atomic physics, covering first spectroscopy, then laser cooling, and finally the exploration of quantum dynamics of many-particle states of ultra-cold atoms in optical lattices. We begin with a description of the theory of atomic line shapes with unresolvable hyperfine structure. We apply this theory to experimentally measured spectra of the Lithium D lines and report improved determination of the absolute transition frequencies and an improved bound of the difference in 6Li-7Li nuclear charge radius. We then discuss multi-photon processes in laser cooling and report experimental implementation of multi-photon laser cooling and magneto optical trapping using short lived excited to excited transitions in 133Cs. We present a theoretical proposal to laser cool (Anti-) Hydrogen using a Doppler selective 1S-2S excitation and the Sisyphus effect on the 2S-3P transition. Finally, we detail the construction and operation of an ultracold 87Rb apparatus with a double well optical lattice. We use this lattice to prepare excited many-body states with N´eel antiferromagnetic order and to study the resulting non-equilibrium magnetization dynamics. We observe regimes where the dynamics is dominated by superexchange mediated magnetic interactions.
The work described in this thesis is related to various projects that I worked on towards the production of ultra-cold ensembles of ⁸⁵Rb, ⁸⁷Rb and fermionic ⁶Li. In the past few years, ultra-cold atomic gases have evolved into a mature field of research, driving various theoretical and experimental groups towards new possibilities. This thesis starts with an overview of the research direction of the field and the lab in particular, to use ultra-cold fermionic atoms as quantum simulators for several condensed matter problems. It discusses the experimental route to quantum degeneracy in a sample of ultra-cold atoms and techniques to get there. The rest of the thesis primarily discusses the first step to degeneracy- production of ultra-cold ensembles of rubidium and lithium. It starts with the theoretical concepts that enable laser cooling and trapping. The interaction between light and atoms and how it leads to a decrease in temperature of the ensemble is discussed. The limits of different cooling mechanism with relevance of the atoms of interest are described. The starting point for all laser cooling experiments is an atomic source, the details of the requirements and efficiency of different atomic sources is discussed, emphasizing our choice of sources for the two atoms. Other technical details such as the vacuum system and the control system for the experiment are briefly discussed. Preliminary data from our first ensembles of ultra-cold lithium and rubidium is shown. At the end, the planning and progress of the first experiments that we aim to achieve with these ultra-cold atoms namely looking for Feshbach resonances and studying the effect of DC electric fields on them, and studies with ultra-cold lithium atoms in optical lattices, is discussed.
This thesis gives an account of work done on semi-classical and quantum Monte Carlo simulations in far-detuned optical lattices. Firstly, the basic principles of laser cooling of atoms are presented including a short introduction to optical lattices in the near and far-detuned regime. A detailed analysis is made of the band-structure of optical lattices, using the Bloch formalism, and of the bound-state population distribution appropriate for a thermal sample of trapped atoms. Secondly, a general overview is given of the quantum Monte Carlo method for simulating the dynamics of atom-light interactions. This is followed by a detailed study of the concept of Raman cooling, which is a useful tool to prepare atoms in the ground motional state of the lattice and an important first step to achieving quantum state control with ultra-cold atoms. A simplified model of Raman cooling is introduced and simulated using the quantum Monte Carlo wave-function approach. Then the implementation of simulations of resolved-sideband Raman cooling based on this model is discussed as is how the results were used to optimize the experimental work done by our group. The results of these simulations show for the first time that the quantum Zeno effect has a crucial impact on the efficiency of Raman cooling experiments. Also the experimental measurements of the temperature of Raman sideband cooled atoms for a range of parameters are compared with theoretical results and shows a good qualitative agreement. Thirdly, the results of semi-classical numerical simulations of parametric excitation in optical lattices are presented. It is shown that the modulation of the potential can result in selective parametric excitation of trapped atoms. The theoretical results show good qualitative agreement with experiment. The thesis is concluded with a description of possible avenues for future studies on quantum state control in optical lattices.
