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arXiv:2610.28020

Enhanced orbital-angular-momentum dimensionality and spatial-spectral decoupling in thin-film SPDC

Dmitrii Akatev, Jakub Lewandowski, Maria Chekhova

physics.opticsquant-phSubmitted Oct 20, 2026• Announced Oct 21, 2026• 0 citations
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Abstract

Thin-film spontaneous parametric down-conversion, due to the relaxed phase-matching condition, generates photon pairs that are extremely broadband in frequency and angle and highly entangled in time/frequency and position/momentum. Here we show that it also provides a very broad orbital angular momentum (OAM) spectrum, which, in contrast to the case of bulk crystals, is decoupled from the frequency spectrum. To demonstrate it experimentally, we generate photon pairs in a $7~μ\mathrm{m}$-thick lithium niobate film and compare them with those from a $500~μ\mathrm{m}$-thick periodically poled lithium niobate crystal under identical pump conditions. The thin-film source exhibits a substantially broader OAM spectrum, with the azimuthal Schmidt number almost 9 times larger than that of the bulk source. On this highly entangled state, we perform quantum-state tomography in selected two- and four-dimensional OAM subspaces, demonstrating high-purity maximally entangled states. These results highlight thin nonlinear films as a promising platform for high-dimensional quantum-state generation with weak spatial--spectral coupling.

Comments
10 pages, 5 figures, 1 table

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Thin-film spontaneous parametric down-conversion, due to the relaxed phase-matching condition, generates photon pairs that are extremely broadband in frequency and angle and highly entangled in time/frequency and position/momentum. Here we show that it also provides a very broad orbital angular momentum (OAM) spectrum, which, in contrast to the case of bulk crystals, is decoupled from the frequency spectrum. To demonstrate it experimentally, we generate photon pairs in a 7 μm7~μ\mathrm{m}7 μm-thick lithium niobate film and compare them with those from a 500 μm500~μ\mathrm{m}500 μm-thick periodically poled lithium niobate crystal under identical pump conditions. The thin-film source exhibits a substantially broader OAM spectrum, with the azimuthal Schmidt number almost 9 times larger than that of the bulk source. On this highly entangled state, we perform quantum-state tomography in selected two- and four-dimensional OAM subspaces, demonstrating high-purity maximally entangled states. These results highlight thin nonlinear films as a promising platform for high-dimensional quantum-state generation with weak spatial--spectral coupling.
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Abstract Chip-integrated photon-pair sources based on spontaneous parametric down-conversion (SPDC) have emerged as a promising solution for scalable quantum light generation. Thin-film lithium tantalate (TFLT) is a compelling χ(2)\chi^{(2)}χ(2) platform, combining strong nonlinearity with a high optical-damage threshold, weak photorefractive response, and ferroelectricity that enables quasi-phase matching. However, SPDC-based photon-pair generation on TFLT has not yet been demonstrated. Here, we combine high-quality periodic poling with low-loss nanophotonic waveguides to realize photon-pair sources on TFLT in both traveling-wave and resonant configurations. In periodically poled straight waveguides, we achieve broadband photon-pair generation with high efficiency (2.1~GHz~mW−1^{-1}−1) and coincidence-to-accidental ratio (up to 3.8×1053.8\times10^{5}3.8×105). We further confirm high-purity single-photon operation via heralded second-order correlation (gH(2)(0)=0.0018±0.0002g^{(2)}_\mathrm{H}(0) = 0.0018 \pm 0.0002gH(2)​(0)=0.0018±0.0002) and high-fidelity time-energy entanglement through Franson interference (visibility of 98.9±0.5%98.9 \pm 0.5\%98.9±0.5%). In periodically poled racetrack resonators, we map out a broad quantum frequency comb spanning the telecom C- and L-bands. By isolating individual frequency-correlated pairs, we measure a high spectral brightness of 11~GHz~mW−1^{-1}−1~GHz−1^{-1}−1. These results are competitive with the state of the art across χ(2)\chi^{(2)}χ(2) integrated platforms, positioning TFLT as a strong contender for integrated quantum light sources, with applications in wavelength-multiplexed quantum communications and photonic quantum information processing.
The orbital angular momentum (OAM) of photons provides a high-dimensional resource for quantum information protocols. The dimensionality of OAM-entangled states generated via spontaneous parametric down-conversion (SPDC) is quantified by the angular Schmidt spectrum. Here, we experimentally investigate the dependence of the angular Schmidt spectrum on the thickness of the nonlinear crystal. Contrary to previous studies reporting a monotonic decrease in the Schmidt number with increasing crystal thickness, we report the first experimental observation of a nonmonotonic behavior, as we demonstrate an increase in the Schmidt number beyond a certain crystal thickness. We attribute this to the spatial walk-off effect in the anisotropic nonlinear crystal and explain it using a theoretical model that is devoid of standard phase-matching approximations. These findings can have important implications for high-dimensional entangled state generation.
Entanglement, as a crucial feature of quantum systems, is essential for various applications of quantum technologies. High-dimensional entanglement has the potential to encode arbitrary large amount of information and enhance robustness against eavesdropping and quantum cloning. The orbital angular momentum (OAM) entanglement can achieve the high-dimensional entanglement nearly for free stems due to its discrete and theoretically infinite-dimensional Hilbert space. A stringent limitation, however, is that the phase-matching condition limits the entanglement dimension because the coincidence rate decreases significantly for high-order modes. Here we demonstrate relatively flat high-dimensional OAM entanglement based on a spontaneous parametric down conversion (SPDC) from an ultrathin nonlinear lithium niobite crystal. The difference of coincidences between the different-order OAM modes significantly decreases. To further enhance the nonlinear process, this microscale SPDC source will provide a promising and integrated method to generate optimal high-dimensional OAM entanglement.
Abstract Broadband photon pairs are highly desirable for quantum metrology, quantum sensing, and quantum communication. Such sources are usually designed through type-0 phase-matching spontaneous parametric down-conversion (SPDC) that makes the photon pairs hard to separate in the frequency-degenerate case and thus limits their applications. In this paper, we design a broadband frequency-degenerate telecom-band photon pair source via the type-II SPDC in a dispersion-engineered thin-film lithium niobate waveguide, where the polarization modes of photon pairs are orthogonal and thus are easily separated deterministically. With a 5-mm-long waveguide, our design can achieve a bandwidth of 5.56 THz (44.8 nm), which is 8.6 times larger than that of the bulk lithium niobate, and the central wavelength can be flexibly adjusted. Our design is a promising approach towards high-quality integrated photon sources and may have wide applications in photonic quantum technologies.
Entangled photon pairs play a major role in various modern technologies such as quantum imaging, communication, and computing. Conventional photon-pair sources are often based on spontaneous parametric down-conversion in bulk nonlinear crystals. Recent advances have also shown entangled photon-pairs from transition metal dichalcogenide thin-films, however, these materials are not widely available and are not compatible with existing fabrication capabilities. We present a new thin-film lithium niobate source of polarization-entangled photon pairs at the telecom wavelength that requires no additional optical elements for entanglement generation and allows for easy application using the existing lithium niobate fabrication technologies. We demonstrate tunable entanglement generation using the three-fold rotational crystal symmetry of lithium niobate, allowing the generation of different maximally entangled Bell states or completely separable states depending on the polarization of the pump beam.