This thesis gives an account of work done on semi-classical and quantum Monte Carlo simulations in far-detuned optical lattices. Firstly, the basic principles of laser cooling of atoms are presented including a short introduction to optical lattices in the near and far-detuned regime. A detailed analysis is made of the band-structure of optical lattices, using the Bloch formalism, and of the bound-state population distribution appropriate for a thermal sample of trapped atoms. Secondly, a general overview is given of the quantum Monte Carlo method for simulating the dynamics of atom-light interactions. This is followed by a detailed study of the concept of Raman cooling, which is a useful tool to prepare atoms in the ground motional state of the lattice and an important first step to achieving quantum state control with ultra-cold atoms. A simplified model of Raman cooling is introduced and simulated using the quantum Monte Carlo wave-function approach. Then the implementation of simulations of resolved-sideband Raman cooling based on this model is discussed as is how the results were used to optimize the experimental work done by our group. The results of these simulations show for the first time that the quantum Zeno effect has a crucial impact on the efficiency of Raman cooling experiments. Also the experimental measurements of the temperature of Raman sideband cooled atoms for a range of parameters are compared with theoretical results and shows a good qualitative agreement. Thirdly, the results of semi-classical numerical simulations of parametric excitation in optical lattices are presented. It is shown that the modulation of the potential can result in selective parametric excitation of trapped atoms. The theoretical results show good qualitative agreement with experiment. The thesis is concluded with a description of possible avenues for future studies on quantum state control in optical lattices.
This thesis gives an account of work done on semi-classical and quantum Monte Carlo simulations in far-detuned optical lattices. Firstly, the basic principles of laser cooling of atoms are presented including a short introduction to optical lattices in the near and far-detuned regime. A detailed analysis is made of the band-structure of optical lattices, using the Bloch formalism, and of the bound-state population distribution appropriate for a thermal sample of trapped atoms. Secondly, a general overview is given of the quantum Monte Carlo method for simulating the dynamics of atom-light interactions. This is followed by a detailed study of the concept of Raman cooling, which is a useful tool to prepare atoms in the ground motional state of the lattice and an important first step to achieving quantum state control with ultra-cold atoms. A simplified model of Raman cooling is introduced and simulated using the quantum Monte Carlo wave-function approach. Then the implementation of simulations of resolved-sideband Raman cooling based on this model is discussed as is how the results were used to optimize the experimental work done by our group. The results of these simulations show for the first time that the quantum Zeno effect has a crucial impact on the efficiency of Raman cooling experiments. Also the experimental measurements of the temperature of Raman sideband cooled atoms for a range of parameters are compared with theoretical results and shows a good qualitative agreement. Thirdly, the results of semi-classical numerical simulations of parametric excitation in optical lattices are presented. It is shown that the modulation of the potential can result in selective parametric excitation of trapped atoms. The theoretical results show good qualitative agreement with experiment. The thesis is concluded with a description of possible avenues for future studies on quantum state control in optical lattices.
Optical lattices induced by light detuned far from the frequency of any atomic resonance transition are ideal systems in which to develop techniques for the coherent control of atomic motional and internal states. Decoherence arising from spontaneous emission can be eliminated to an arbitrary degree by varying the detuning of the optical field. The atoms trapped in these lattices are to a large extent isolated from environmental disturbances and from each other. The first step towards the coherent control of atoms in a far-detuned lattice is their preparation in a single motional state. In this thesis the preparation of atoms in the ground vibrational state of a two-dimensional far-detuned optical lattice via resolved-sideband Raman cooling is presented. This sideband-cooling scheme involves stimulated Raman transitions between bound vibrational states of a pair of magnetic ground state sublevels, followed by an irreversible step due to optical pumping, resulting in a net loss of one quantum of vibrational energy per cooling cycle. This process provides efficient cooling in two-dimensions and leads to the accumulation of a large fraction of atoms in the 2-D ground vibrational state of a potential well associated with a single Zeeman substate. Experiments aimed at improving and monitoring the characteristics of the lar-detuned lattice and the sideband-Raman cooling efficiency are also described. Parametric excitation experiments and modelling are employed to investigate the degree of anharmonicity of the optical potential and the importance of heating induced by laser intensity noise, whilst Zeeman-state analysis of the sample is performed for monitoring the distribution of atoms over different magnetic sub- states. Finally, spin-polarization experiments are carried out in order to study the paramagnetic properties of the lattice and lead to an evaluation of a spin-temperature for the sample.
This dissertation reports on quantum state preparation of cesium atoms in a two-dimensional optical lattice, by resolved-sideband Raman cooling. An optical lattice is a periodic potential produced by the light shift interaction between an atom and light field. Laser cooled atoms can become strongly localized about the bottom of potential wells in an optical lattice, where they occupy a discrete spectrum of bound vibrational energy levels. The distribution over vibrational levels of atoms in the lattice is characterized by the mean vibrational excitation, n . In an optical lattice, absorption and emission of photons from lattice beams causes n to increase in time. This source of heating is always present, but its rate can be greatly reduced in a lattice detuned far from the atomic resonance. Sideband cooling is an efficient means of transferring atoms from higher into lower-lying vibrational levels and, thus, it reduces n for the ensemble. If the sideband cooling rate is much greater than the heating rate, then n approaches zero and virtually all atoms are in the lowest vibrational level in their potential wells. Our sideband cooling scheme involves stimulated Raman transitions between bound states in the potential wells of a pair of magnetic sublevels, followed by optical pumping, for a net loss of one quantum of vibration per cooling cycle. The process accumulates 98% of atoms in the ground vibrational level of a potential well associated with a single Zeeman substate. Each atom in the lattice is then very close to a pure state. For two-dimensional lattice with sideband cooling we find nx≈ny≈0.008 &parl0;16&parr0; . Various issues related to state preparation and sideband cooling are also discussed in the context of a one dimensional lin ⊥ lin optical lattice. These include improvement of laser cooling in a near resonance lattice by application of weak magnetic fields, transfer of atoms from near into far off-resonance lattices, and heating rates in far off-resonance lattices.