This thesis includes both experimental and theoretical investigations, presented in a series of eight papers. The experimental part ranges from the construction procedures of an apparatus for Bose-Einstein condensates, to full scale experiments using three different set-ups for ultracold atoms in optical lattices. As one of the main themes of the thesis, an experimental apparatus for production of Bose-Einstein Condensates is under construction. A magneto-optically trapped sample, hosting more than 200 million 87Rb atoms, have successfully been loaded into a magnetic trap with high transfer rate. The lifetime of the sample in the magnetic trap is in the range of 9 s, and the atoms have been shown to respond to evaporative cooling. The experiment is ready for optimization of the magnetic trap loading, and evaporative cooling parameters, which are the final steps for reaching Bose-Einstein condensation. The set-up is designed to host experiments including variable geometry optical lattices, and includes the possibility to align laser beams with high angular precision for this purpose. The breakdown of Bloch waves in a Bose-Einstein condensate is studied, attributed to the effect of energetic and dynamical instability. This experimental study is performed using a Bose-Einstein condensate in a moving one-dimensional optical lattice at LENS, Florence Italy. The optical lattice parameters, and the thermal distribution of the atomic sample required to trigger the instabilities, are detected, and compared with a theoretical model developed in parallel with the experiments. In close connection with these one-dimensional lattice studies, an experimental survey to characterize regimes of superradiant Rayleigh scattering and Bragg scattering is presented. Tunneling properties of repulsively bound atom pairs in double well potentials are characterized in an experiment at Johannes Gutenberg University, Mainz Germany. A three-dimensional optical lattice, producing an array of double wells with tunable properties is let to interact with a Bose-Einstein condensate. Pairs of ultracold atoms are produced on one side in the double wells, and their tunneling behavior, dependent on potential barrier and repulsion properties, is studied. A theoretical study of the crossover between one- and two-dimensional systems has been performed. The simulations were made for a two-dimensional array of atoms, where the behavior for different tunneling probabilities and atom-atom repulsion strengths was studied. Scaling relations for systems of variable sizes have been examined in detail, and numerical values for the involved variables have been found.
This thesis describes experiments focused on investigating out-of-equilibrium phenomena in the Bose-Hubbard Model and exploring novel cooling techniques for ultracold gases in optical lattices. In the first experiment, we study quenches across the Mott-insulator-to-superfluid quantum phase transition in the 3D Bose-Hubbard Model. The quench is accomplished by continuously tuning the ratio of the Hubbard energies. We observe that the degree of excitation is proportional to the fraction of atoms that cross the phase boundary, and that the amount of excitations and energy produced during the quench have a power-law dependence on the quench rate. These phenomena suggest an excitation process analogous to the mechanism for defect generation in non-equilibrium classical phase transitions. This experiment constitutes the first observation of the Kibble-Zurek mechanism in a quantum quench. We have reported our findings in Ref. [1]. In a second experiment, published in Ref. [2], we investigate dissipation as a method for cooling a strongly interacting gas. We introduce dissipation via a bosonic reservoir to a strongly interacting bosonic gas in the Mott-insulator regime of a 3D spin-dependent optical lattice. The lattice atoms are excited to a higher energy band using laser-induced Bragg transitions. A weakly interacting superfluid comprised of atoms in a state that does not experience the lattice potential acts as a dissipative bath that interacts with the lattice atoms through collisions. We measure the resulting bath-induced decay using the atomic quasimomentum distribution, and we compare the decay rate with predictions from a weakly interacting model with no free parameters. A competing intrinsic decay mechanism arising from collisions between lattice atoms is also investigated. The presence of intrinsic decay can not be accommodated within a non-interacting framework and signals that strong interactions may play a central role in the lattice-atom dynamics. The intrinsic decay process we observe may negatively impact the success of cooling via dissipation because a fraction of intrinsic decay events can deposit a large amount of energy into the lattice gas. In a third experiment, we develop and carry out the first demonstration of cooling an atomic quasimomentum distribution. Our scheme, applied in a proof-of-principle experiment to 3D Bose-Hubbard gas in the superfluid regime, involves quasimomentum-selective Raman transitions. This experiment is motivated by the search of new cooling techniques for lattice-trapped