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arXiv:2609.20698

Multinegativity and single-letter formulas for asymptotic entanglement

Raphael Brinster, Tulja Varun Kondra, Hermann Kampermann, Dagmar Bruß, Nikolai Wyderka

quant-phSubmitted Sep 17, 2026• Announced Sep 18, 2026• 0 citations
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Abstract

The study of entanglement inevitably leads to the concept of regularization, where measures are evaluated on infinitely many copies of a state. Single-letter formulas try to make these asymptotic entanglement quantities accessible through a calculation on one copy of a state, but are rarely available. We introduce a decreasing hierarchy of computable upper bounds on the asymptotic relative entropy of entanglement with respect to positive-partial-transpose (PPT) states. The regularization of every fixed hierarchy level equals this asymptotic quantity. Additivity at any level therefore yields a single-letter formula, even when the usual one-copy relative entropy is nonadditive. We establish such additivity at the first nontrivial level for two broad multiparameter families, both containing all Werner states. The upper-bound construction also extends to sandwiched Renyi divergences. The hierarchy motivates $k$-multinegative states, a generalization of binegative states and the associated $k$-multinegativity, which gives explicit upper bounds on both the asymptotic relative entropy and exact PPT entanglement cost. We construct states which are $k$-multinegative at arbitrarily large depths $k$ that separate consecutive levels of the previously introduced entanglement-cost hierarchy, disproving its conjectured finite collapse. These results provide state-dependent single-letter formulas while identifying a limitation of universal finite-level characterizations.

