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arXiv:2609.01726

Non-Markovian interactions with pulses of quantum radiation

Julien Pinske, Stefan Scheel

quant-phSubmitted Sep 1, 2026• Announced Sep 3, 2026• 0 citations
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Abstract

The interaction of a traveling pulse of quantum light with a localized quantum system shows non-Markovian features when scattering takes place in a structured environment. Here, we devise a non-Markovian input-output theory by coherently coupling the scatterer to a pseudomode, which decays into a Markovian reservoir. This incorporates memory effects of a structured environment without altering the cascaded nature of the Lindblad master equation, whose solution provides the quantum state of the output field of any desired mode. We apply our theory to the stimulated emission by a two-level atom, and to transmission of a Gaussian pulse through a cavity. We observe that the non-Markovian revival of coherence in the scatterer distorts the single-mode nature of the incoming pulse, thus resulting in a multimode output field.

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The interaction of a traveling pulse of quantum light with a localized quantum system shows non-Markovian features when scattering takes place in a structured environment. Here, we devise a non-Markovian input-output theory by coherently coupling the scatterer to a pseudomode, which decays into a Markovian reservoir. This incorporates memory effects of a structured environment without altering the cascaded nature of the Lindblad master equation, whose solution provides the quantum state of the output field of any desired mode. We apply our theory to the stimulated emission by a two-level atom, and to transmission of a Gaussian pulse through a cavity. We observe that the non-Markovian revival of coherence in the scatterer distorts the single-mode nature of the incoming pulse, thus resulting in a multimode output field.
We present a formalism that accounts for the interaction of a local quantum system, such as an atom or a cavity, with traveling pulses of quantized radiation. We assume Markovian coupling of the stationary system to the input and output fields and nondispersive asymptotic propagation of the pulses before and after the interaction. This permits derivation of a master equation where the input and output pulses are treated as single oscillator modes that both couple to the local system in a cascaded manner. As examples of our theory, we analyze reflection by an empty cavity with phase noise, stimulated atomic emission by a quantum light pulse, and formation of a Schrödinger-cat state by the dispersive interaction of a coherent pulse and a single atom in a cavity.
The interaction of a propagating pulse of quantum radiation with a localized quantum system can be described by a cascaded master equation with a distinct initially populated input and a finally populated output field mode [Kiilerich and M\o{}lmer, Phys. Rev. Lett. 123, 123604 (2019)]. By transformation to an appropriate interaction picture, we break the cascaded nature of the master equation and recover an effective time-dependent interaction with a lossless single mode and a supplementary lossy mode. The former closely represents the traveling pulse, while the latter constitutes a non-Markovian component in the exchange of quanta between the scatterer and the quantized field. The transformed master equation offers important insights into the system dynamics, and it permits numerically efficient solutions.
Non-Markovian behaviour in atomic systems coupled to a structured reservoir of quantum EM field modes, such as in high Q cavities, is treated using a quasimode description, and the pseudo mode theory for single quantum reservoir excitations is obtained via Fano diagonalisation. The atomic transitions are coupled to a discrete set of (cavity) quasimodes, which are also coupled to a continuum set of (external) quasimodes with slowly varying coupling constants. Each pseudomode corresponds to a cavity quasimode, and the original reservoir structure is obtained in expressions for the equivalent atom-true mode coupling constants. Cases of multiple excitation of the reservoir are now treatable via Markovian master equations for the atom-discrete quasimode system.
The dynamics of a three-level atom in a cascade configuration with both transitions coupled to a single structured reservoir of quantized field modes is treated using Laplace transform methods applied to the coupled amplitude equations. Results are also obtained from master equations by two different approaches, that is, involving either pseudomodes or quasimodes. Two different types of reservoir are considered, namely a high-Q cavity and a photonic band-gap system, in which the respective reservoir structure functions involve Lorentzians. Non-resonant transitions are included in the model. In all cases non-Markovian behaviour for the atomic system can be found, such as oscillatory decay for the high-Q cavity case and population trapping for the photonic band-gap case. In the master equation approaches, the atomic system is augmented by a small number of pseudomodes or quasimodes, which in the quasimode approach themselves undergo Markovian relaxation into a flat reservoir of continuum quasimodes. Results from these methods are found to be identical to those from the Laplace transform method including two-photon excitation of the reservoir with both emitting sequences. This shows that complicated non-Markovian decays of an atomic system into structured EM field reservoirs can be described by Markovian models for the atomic system coupled to a small number of pseudomodes or quasimodes.
The dynamics of a three-level atom in a cascade configuration with both transitions coupled to a single structured reservoir of quantized field modes is treated using Laplace transform methods applied to the coupled amplitude equations. Results are also obtained from master equations by two different approaches, that is, involving either pseudomodes or quasimodes. Two different types of reservoir are considered, namely a high-Q cavity and a photonic band-gap system, in which the respective reservoir structure functions involve Lorentzians. Non-resonant transitions are included in the model. In all cases non-Markovian behaviour for the atomic system can be found, such as oscillatory decay for the high-Q cavity case and population trapping for the photonic band-gap case. In the master equation approaches, the atomic system is augmented by a small number of pseudomodes or quasimodes, which in the quasimode approach themselves undergo Markovian relaxation into a flat reservoir of continuum quasimodes. Results from these methods are found to be identical to those from the Laplace transform method including two-photon excitation of the reservoir with both emitting sequences. This shows that complicated non-Markovian decays of an atomic system into structured EM field reservoirs can be described by Markovian models for the atomic system coupled to a small number of pseudomodes or quasimodes.
This paper deals with non-Markovian behavior in atomic systems coupled to a structured reservoir of quantum electromagnetic field modes, with particular relevance to atoms interacting with the field in high-Q cavities or photonic band-gap materials. In cases such as the former, we show that the pseudomode theory for single-quantum reservoir excitations can be obtained by applying the Fano diagonalization method to a system in which the atomic transitions are coupled to a discrete set of (cavity) quasimodes, which in turn are coupled to a continuum set of (external) quasimodes with slowly varying coupling constants and continuum mode density. Each pseudomode can be identified with a discrete quasimode, which gives structure to the actual reservoir of true modes via the expressions for the equivalent atom-true mode coupling constants. The quasimode theory enables cases of multiple excitation of the reservoir to now be treated via Markovian master equations for the atom-discrete quasimode system. Applications of the theory to one, two, and many discrete quasimodes are made. For a simple photonic band-gap model, where the reservoir structure is associated with the true mode density rather than the coupling constants, the single quantum excitation case appears to be equivalent to a case with two discrete quasimodes.