The quantum state of a traveling light pulse can qualitatively change the excitation dynamics of a two-level atom. We investigate this dependence for coherent and Fock input states using a virtual-cavity formulation with matched input and output temporal profiles. Analytical treatment of the master equation and numerical simulations show that coherent pulses produce damped Rabi oscillations, whereas Fock pulses can exhibit a partial recovery of the oscillation amplitude in the trailing part of the pulse. We examine how coupling to an auxiliary temporal mode and radiative loss shape this recovery. We also establish a connection with stimulated Raman adiabatic passage through an exact many-photon dark state and derive the associated adiabaticity condition. The observed recovery occurs away from ideal dark-state following. These results distinguish transient recovery in traveling-pulse scattering from conventional cavity collapse and revival, and clarify the scope of an adiabatic-transfer interpretation.
The quantum state of a traveling light pulse can qualitatively change the excitation dynamics of a two-level atom. We investigate this dependence for coherent and Fock input states using a virtual-cavity formulation with matched input and output temporal profiles. Analytical treatment of the master equation and numerical simulations show that coherent pulses produce damped Rabi oscillations, whereas Fock pulses can exhibit a partial recovery of the oscillation amplitude in the trailing part of the pulse. We examine how coupling to an auxiliary temporal mode and radiative loss shape this recovery. We also establish a connection with stimulated Raman adiabatic passage through an exact many-photon dark state and derive the associated adiabaticity condition. The observed recovery occurs away from ideal dark-state following. These results distinguish transient recovery in traveling-pulse scattering from conventional cavity collapse and revival, and clarify the scope of an adiabatic-transfer interpretation.
The interaction of a traveling pulse of quantum light with a localized quantum system shows non-Markovian features when scattering takes place in a structured environment. Here, we devise a non-Markovian input-output theory by coherently coupling the scatterer to a pseudomode, which decays into a Markovian reservoir. This incorporates memory effects of a structured environment without altering the cascaded nature of the Lindblad master equation, whose solution provides the quantum state of the output field of any desired mode. We apply our theory to the stimulated emission by a two-level atom, and to transmission of a Gaussian pulse through a cavity. We observe that the non-Markovian revival of coherence in the scatterer distorts the single-mode nature of the incoming pulse, thus resulting in a multimode output field.
We present a formalism that accounts for the interaction of a local quantum system, such as an atom or a cavity, with traveling pulses of quantized radiation. We assume Markovian coupling of the stationary system to the input and output fields and nondispersive asymptotic propagation of the pulses before and after the interaction. This permits derivation of a master equation where the input and output pulses are treated as single oscillator modes that both couple to the local system in a cascaded manner. As examples of our theory, we analyze reflection by an empty cavity with phase noise, stimulated atomic emission by a quantum light pulse, and formation of a Schrödinger-cat state by the dispersive interaction of a coherent pulse and a single atom in a cavity.
Abstract The future of quantum information processing hinges on chip-scale nanophotonics, specifically cavity QED and waveguide QED. One of the foremost processes underpinning quantum photonic technologies is the phenomenon of Rabi oscillations, which manifests when a qubit is irradiated by an intense laser source. Departing from the conventional semiclassical framework, we explore the more general, quantum theoretical case where the optical excitation takes the form of a multiphoton Fock state, and the qubit couples to a continuum of radiation modes. By employing the real-space formalism, we analytically explore the scattering dynamics of the photonic Fock state as it interfaces with a two-level emitter. The resulting amplitude for atomic excitation features a linear superposition of various independent scattering events that are triggered by the potential of sequential, time-delayed photon absorptions and emissions. The lowest-order excitation event, initiated by the stochastic scattering of one of the several photons, appropriately characterizes the dynamics in a weak-field environment. This event is complemented by a multitude of higher-order scattering events ensuing from repeated atom–photon interactions. The temporal evolution of the qubit excitation in our configuration closely mirrors the semiclassical predictions, particularly in the strong-pumping limit where Rabi oscillations unfold. Notably, this compatibility with the semiclassical paradigm transcends beyond the strong-excitation regime and applies both to the weak-driving and large-detuning limits. In a nutshell, our analysis extends the existing results on quantum Rabi oscillations pertinent to single-mode cavity QED, to the multimode, waveguide-QED configurations wherein flying photons are the information carriers. Additionally, we delve into the dynamics of pulsed wave packets, shedding light on the potential to substantially enhance excitation efficiency, even in scenarios involving just a few photons. Beyond their theoretical merit, these findings should hold practical relevance for future Fock-state-based quantum computing and emerging waveguide-integrated photonic technologies such as those involving superconducting circuitry.
We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the pulse's spatial and temporal profiles on the atomic excitation. In particular, we find the ideal shape for a pulse to put exactly one excitation in any desired state of the bi-atomic system. Furthermore, we analyze the differences in the atomic dynamics between the cases of Fock state pulses and coherent state pulses.
We present a detailed quantum theory and simulations of few-photon Fock state pulses interacting with a two-level system (TLS) in an open waveguide-QED system. For a rectangular pulse shape, we present an exact temporal scattering theory to derive analytical expressions for the TLS population, using one-photon and two-photon pulses, for both chiral and symmetric emitters. We also derive the stationary (long-time) and time-dependent spectra for one-photon excitation, and show how these differ at a fundamental level when considering TLS population effects. Numerically, we also present matrix product state (MPS) simulations, which allow us to compute more general photon correlation functions for arbitrary quantum pulses, and we use this approach to also show results for Gaussian quantum pulses and to confirm the accuracy of our analytical solutions. In the case of a chiral TLS, we show how a one-photon pulse, of any temporal shape, yields a transmitted long-time spectrum that is identical to the input pulse, despite significant TLS population effects. However, the dynamical spectra and spectral intensity show rich population effects, allowing for their detection in spectroscopic experiments. We also show the striking differences between one-photon and two-photon excitation, where the latter shows clear signatures of nonlinear saturation effects. In addition, we demonstrate how significant population TLS dynamics also occur for pulses that are relatively long compared to the radiative decay time (showing that a weak excitation approximation, which neglects finite TLS population effects, cannot be made) and investigate the population signatures, nonlinear features and dynamical behavior as a function of quantum pulse length.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.