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The study of entanglement inevitably leads to the concept of regularization, where measures are evaluated on infinitely many copies of a state. Single-letter formulas try to make these asymptotic entanglement quantities accessible through a calculation on one copy of a state, but are rarely available. We introduce a decreasing hierarchy of computable upper bounds on the asymptotic relative entropy of entanglement with respect to positive-partial-transpose (PPT) states. The regularization of every fixed hierarchy level equals this asymptotic quantity. Additivity at any level therefore yields a single-letter formula, even when the usual one-copy relative entropy is nonadditive. We establish such additivity at the first nontrivial level for two broad multiparameter families, both containing all Werner states. The upper-bound construction also extends to sandwiched Renyi divergences. The hierarchy motivates kkk-multinegative states, a generalization of binegative states and the associated kkk-multinegativity, which gives explicit upper bounds on both the asymptotic relative entropy and exact PPT entanglement cost. We construct states which are kkk-multinegative at arbitrarily large depths kkk that separate consecutive levels of the previously introduced entanglement-cost hierarchy, disproving its conjectured finite collapse. These results provide state-dependent single-letter formulas while identifying a limitation of universal finite-level characterizations.
Quantum information theory is plagued by the problem of regularizations, which require the evaluation of formidable asymptotic quantities. This makes it computationally intractable to gain a precise quantitative understanding of the ultimate efficiency of key operational tasks such as entanglement manipulation. Here, we consider the problem of computing the asymptotic entanglement cost of preparing noisy quantum states under quantum operations with positive partial transpose (PPT). By means of an analytical example, a previously claimed solution to this problem is shown to be incorrect. Building on a previous characterization of the PPT entanglement cost in terms of a regularized formula, we construct instead a hierarchy of semidefinite programs that bypasses the issue of regularization altogether, and converges to the true asymptotic value of the entanglement cost. Our main result establishes that this convergence happens exponentially fast, thus yielding an efficient algorithm that approximates the cost up to an additive error ϵ in time poly(D,log(1/ϵ)), where D is the underlying Hilbert space dimension. To our knowledge, this is the first time that an asymptotic entanglement measure is shown to be efficiently computable despite no closed-form formula being available.
We study entanglement distillation under operations that remain completely positive under partial-transpose conjugation, a.k.a. PPT channels, in the standard quantum Shannon theory regime of asymptotically vanishing but non-zero error. Our main results are: (a) a regularised formula for the PPT distillable entanglement in terms of a measured-relative-entropy-like quantity; and (b) two different single-letter converses, one based on operator quadratic forms and the other on Hirschman's strengthening of the Hadamard three-line theorem. As an immediate application of (b), we show that the PPT distillable entanglement can be strictly smaller than the regularised Rains bound, thereby resolving an open problem in the theory of entanglement manipulation [Regula et al., NJP 21:103017, 2019]. A gap appears already for 3×33\times 33×3 Werner states: at antisymmetric weight 25/2625/2625/26, a certified upper bound of 0.621070.621070.62107 ebits lies below the (regularised) Rains bound, which equals 2526log⁡25−log⁡23≈0.64766\frac{25}{26} \log_2 5 - \log_2 3 \approx 0.647662625​log2​5−log2​3≈0.64766 ebits. On a different note, (a) implies a faithful lower bound on the PPT distillable entanglement in terms of the entanglement negativity, which provides a quantitative counterpart to the qualitatively known fact that any NPT state is PPT distillable [Eggeling et al., PRL 87:257902, 2001].
The one-way distillable entanglement is a central operational measure of bipartite entanglement, quantifying the optimal rate at which maximally entangled pairs can be extracted by one-way LOCC. Despite its importance, it is notoriously hard to compute, since it is defined by a regularized optimization over many copies and adaptive one-way protocols. At present, single-letter formulas are only known for (conjugate) degradable and PPT states. More generally, it has remained unclear when one-way distillable entanglement can still be additive beyond degradability and PPT settings, and how such additivity relates to additivity questions of quantum capacity of channels. In this paper, we address this gap by identifying three explicit families of non-degradable and non-PPT states whose one-way distillable entanglement is nevertheless single-letter. First, we introduce two weakened degradability-type conditions--regularized less-noisy and informationally degradable--and prove that each guarantees additivity and hence a single-letter formula. Second, we show a stability result for orthogonally flagged mixtures: when one component has orthogonal support on Alice's system and zero one-way distillable entanglement, the mixture remains single-letter, even though degradability is typically lost under such mixing. Finally, we propose a generalized spin-alignment principle for entropy minimization in tensor-product settings, which we establish in several key cases, including a complete Rényi-2 result. As an application, we obtain additivity results for generalized direct-sum channels and their corresponding Choi states.
This paper establishes single-letter formulas for the exact entanglement cost of simulating quantum channels under free quantum operations that completely preserve positivity of the partial transpose (PPT). First, we introduce the $\ensuremath{\kappa}$-entanglement measure for point-to-point quantum channels, based on the idea of the $\ensuremath{\kappa}$ entanglement of bipartite states, and we establish several fundamental properties for it, including amortization collapse, monotonicity under PPT superchannels, additivity, normalization, faithfulness, and nonconvexity. Second, we introduce and solve the exact entanglement cost for simulating quantum channels in both the parallel and sequential settings, along with the assistance of free PPT-preserving operations. In particular, we establish that the entanglement cost in both cases is given by the same single-letter formula, the $\ensuremath{\kappa}$-entanglement measure of a quantum channel. We further show that this cost is equal to the largest $\ensuremath{\kappa}$ entanglement that can be shared or generated by the sender and receiver of the channel. This formula is calculable by a semidefinite program, thus allowing for an efficiently computable solution for general quantum channels. Noting that the sequential regime is more powerful than the parallel regime, another notable implication of our result is that both regimes have the same power for exact quantum channel simulation, when PPT superchannels are free. For several basic Gaussian quantum channels, we show that the exact entanglement cost is given by the Holevo-Werner formula [Holevo and Werner, Phys. Rev. A 63, 032312 (2001)], giving an operational meaning of the Holevo-Werner quantity for these channels.
Exact entanglement distillation converts a noisy bipartite state into a maximally entangled state with zero error. Under completely PPT-preserving operations, the additive min-Rains relative entropy provides a single-letter upper bound on the regularized distillation rate. An interesting problem in entanglement theory dating back to 2016 has been whether this bound is always tight. Here we resolve this question in the negative. The key is a tensor-stable rigidity absent from the min-Rains relaxation: every feasible exact-distillation effect must act as the identity on the support of the input state. We convert this constraint into a new single-letter upper bound using a generally non-Hermitian, range-supported witness. For a rank-three subspace, we show this upper bound lies strictly below the min-Rains relative entropy for every state with that support. Thus, the constraint discarded by the min-Rains relaxation remains relevant under arbitrary tensor powers. Our result rules out the min-Rains relative entropy as a closed-form formula for exact PPT distillable entanglement and reveals the subtle asymptotic structure of exact entanglement manipulation under PPT operations.
Quantum catalysts can overcome otherwise impossible quantum state transformations without being consumed, and allowing them to become correlated with the output makes this assistance substantially more powerful. This raises a fundamental question for entanglement theory: which limitations on state manipulation remain when such correlated catalysts are freely available? We answer this question in the positive-partial-transpose (PPT) resource theory, which allows a substantially broader class of operations than local operations and classical communication (LOCC). We identify general conditions under which regularized relative-entropy measures become strongly superadditive, and use them to construct monotones that constrain correlated catalytic PPT transformations without any knowledge of the catalyst. In particular, we prove that the regularized PPT relative entropy is fully additive and strongly superadditive, resolving an open problem in entanglement theory. Most importantly, these constraints show that even arbitrary correlated catalysts cannot restore asymptotic reversibility: for an explicit state, the optimal entanglement distillation rate remains strictly smaller than the entanglement cost. Thus, substantial catalytic assistance does not remove some of the fundamental limitations of mixed-state entanglement manipulation.