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arXiv:2609.31043

Single-shot coherent process tomography and mid-infrared polarimetry with undetected photons

Marthe Zeja, Wen-Zhe Yan, Zhibo Hou, Sven Ramelow

quant-phphysics.opticsSubmitted Sep 25, 2026• Announced Sep 28, 2026• 0 citations
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Abstract

Measurements with undetected photons infer properties of a probe beam that is never detected, transferring mid-infrared information onto silicon-friendly wavelengths. Tomography in this paradigm has so far relied on switched settings or scanned phases, referenced across a drift-sensitive campaign; no protocol reads all Jones parameters from one frame. We show that a folded nonlinear interferometer with a diagonally pumped crossed-crystal source performs coherent process tomography of the undetected beam in a single spectrometer frame: it reconstructs all seven parameters of the beam's round-trip Jones matrix, the coherent part of the channel. Birefringent group-delay walk-off, normally a calibration nuisance, acts as a frequency multiplexer: each Jones-matrix element is assigned its own carrier, a spectral fringe period paired with a detector port. Because the multiplexing exploits the down-conversion bandwidth rather than merely tolerating it, a single Fourier transform per detector trace returns all four moduli and all three relative phases across that bandwidth, i.e., the full round-trip Jones spectrum up to a global phase, with no scan or setting change (after a one-time reference frame). Simultaneity makes every relative phase immune to common-mode drift, and a dark carrier, a self-interference term that unitarity forces to vanish, provides a built-in null test. For realistic parameters of a periodically poled KTP source the scheme yields wavelength-resolved mid-infrared polarimetry across 3.5-4.2 microns (~80 spectral points per Jones element) on a silicon camera, extending to depth-resolved Jones matrices, i.e., polarization-sensitive optical coherence tomography with undetected photons. A Fisher-information analysis, the first we are aware of in undetected-photon tomography, sets the precision budget and compares delay multiplexing to sequential protocols at equal photon number.

