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arXiv:2610.12406

Local polarization control of optical tweezer arrays

Xiangkai Sun, Richard Bing-Shiun Tsai, Andrew Winnicki, Yuan Le, Kon H. Leung, Nelson Darkwah Oppong, Manuel Endres

physics.atom-phphysics.opticsquant-phSubmitted Oct 8, 2026• Announced Oct 9, 2026• 0 citations
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Abstract

Optical tweezer arrays trapping ultracold atoms and molecules are a versatile quantum science platform with broad impact in quantum simulation, quantum computation, and quantum metrology. The polarization dependence of anisotropic vector and tensor light shifts offers a degree of freedom for precise quantum state engineering of trapped particles. Similarly, state-selective operations depend on the polarization of the addressing light through the atom--light coupling strength. Yet, methods for controlling the polarization of individual tweezers or local addressing beams remain an experimental challenge. Here, we demonstrate independent, site-resolved linear polarization rotation across an optical tweezer array by exploiting the local birefringence tunability of a spatial light modulator. Applying this capability to an array of $^{88}\rm{Sr}$ atoms, we homogenize differential light shifts imparted by the 813-nm tweezers to the narrow ${^1{\rm S}_0}\leftrightarrow{^3{\rm P}_1}$ transition, enabling sideband cooling under a magic-angle condition. Furthermore, we show dynamic transport of trapped atoms across distinct polarization zones with high survival and preserved coherence. Finally, we characterize tweezer polarization noise and demonstrate closed-loop stabilization referenced to the atomic transition frequency, reaching mrad-level stability. Our work establishes a technique for manipulating polarization-sensitive atomic and molecular transitions in tweezer architectures, with immediate applications to optical tweezer clocks and multi-zone quantum processors.

