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arXiv:2608.10087

Long-lived memory effects in the defect bath of superconducting qubits

Abhishek Agarwal, Masum Uddin, Shroya Vaidya, Lachlan P. Lindoy, Ehsaneh Daghigh Ahmadi, Tobias Lindström, Sebastian E. de Graaf, Ivan Rungger

quant-phSubmitted Aug 10, 2026• Announced Aug 12, 2026• 0 citations
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Abstract

We reveal long-lived memory effects in the defect bath of a superconducting transmon qubit through electric-field tuning of two-level system (TLS) defects coupled to the qubit. Using a fast TLS mapping method we observe several hysteretic effects in the TLS environment with memory timescales of the order of seconds, far beyond the lifetimes of individual TLS defects. The observations can be explained by TLS coupling to electric field-polarised charge fluctuators in the defect bath. Our method enables detailed mapping of the dynamics of the bath's coupled microscopic degrees of freedom and the associated memory effects which can introduce temporally correlated noise. This information may be used to improve qubit-stabilisation and quantum error correction protocols.

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We reveal long-lived memory effects in the defect bath of a superconducting transmon qubit through electric-field tuning of two-level system (TLS) defects coupled to the qubit. Using a fast TLS mapping method we observe several hysteretic effects in the TLS environment with memory timescales of the order of seconds, far beyond the lifetimes of individual TLS defects. The observations can be explained by TLS coupling to electric field-polarised charge fluctuators in the defect bath. Our method enables detailed mapping of the dynamics of the bath's coupled microscopic degrees of freedom and the associated memory effects which can introduce temporally correlated noise. This information may be used to improve qubit-stabilisation and quantum error correction protocols.
Understanding the microscopic environment of superconducting qubits is a central challenge for quantum technologies. Parasitic two-level systems (TLSs) of various microscopic origins are ubiquitous and limit qubit performance through decoherence, frequency drifts, and leakage. Recently, long-lived TLSs with lifetimes exceeding those of state-of-the-art qubits have been shown to induce correlated qubit dynamics, with direct implications for quantum error correction. Here, we perform wide-band quantum-jump correlation spectroscopy on flux-tunable transmon qubits and identify microscopic degrees of freedom that outlive the qubit by orders of magnitude. Pump-probe measurements at varying detunings from these objects reveal intrinsic lifetimes exceeding one second. Their weak coupling to the qubit, in the kilohertz range, is consistent with positional defects described by the standard tunneling model, without excluding other microscopic origins such as magnetic spin impurities or trapped quasiparticles. More broadly, these results establish superconducting qubits as a sensitive probe of exceptionally long-lived microscopic degrees of freedom and open a route toward their controlled access and functionalization.
Materials improvements in transmon qubits have yielded remarkable advances in qubit lifetimes (T1)and coherence times (T2). However, state-of-the-art superconducting qubits experience temporal fluctuations in their performance, which limit gate fidelities and quantum processor performance. We observe correlated increases in qubit relaxation and dephasing rates that last for minutes to hours, which we call T1 and T2 excursions. Using interleaved lifetime and coherence time measurements, noise spectroscopy, and two-level-system (TLS) spectroscopy, we find that these excursions are caused by single or few strongly-coupled TLS defects that spectrally diffuse into resonance with the qubit frequency. Our measurement protocol provides a powerful tool for understanding the noise sources that cause temporal fluctuations in superconducting qubit performance.
Microscopic two-level systems (TLS) -- ubiquitous atomic-scale defects in solid-state quantum devices -- are a dominant source of qubit decoherence, yet their role is often considered local and short-memoried. Here, we report the observation of a coherent TLS that couples simultaneously to two spatially distant superconducting qubits. The TLS is identified to reside within the tunable coupler linking the qubits, enabling controllability of the TLS-qubit coupling strength via coupler frequency -- a capability absent in earlier studies. This tunability allows us to systematically probe how TLS distorts qubit dynamics, revisiting the decoherence model in the presence of non-Markovian TLS dephasing noise. This is corroborated by the reconstructed 1/f1/f1/f noise spectrum of TLS frequency fluctuation spanning more than ten orders of magnitude (0.1\,mHz -- 1\,MHz) that reveals discrete fluctuator signatures. Quantum process tomography further unveils TLS-induced correlated qubit dynamics, highlighting the long-lived TLS as an effective source of non-Markovianity. Our findings expose a previously overlooked interaction mechanism in scalable quantum architectures: defects embedded in coupling elements can simultaneously affect multiple qubits with variable impact. Beyond immediate implications for system characterization and calibration, this situation provides a powerful testbed for studying defect-driven quantum dynamics, refining error suppression strategies, and advancing architecture design for scalable quantum technologies.
Achieving fault tolerance with superconducting quantum processors requires qubits to operate within the regime of threshold theorems based on the Born-Markov approximation. This approximation, which models dissipation as constant energy decay into a memoryless environment, breaks down when qubits couple to long-lived two-level systems (TLSs) that become polarized during operation and retain memory of past qubit states. Here, we show that non-Poissonian quantum jump traces carry the information required to distinguish long-lived TLSs from the standard Markovian bath. By fitting the Solomon equations to measured quantum jumps dynamics arising naturally due to thermal fluctuations, we can disentangle the coupling of the qubit to the two environments. Sweeping the qubit frequency reveals distinct peaks, each associated with a TLS that outlives the qubit, providing a handle to understand their microscopic origin.
Transmon qubits are a cornerstone of modern superconducting quantum computing platforms. Temporal fluctuations of energy relaxation in these qubits are widely attributed to microscopic two-level systems (TLSs) in device dielectrics and interfaces, yet isolating individual defects typically relies on tuning the qubit or the TLS into resonance. We demonstrate a novel spectroscopy method for fixed-frequency transmons based on multilevel relaxation: repeated preparation of the second excited state and simultaneous T1T_1T1​ extraction of the first and second excited states reveals characteristic correlations in the decay rates of adjacent transitions. From these correlations we identify one or more dominant TLSs and reconstruct their frequency drift over time. Remarkably, we find that TLSs detuned by ≳100 MHz\gtrsim 100\,\mathrm{MHz}≳100MHz from the qubit transition can still significantly influence relaxation. The proposed method provides a powerful tool for TLS spectroscopy without the need to tune the transmon frequency, either via a flux-tunable inductor or AC-Stark shifts.
Parasitic two-level-system (TLS) defects are a major source of energy relaxation and temporal instability in superconducting quantum processors. Our sub-second adaptive spectroscopy reveals telegraphic switching of TLSs with a characteristic timescale of a few seconds and spectral diffusion with diffusivity D≈0.9 MHz2/sD \approx 0.9~\mathrm{MHz}^2/\mathrm{s}D≈0.9 MHz2/s. These timescales are about 3×1023 \times 10^23×102 times faster than what is observed in conventional nonadaptive spectroscopy, which typically requires hours of measurement time. We resolve such fast dynamics on a field-programmable gate array (FPGA)-based controller that enables measurement of frequency- and time-resolved relaxations with sub-second temporal resolution in flux-tunable superconducting qubits. We observe similar defect dynamics across multiple qubits in independently fabricated devices measured in different laboratories. We correlate TLS-induced fluctuations with gate-level errors using randomized benchmarking. Our results reveal a previously inaccessible regime of frequency-resolved TLS dynamics and redefine the timescales relevant to TLS-aware characterization and calibration of superconducting quantum processors.