Comments
27 pages, 3 figures, 5 tables

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Measurements with undetected photons infer properties of a probe beam that is never detected, transferring mid-infrared information onto silicon-friendly wavelengths. Tomography in this paradigm has so far relied on switched settings or scanned phases, referenced across a drift-sensitive campaign; no protocol reads all Jones parameters from one frame. We show that a folded nonlinear interferometer with a diagonally pumped crossed-crystal source performs coherent process tomography of the undetected beam in a single spectrometer frame: it reconstructs all seven parameters of the beam's round-trip Jones matrix, the coherent part of the channel. Birefringent group-delay walk-off, normally a calibration nuisance, acts as a frequency multiplexer: each Jones-matrix element is assigned its own carrier, a spectral fringe period paired with a detector port. Because the multiplexing exploits the down-conversion bandwidth rather than merely tolerating it, a single Fourier transform per detector trace returns all four moduli and all three relative phases across that bandwidth, i.e., the full round-trip Jones spectrum up to a global phase, with no scan or setting change (after a one-time reference frame). Simultaneity makes every relative phase immune to common-mode drift, and a dark carrier, a self-interference term that unitarity forces to vanish, provides a built-in null test. For realistic parameters of a periodically poled KTP source the scheme yields wavelength-resolved mid-infrared polarimetry across 3.5-4.2 microns (~80 spectral points per Jones element) on a silicon camera, extending to depth-resolved Jones matrices, i.e., polarization-sensitive optical coherence tomography with undetected photons. A Fisher-information analysis, the first we are aware of in undetected-photon tomography, sets the precision budget and compares delay multiplexing to sequential protocols at equal photon number.
Mid-infrared (mid-IR) light scatters much less than shorter wavelengths, allowing greatly enhanced penetration depths for optical imaging techniques such as optical coherence tomography (OCT). However, both detection and broadband sources in the mid-IR are technologically challenging. Interfering entangled photons in a nonlinear interferometer enables sensing with undetected photons, making mid-IR sources and detectors obsolete. Here we implement mid-IR frequency-domain OCT based on ultra-broadband entangled photon pairs spanning from 3.3 to 4.3 µm. We demonstrate 10 µm axial and 20 µm lateral resolution 2D and 3D imaging of strongly scattering ceramic and paint samples. By intrinsically being limited only by shot noise, we observe times more sensitivity per integration time and power of the probe light. Together with the vastly reduced footprint and technical complexity, our technique can outperform conventional approaches with classical mid-IR light sources.
We propose a theoretical polarization tomography scheme within the quantum imaging with undetected photons (QIUP) framework that extracts the Jones matrix elements, describing the sample's polarization response from interference visibilities and phase shifts. By exploiting inherent constraints among the Jones matrix elements based on the assumptions of fully polarized pure states and linear, non-depolarizing components, the method reduces the number of unknowns required for reliable reconstruction. The same interference-based protocol is also demonstrated for a fully generalized Jones matrix, extending the approach to a broader class of polarization responses. This scheme is well suited for polarization-resolved QIUP implementations with minimal measurement requirements and enables non-invasive characterization of complex samples at different probing and detection wavelengths.
Quantum imaging with undetected photons (QIUP) allows an object to be probed at mid-infrared frequencies by only measuring interference in the visible range, thus leveraging silicon camera technology. We show that non-collinear phase-matching in a silver thiogallate (AgGaS2_22​) crystal enables wide-field QIUP in the wavelength range of 6-10 μμμm (1670-1000 cm−1^{-1}−1). A combination of coherent detection and infrared photons being ``undetected'' enables imaging at ${\sim}$100 times better than the background-limited infrared photodetection (BLIP) limit. At 8 μμμm, our images have over 8000 ±\pm± 100 resolvable elements with a 297 ±\pm± 5 μμμm resolution, and 10 s acquisition time. Our results pave the way to fast, background-noise-free, room-temperature, spectrally-selective mid-infrared imaging.
Quantum sensing in the infrared regime often demands the use of expensive and cryogenically operated detectors. Nonlinear interferometry has paved the way for information transfer from the infrared to the near--infrared or visible regime in various quantum technologies. A particularly interesting application of these interferometers involves spectrally--resolved quantum imaging using undetected photons, enabled by the use of temperature--tunable parametric amplifiers. In this work, we demonstrate spectrally resolved transmission imaging with undetected photons around 1550 nm using a spontaneous parametric down conversion based folded nonlinear interferometric scheme, registering the attenuation of a zebrafish larva as a biological feasibility test. We characterize and calibrate the interferometer, having achieved spectrally resolved interference fringes with a maximum baseline visibility of ∼74%\sim 74\%∼74% in the near--infrared regime. Phase--stepped readout of a grating spectrometer gives a resolving power of ∼1460\sim1460∼1460 (from the spectrometer's point spread function) at 1550 nm, and ∼730\sim 730∼730 from the coherence length, the finest reported for imaging with undetected photons, over an instantaneous spectral window of ≈51\approx 51≈51 cm−1^{-1}−1.
Nonlinear SU(1,1) quantum interferometers based on non-degenerate optical parametric down-conversion exhibit strong unbalanced group velocity dispersion (GVD). This feature is intrinsic to this type of interferometer as correlated photons of vastly different frequencies propagate through a dispersive nonlinear crystal; consequently, the dispersion arises from the source itself. The resulting GVD degrades the axial point-spread function (PSF) in optical coherence tomography (OCT) with undetected photons; and physical compensation is less straightforward, in particular for non-degenerate broadband regimes due to the limited number of suitable materials. In this contribution, we analyze dispersion in bulk nonlinear interferometry and describe its implications for OCT imaging. Aspects of hardware compensation are addressed, and a novel empirical numerical method of compensation is proposed. The approach is based on the extraction of the phase component directly from the time-domain modality (high precision linearized quantum Fourier transform infrared spectrometer) and its injection into the mid-IR spectral-domain OCT signals (central wavelength of around 3770 nm) before the Fourier transform. The proposed method is compared with an alternative numerical technique. The results demonstrate a 2.2-fold improvement in axial resolution and outperform the alternative correction method in overall imaging performance.