Comments
11 pages, 5 figures

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Optical tweezer arrays trapping ultracold atoms and molecules are a versatile quantum science platform with broad impact in quantum simulation, quantum computation, and quantum metrology. The polarization dependence of anisotropic vector and tensor light shifts offers a degree of freedom for precise quantum state engineering of trapped particles. Similarly, state-selective operations depend on the polarization of the addressing light through the atom--light coupling strength. Yet, methods for controlling the polarization of individual tweezers or local addressing beams remain an experimental challenge. Here, we demonstrate independent, site-resolved linear polarization rotation across an optical tweezer array by exploiting the local birefringence tunability of a spatial light modulator. Applying this capability to an array of 88Sr^{88}\rm{Sr}88Sr atoms, we homogenize differential light shifts imparted by the 813-nm tweezers to the narrow 1S0↔3P1{^1{\rm S}_0}\leftrightarrow{^3{\rm P}_1}1S0​↔3P1​ transition, enabling sideband cooling under a magic-angle condition. Furthermore, we show dynamic transport of trapped atoms across distinct polarization zones with high survival and preserved coherence. Finally, we characterize tweezer polarization noise and demonstrate closed-loop stabilization referenced to the atomic transition frequency, reaching mrad-level stability. Our work establishes a technique for manipulating polarization-sensitive atomic and molecular transitions in tweezer architectures, with immediate applications to optical tweezer clocks and multi-zone quantum processors.
Ultracold molecules are attractive candidates for various applications including ultracold chemistry, quantum information processing, quantum simulation and searches for physics beyond the standard model. Combined with optical tweezer techniques, an optical tweezer array of ultracold polar molecules holds promise for versatile quantum applications. Their long-lived molecular rotational states form robust qubits, while the long-range dipolar interaction between molecules provides quantum entanglement. In this thesis, we build a new generation experiment of optical tweezer array of ultracold CaF molecules. We optically transport the laser cooled and optically trapped molecules into a science glass cell using a hybrid method, where high numerical aperture optical access allows for tighter optical tweezers. In an array of these tight optical tweezers, we demonstrate dipolar spin-exchange interactions between single CaF molecules for the first time. We realize the spin-12\frac{1}{2}21​ quantum XY model by encoding an effective spin-12\frac{1}{2}21​ system into the rotational states of the molecules, and use it to generate a Bell state through an iSWAP operation. Conditioned on the verified existence of molecules in both tweezers at the end of the measurement, we obtain a Bell state fidelity of 0.89(6). Employing interleaved tweezer arrays, we demonstrate single site molecular addressability. To further improve the platform, cooling of the molecules to near the motional ground state is crucial for reducing various dephasings. We demonstrate Raman sideband cooling (RSC) of CaF molecules in optical tweezers to near their 3-D motional ground state, with a 3-D motional ground state probability of 54±18%54\pm18\%54±18% of the molecules that survive the RSC. This paves the way to increase molecular coherence times in optical tweezers for robust quantum information processing and simulation applications in the near future.
Laser cooling of single atoms in optical tweezers is a prerequisite for neutral atom quantum computing and simulation. Resolved sideband cooling comprises a well-established method for efficient motional ground-state preparation, but typically requires careful cancellation of light shifts in so-called magic traps. Here, we study a novel laser cooling scheme which overcomes such constraints, and applies when the ground state of a narrow cooling transition is trapped stronger than the excited state. We demonstrate our scheme, which exploits sequential addressing of red sideband transitions via frequency chirping of the cooling light, at the example of 88Sr^{88}\mathrm{Sr}88Sr atoms and report ground-state populations compatible with recent experiments in magic tweezers. The scheme also induces light-assisted collisions, which are key to the assembly of large atom arrays. Our work enriches the toolbox for tweezer-based quantum technology, also enabling applications for tweezer-trapped molecules and ions that are incompatible with resolved sideband cooling conditions.
Optical tweezer arrays 1,2 have transformed atomic and molecular physics, now forming the backbone for a range of leading experiments in quantum computing 3–8 , simulation 1,9–12 , and metrology 13–15 . Typical experiments trap tens to hundreds of atomic qubits, and recently systems with around one thousand atoms were realized without defining qubits or demonstrating coherent control 16–18 . However, scaling to thousands of atomic qubits with long coherence times, low-loss, and high-fidelity imaging is an outstanding challenge and critical for progress in quantum science, particularly towards quantum error correction 19,20 . Here, we experimentally realize an array of optical tweezers trapping over 6,100 neutral atoms in around 12,000 sites, simultaneously surpassing state-of-the-art performance for several metrics that underpin the success of the platform. Specifically, while scaling to such a large number of atoms, we demonstrate a coherence time of 12.6(1) seconds, a record for hyperfine qubits in an optical tweezer array. We show room-temperature trapping lifetimes of ~ 23 minutes, enabling record-high imaging survival of 99.98952(1)% with an imaging fidelity of over 99.99%. We present a plan for zone-based quantum computing 5,21 and demonstrate necessary coherence-preserving qubit transport and pick-up/drop-off operations on large spatial scales, characterized through interleaved randomized benchmarking. Our results, along with recent developments 8,22–24 , indicate that universal quantum computing and quantum error correction with thousands to tens of thousands of physical qubits could be a near-term prospect.
Neutral atoms trapped by laser light are among the most promising candidates for storing and processing information in a quantum computer or simulator. The application certainly calls for a scalable and flexible scheme for addressing and manipulating the atoms. We have now made this a reality by implementing a fast and versatile method to dynamically control the position of neutral atoms trapped in optical tweezers. The tweezers result from a spatial light modulator (SLM) controlling and shaping a large number of optical dipole-force traps. Trapped atoms adapt to any change in the potential landscape, such that one can rearrange and randomly access individual sites within atom-trap arrays.
Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the control and readout of individually trapped polar molecules in an array of optical tweezers. Starting with arrays of up to eight Rb and eight Cs atoms, we assemble arrays of RbCs molecules in their rovibrational and hyperfine ground state with an overall efficiency of 48(2)%. We demonstrate global microwave control of multiple rotational states of the molecules and use an auxiliary tweezer array to implement site-resolved addressing and state control. We show how the rotational state of the molecule can be mapped onto the position of Rb atoms and use this capability to readout multiple rotational states in a single experimental run. Further, using a scheme for the midsequence detection of molecule formation errors, we perform rearrangement of assembled molecules to prepare small defect-free arrays. Finally, we discuss a feasible route to scaling to larger arrays of molecules. Published by the American Physical Society 2024
Optical tweezer arrays of neutral atoms have emerged as a versatile and powerful platform for quantum simulation and quantum information processing. In this thesis, I present the realization of an experimental platform for quantum simulation based on individually trapped strontium atoms in optical tweezer arrays. The experiment combines precise laser cooling, optical control, and high-resolution imaging to enable the manipulation and high fidelity detection of single atoms. I developed and optimized a two-stage three-dimensional magneto-optical trap (3D-MOT) that produces cold and dense samples of strontium atoms from a thermal beam. In the f irst stage, atoms are captured and precooled using the dipole-allowed 1S0 → 1P1 transition at 461nm (which has a linewidth of !=2ω ↑ 32MHz). The second stage employs the 1S0 → 3P1 narrow intercombination transition at 689nm (with a linewidth of !=2ω ↑7.5kHz) to further cool and compress the atomic cloud. By optimizing the trapping parameters, I achieved clouds with temperatures around 5μK and densities above 1010cm→3, providing ideal initial conditions for e!cient loading into optical tweezers. A 3↑3 array of 360μK deep optical tweezers is generated by spatially modulating an 813.4nm laser beam using two crossed acousto-optic deflectors. The deflected beams are relayed and focused into the science chamber using a high–numericalaperture objective, which simultaneously serves as the collection optics for atomic f luorescence. The fluorescence light emitted by the atoms is imaged onto a scientific qCMOS camera, enabling site-resolved detection of individual atoms. I implemented and optimized the in-trap cooling dynamics to prevent atom loss during imaging and to minimize residual thermal motion. In addition, by precisely tuning lightassisted collisions, multiple atoms occupancies are removed from the traps and a single-atom regime is reached in the array, with a filling fraction of about 50%. I have demonstrated a single-atom detection fidelity of 99,986(1)% and a survival probability of 97(2)% between subsequent image acquisition, comparable to other current state-of-the-art experiments. To characterize the platform, I carried out release-and-recapture experiments, from which it is possible to measure a temperature for the individually trapped atoms of 12.95(5)μK. These results demonstrate the successful implementation of a robust and high-fidelity platform for optical trapping and imaging of single strontium atoms. The apparatus provides the foundation for future quantum simulation experiments with alkalineearth atoms excited to the Rydberg state, o"ering precise control over individual particles and the ability to scale towards larger, programmable atomic arrays.