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arXiv:2602.11127

Two-Level System Spectroscopy from Correlated Multilevel Relaxation in Superconducting Qubits

Tanay Roy, Xinyuan You, David van Zanten, Francesco Crisa, Sabrina Garattoni, Shaojiang Zhu, Anna Grassellino, Alexander Romanenko

quant-phSubmitted Feb 11, 2026• Announced Feb 12, 2026• 0 citations
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Abstract

Transmon qubits are a cornerstone of modern superconducting quantum computing platforms. Temporal fluctuations of energy relaxation in these qubits are widely attributed to microscopic two-level systems (TLSs) in device dielectrics and interfaces, yet isolating individual defects typically relies on tuning the qubit or the TLS into resonance. We demonstrate a novel spectroscopy method for fixed-frequency transmons based on multilevel relaxation: repeated preparation of the second excited state and simultaneous $T_1$ extraction of the first and second excited states reveals characteristic correlations in the decay rates of adjacent transitions. From these correlations we identify one or more dominant TLSs and reconstruct their frequency drift over time. Remarkably, we find that TLSs detuned by $\gtrsim 100\,\mathrm{MHz}$ from the qubit transition can still significantly influence relaxation. The proposed method provides a powerful tool for TLS spectroscopy without the need to tune the transmon frequency, either via a flux-tunable inductor or AC-Stark shifts.

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4 pages, 3 figures

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Applied Sciences•May 30, 2023•1 citation
Transmon qubits are a cornerstone of modern superconducting quantum computing platforms. Temporal fluctuations of energy relaxation in these qubits are widely attributed to microscopic two-level systems (TLSs) in device dielectrics and interfaces, yet isolating individual defects typically relies on tuning the qubit or the TLS into resonance. We demonstrate a novel spectroscopy method for fixed-frequency transmons based on multilevel relaxation: repeated preparation of the second excited state and simultaneous T1T_1T1​ extraction of the first and second excited states reveals characteristic correlations in the decay rates of adjacent transitions. From these correlations we identify one or more dominant TLSs and reconstruct their frequency drift over time. Remarkably, we find that TLSs detuned by ≳100 MHz\gtrsim 100\,\mathrm{MHz}≳100MHz from the qubit transition can still significantly influence relaxation. The proposed method provides a powerful tool for TLS spectroscopy without the need to tune the transmon frequency, either via a flux-tunable inductor or AC-Stark shifts.
Materials improvements in transmon qubits have yielded remarkable advances in qubit lifetimes (T1)and coherence times (T2). However, state-of-the-art superconducting qubits experience temporal fluctuations in their performance, which limit gate fidelities and quantum processor performance. We observe correlated increases in qubit relaxation and dephasing rates that last for minutes to hours, which we call T1 and T2 excursions. Using interleaved lifetime and coherence time measurements, noise spectroscopy, and two-level-system (TLS) spectroscopy, we find that these excursions are caused by single or few strongly-coupled TLS defects that spectrally diffuse into resonance with the qubit frequency. Our measurement protocol provides a powerful tool for understanding the noise sources that cause temporal fluctuations in superconducting qubit performance.
An outstanding challenge in superconducting quantum circuits is mitigating loss from two-level system (TLS) defects. SWAP spectroscopy with flux-tunable qubits can detect individual TLSs, but the Rabi chevrons that signal coherent exchange have been observed only for the most strongly coupled defects. Here, we introduce a sequence with fast flux pulses only at state preparation and readout, switched off during the energy-relaxation delay for finer frequency resolution and longer interaction times. We detect Rabi chevrons at swap rates as low as 0.1 MHz, an order of magnitude lower than previously reported. In the dressed-state picture, we fit the coherent swap oscillations to extract the TLS energy-relaxation time. These Rabi chevrons reveal coherent TLSs with a median energy-relaxation time of 10 microseconds, at coupling strengths previously associated with incoherent TLSs. The swap coherence times exceed the qubit T2* limited by flux noise, indicating that the dressed gap protects them from low-frequency 1/f noise.
Abstract Superconducting qubits are a leading candidate for quantum computing but display temporal fluctuations in their energy relaxation times T 1 . This introduces instabilities in multi-qubit device performance. Furthermore, autocorrelation in these time fluctuations introduces challenges for obtaining representative measures of T 1 for process optimization and device screening. These T 1 fluctuations are often attributed to time varying coupling of the qubit to defects, putative two level systems (TLSs). In this work, we develop a technique to probe the spectral and temporal dynamics of T 1 in single junction transmons by repeated T 1 measurements in the frequency vicinity of the bare qubit transition, via the AC-Stark effect. Across 10 qubits, we observe strong correlations between the mean T 1 averaged over approximately nine months and a snapshot of an equally weighted T 1 average over the Stark shifted frequency range. These observations are suggestive of an ergodic-like spectral diffusion of TLSs dominating T 1 , and offer a promising path to more rapid T 1 characterization for device screening and process optimization.
Understanding the microscopic environment of superconducting qubits is a central challenge for quantum technologies. Parasitic two-level systems (TLSs) of various microscopic origins are ubiquitous and limit qubit performance through decoherence, frequency drifts, and leakage. Recently, long-lived TLSs with lifetimes exceeding those of state-of-the-art qubits have been shown to induce correlated qubit dynamics, with direct implications for quantum error correction. Here, we perform wide-band quantum-jump correlation spectroscopy on flux-tunable transmon qubits and identify microscopic degrees of freedom that outlive the qubit by orders of magnitude. Pump-probe measurements at varying detunings from these objects reveal intrinsic lifetimes exceeding one second. Their weak coupling to the qubit, in the kilohertz range, is consistent with positional defects described by the standard tunneling model, without excluding other microscopic origins such as magnetic spin impurities or trapped quasiparticles. More broadly, these results establish superconducting qubits as a sensitive probe of exceptionally long-lived microscopic degrees of freedom and open a route toward their controlled access and functionalization.
Parasitic two-level-system (TLS) defects are a major source of energy relaxation and temporal instability in superconducting quantum processors. Our sub-second adaptive spectroscopy reveals telegraphic switching of TLSs with a characteristic timescale of a few seconds and spectral diffusion with diffusivity D≈0.9 MHz2/sD \approx 0.9~\mathrm{MHz}^2/\mathrm{s}D≈0.9 MHz2/s. These timescales are about 3×1023 \times 10^23×102 times faster than what is observed in conventional nonadaptive spectroscopy, which typically requires hours of measurement time. We resolve such fast dynamics on a field-programmable gate array (FPGA)-based controller that enables measurement of frequency- and time-resolved relaxations with sub-second temporal resolution in flux-tunable superconducting qubits. We observe similar defect dynamics across multiple qubits in independently fabricated devices measured in different laboratories. We correlate TLS-induced fluctuations with gate-level errors using randomized benchmarking. Our results reveal a previously inaccessible regime of frequency-resolved TLS dynamics and redefine the timescales relevant to TLS-aware characterization and calibration of superconducting quantum processors.
One significant source of decoherence in superconducting circuits is known as two-level systems (TLSs), found in amorphous oxide layers. These circuits can, however, also be utilized as spectral and temporal TLS probes. Comprehensive investigations on the physics of TLSs are now possible thanks to recent advancements in superconducting qubits. Here, we simultaneously measure the tunable Xmon qubit decoherence time as well as the resonance frequency for more than 3 days to investigate stochastic fluctuations. Time-domain Allan deviation and frequency-domain power spectral density analysis indicate that two TLSs in near resonance with the qubit are responsible for the fluctuations. From the extracted oscillation in T1 decay, we locate the two TLSs near the junctions.