In this thesis, detailed experimental studies and numerical simulations are presented of laser cooling mechanisms in dissipative optical lattices and results of the first realized three dimensional Brownian motor in optical lattices. A dissipative optical lattice is a periodic light shift potential, created in the interference patterns of laser beams. In this, atoms can be both cooled and trapped, and the most important relaxation mechanism is generally considered to be “Sisyphus cooling”. However, careful experimental and theoretical investigations indicate the presence of other cooling processes as well. This is studied by varying different parameters such as irradiance and frequency of the lattice light. The time evolution of atoms in optical lattices show strong evidence of a bimodal velocity distribution, where a population transfer between one mode containing “hot” atoms and one mode containing “cold” atoms is evident. The normal diffusion of atoms in optical lattices is characterized by isotrop random fluctuations and exhibit the nature of Brownian motion. We have realized a technique where this motion is rectified and controlled. This is done in a three dimensional double optical lattice. This Brownian motor has control properties for both its speed and its direction in three dimensions. Our three dimensional double optical lattice is created by using laser light, exploiting two transitions, in the D2 line of cesium. Two three dimensional optical lattices are spatially overlapped; each optical lattice traps atoms in one of two hyperfine ground states. The controllability comes about by inducing phase shifts in the lattice laser beams, which displace the lattices relative to each other. This type of highly controlled Brownian motor is of fundamental interest since Brownian motion is present in almost all systems and for the role they play in protein motors and the function of living cells, and for the potential applications in nanotechnology. Brownian motors of this kind also open the way to possible studies of quantum Brownian motors and quantum resonances that are predicted for atomic ratchets. Optical lattices, and especially double optical lattices, have also been suggested as a platform for quantum state manipulations due to the good isolation from environment and ambient effects. Most of the work in this thesis is a first step towards the implementation of quantum manipulation schemes in a double optical lattice.
In this thesis, I study the properties of cold neutral atoms, including Bose-Einstein condensates (BEC), inside periodic light-shift potentials created by optical lattices. In the first part, a new optical-lattice scheme, employing Raman transitions, hereafter referred to as a Raman Optical Lattice (ROL), is investigated. This optical lattice possesses a novel sub-Doppler cooling mechanism and a reduced periodicity. Both theoretical and experimental results con¯rm these two characteristics of the ROL. In the second half of the thesis, instead of thermal atoms, optical lattices are loaded with condensate atoms. Our BEC apparatus and the procedure towards forming a BEC are described in detail. After the achievement of the BEC, a 1D far-detuned optical lattice is applied to the BEC. A number of phenomena are observed, including Kapitza-Dirac diffraction, thermal atom interference, atom interferometry, Bloch oscillations, and a superfluid to Mott-insulator transition. Finally a brief discussion about future work is given.
The purpose of our master thesis is to present an original synthesis of various works dealing with the Monte-Carlo wavefunction (MCWF) method in quantum optics and its applications to laser cooling of atoms with a particular focus on Doppler and Sisyphus cooling mechanisms. We introduce the MCWF method which is used to solve master equations describing the dynamics of open quantum systems in quantum optics. This method turns out to be much more efficient than a method based on the full integration of the density matrix. We perform laser cooling simulations in 1D both with a classical and a quantum treatment of the atomic centre-of-mass motion and investigate Doppler and Sisyphus cooling. Our numerical results turn out to be in very good agreement with those predicted by semiclassical theories, except for large detuning and/or low intensity laser where semiclassical theories fail. For such cases, our method provides a good alternative and predicts temperatures much larger than the recoil temperature. Finally, we also consider a classical treatment of the centre-of-mass motion and we compare the subsequent results with those obtained with a full quantum approach.
This thesis is a collection of three separate projects ordered according to the historical development of atomic physics, covering first spectroscopy, then laser cooling, and finally the exploration of quantum dynamics of many-particle states of ultra-cold atoms in optical lattices. We begin with a description of the theory of atomic line shapes with unresolvable hyperfine structure. We apply this theory to experimentally measured spectra of the Lithium D lines and report improved determination of the absolute transition frequencies and an improved bound of the difference in 6Li-7Li nuclear charge radius. We then discuss multi-photon processes in laser cooling and report experimental implementation of multi-photon laser cooling and magneto optical trapping using short lived excited to excited transitions in 133Cs. We present a theoretical proposal to laser cool (Anti-) Hydrogen using a Doppler selective 1S-2S excitation and the Sisyphus effect on the 2S-3P transition. Finally, we detail the construction and operation of an ultracold 87Rb apparatus with a double well optical lattice. We use this lattice to prepare excited many-body states with N´eel antiferromagnetic order and to study the resulting non-equilibrium magnetization dynamics. We observe regimes where the dynamics is dominated by superexchange mediated magnetic interactions.