gases. Efficient cooling exceeding heating rates is achieved by iteratively removing high quasimomentum atoms from the lattice. Quasimomentum equilibration, which is necessary for cooling, is investigated by directly measuring rethermalization rates after bringing the quasimomentum distribution of the gas out of equilibrium. The measured relaxation rate is consistent at high lattice depths with a short-range, two-particle scattering model without free parameters, despite an apparent violation of the Mott-Ioffe-Regel bound. Our results may have implications for models of unusual transport phenomena in materials with strong interactions, such as heavy fermion materials and transition metal oxides. The cooling method we have developed is applicable to any species, including fermionic atoms. Our results are available in Ref. [3]
A complete laser cooling setup was built, with focus on threedimensional near-resonant optical lattices for cesium. These consist of regularly ordered micropotentials, created by the interference of four laser beams. One key feature of optical lattices is an inherent ”Sisyphus cooling” process. It efficiently extracts kinetic energy from the atoms, leading to equilibrium temperatures of a few µK. The corresponding kinetic energy is lower than the depth of the potential wells, so that atoms can be trapped. We performed detailed studies of the cooling processes in optical lattices by using the time-of-flight and absorption-imaging techniques. We investigated the dependence of the equilibrium temperature on the optical lattice parameters, such as detuning, optical potential and lattice geometry. The presence of neighbouring transitions in the cesium hyperfine level structure was used to break symmetries in order to identify, which role “red” and “blue” transitions play in the cooling. We also examined the limits for the cooling process in optical lattices, and the possible difference in steady-state velocity distributions for different directions. Moreover, in collaboration with ´Ecole Normale Sup´erieure in Paris, numerical simulations were performed in order to get more insight in the cooling dynamics of optical lattices. Optical lattices can keep atoms almost perfectly isolated from the environment and have therefore been suggested as a platform for a host of possible experiments aimed at coherent quantum manipulations, such as spin-squeezing and the implementation of quantum logic-gates. We developed a novel way to trap two different cesium ground states in two distinct, interpenetrating optical lattices, and to change the distance between sites of one lattice relative to sites of the other lattice. This is a first step towards the implementation of quantum simulation schemes in optical lattices.
In this thesis, detailed experimental studies and numerical simulations are presented of laser cooling mechanisms in dissipative optical lattices and results of the first realized three dimensional Brownian motor in optical lattices. A dissipative optical lattice is a periodic light shift potential, created in the interference patterns of laser beams. In this, atoms can be both cooled and trapped, and the most important relaxation mechanism is generally considered to be “Sisyphus cooling”. However, careful experimental and theoretical investigations indicate the presence of other cooling processes as well. This is studied by varying different parameters such as irradiance and frequency of the lattice light. The time evolution of atoms in optical lattices show strong evidence of a bimodal velocity distribution, where a population transfer between one mode containing “hot” atoms and one mode containing “cold” atoms is evident. The normal diffusion of atoms in optical lattices is characterized by isotrop random fluctuations and exhibit the nature of Brownian motion. We have realized a technique where this motion is rectified and controlled. This is done in a three dimensional double optical lattice. This Brownian motor has control properties for both its speed and its direction in three dimensions. Our three dimensional double optical lattice is created by using laser light, exploiting two transitions, in the D2 line of cesium. Two three dimensional optical lattices are spatially overlapped; each optical lattice traps atoms in one of two hyperfine ground states. The controllability comes about by inducing phase shifts in the lattice laser beams, which displace the lattices relative to each other. This type of highly controlled Brownian motor is of fundamental interest since Brownian motion is present in almost all systems and for the role they play in protein motors and the function of living cells, and for the potential applications in nanotechnology. Brownian motors of this kind also open the way to possible studies of quantum Brownian motors and quantum resonances that are predicted for atomic ratchets. Optical lattices, and especially double optical lattices, have also been suggested as a platform for quantum state manipulations due to the good isolation from environment and ambient effects. Most of the work in this thesis is a first step towards the implementation of quantum manipulation schemes in a double optical lattice.