The amplification of quantum information carried by a single quantum excitation is a recurring challenge across diverse quantum platforms. The coupling between a single qubit and a mesoscopic ensemble of spins, for example, can be leveraged to realize non-destructive detection of the qubit state. However, realizing robust couplings between such systems is experimentally challenging and typically requires programmable quantum gates or native long-range interactions. Here, we introduce a platform that couples a single qubit, encoded in the ground-to-Rydberg transition of a control atom, to a Rydberg-dressed target ensemble of ground-state atoms trapped in an optical lattice. We show that the state of the control qubit can be coherently mapped onto the ensemble via a qubit-controlled collective phase shift. By Rydberg-dressing the ensemble, the controlled phase shift per target atom becomes independent of the number of target atoms, making the protocol intrinsically insensitive to atom-number fluctuations and atom loss, which are the dominant experimental imperfections in our system. Exploiting the collective response of up to eight target spins, we demonstrate the efficacy of the scheme by realizing non-destructive detection of a single Rydberg excitation with a state-assignment fidelity of $\mathcal{F} = 99.81^{+0.17}_{-1.47}\,\%$. Our approach demonstrates the key ingredients for high-fidelity transfer of quantum information from a single qubit to a mesoscopic ensemble, opening a route to non-destructive mid-circuit readout of Rydberg states and to efficient interfaces between single qubits and photonic modes.
The amplification of quantum information carried by a single quantum excitation is a recurring challenge across diverse quantum platforms. The coupling between a single qubit and a mesoscopic ensemble of spins, for example, can be leveraged to realize non-destructive detection of the qubit state. However, realizing robust couplings between such systems is experimentally challenging and typically requires programmable quantum gates or native long-range interactions. Here, we introduce a platform that couples a single qubit, encoded in the ground-to-Rydberg transition of a control atom, to a Rydberg-dressed target ensemble of ground-state atoms trapped in an optical lattice. We show that the state of the control qubit can be coherently mapped onto the ensemble via a qubit-controlled collective phase shift. By Rydberg-dressing the ensemble, the controlled phase shift per target atom becomes independent of the number of target atoms, making the protocol intrinsically insensitive to atom-number fluctuations and atom loss, which are the dominant experimental imperfections in our system. Exploiting the collective response of up to eight target spins, we demonstrate the efficacy of the scheme by realizing non-destructive detection of a single Rydberg excitation with a state-assignment fidelity of F=99.81−1.47+0.17%. Our approach demonstrates the key ingredients for high-fidelity transfer of quantum information from a single qubit to a mesoscopic ensemble, opening a route to non-destructive mid-circuit readout of Rydberg states and to efficient interfaces between single qubits and photonic modes.
Scalable quantum computers and quantum networks require the combination of quantum processing nodes with efficient light-matter interfaces to distribute quantum information in local or long-distance quantum networks. Neutral-atom arrays have both been coupled to Rydberg states to enable high-fidelity quantum gates in universal processing architectures, and to optical cavities to realize interfaces to photons. However, combining these two capabilities and coupling atom arrays to highly excited Rydberg states in the mode of an optical cavity has been an outstanding challenge. Here we present a novel cavity-coupled Rydberg array that achieves this long-standing goal. We prepare, detect, and control individual atoms in a scalable optical tweezer array, couple them strongly to the optical mode of a high-finesse optical cavity and excite them in a controlled way to Rydberg states. We show that high-cooperativity coupling to an optical cavity -- demonstrated via the dispersive shift of the resonance of the cavity in presence of the atoms -- and strong Rydberg interactions -- demonstrated via the collective enhancement of Rydberg coupling in the atomic array -- can be achieved in our setup at the same spatial location. Our presented experimental platform opens the path to several new directions, including the realization of quantum network nodes, quantum simulation of long-range interacting, open quantum systems and photonic-state engineering leveraging high-fidelity Rydberg control.
This thesis reports progress towards using hyperfine-encoded neutral atomic ensembles for quantum information applications. Ensemble qubits are alternative building blocks to process quantum information, while circumventing the challenges preparing a low-entropy single-atom qubit register. While ensemble approach inherits the single-atom quantum gate protocols, cooperative atom-light interaction makes it favorable platform to implement atom-photon interface, such as quantum memory. We have demonstrated semi-deterministic preparation of W-state, which we use as an ensemble qubit. Observed 50–60% preparation fidelity shows discrepancy to expected > 80% fidelity including known imperfections. We suspect Ground-Rydberg and Rydberg-Rydberg molecular interactions within the ensemble modify the dynamics. State tomography and Ramsey experiment clearly identified that majority of constituents in an ensemble are indeed entangled. We report the first measurement of W-state coherence time as 2.6ms for 7.6 atoms, which is long enough to perform 2600 Rydberg-mediated quantum gate operations. The first demonstration of Rydberg blockade between two ensembles happened in the same apparatus. We observe blockade fidelity of 0.89 (uncorrected) and near unity when post-selected on successful N = 1 Fock state preparation of Control ensemble. For weakly blockaded cases, Target ensemble remained as a perturber inhibiting Control ensemble from de-excitation. We discuss the efficacy of optical lattice insertion to suppress molecular interactions that might have been affecting the Rydberg dynamics. High fidelity, parallel, low loss fluorescence detection of hyperfine ground state of rubidium atoms is presented. Enforced cycling transition scattering minimally alters the internal states. We achieve mean state detection fidelity of 97% (uncorrected) and 98.7% (SPAM error corrected), with atom loss rate < 2% and hyperfine-changing rate < 2%. This scalable technique is also compatible with ensemble qubits and error correcting schemes. Technical developments on apparatus, lasers, supporting hardware and software are discussed. Automatic beam alignment system is implemented to correct long term drift of tightly focused addressing beams. Achieved pointing stability of 60 nm. Two home-made, high performing, cavity-enhanced frequency doubling systems were constructed to meet experimental demand. We observe 960/480 system output as high as 180 mW with 600 mW fundamental, and 1540/770 system output as high as 13.97 W from 19 W fundamental.
The dipole blockade of multiple Rydberg excitations in mesoscopic atomic ensembles allows the implementation of various quantum information tasks using collective states of cold, trapped atoms. Precise coherent manipulations of the collective ground and single Rydberg excitation states of an atomic ensemble requires the knowledge of the number of atoms with small uncertainty. We present an efficient method to acquire such information by interrogating the atomic ensemble with resonant pulses while monitoring the resulting Rydberg excitations. We show that after several such steps accompanied by feedback the number of atoms in an ensemble can be assessed with high accuracy. This will facilitate the realization of high-fidelity quantum gates, long-term storage of quantum information, and deterministic sources of single photons with Rydberg-blockaded atomic ensembles.
Integrating Rydberg-state control of atom-atom interactions with cavity control of atom-light interactions enables the combination of local entangling operations with photon-mediated long-range coupling, measurement, and communication. Such integration is challenging because electric fields generated by charges on cavity optics and by cavity-stabilizing actuators may disturb Rydberg-state coherence. Here, we couple a Rydberg tweezer array to a high-cooperativity optical cavity, suppressing the electric fields produced by cavity length actuation so that the residual field variation of about 3mV/cm rms does not limit Rydberg coherence. We demonstrate two capabilities that neither system provides alone. First, we use Purcell-enhanced fluorescence to read out atoms directly in the ground-Rydberg basis within 7.5μs, well within the Rydberg-state lifetime, with ground- and Rydberg-state detection infidelities of 3% and 5%, respectively, and with low atom loss. Second, we use Rydberg-Rydberg interactions to control collective light-atom scattering into the cavity mode. Specifically, we drive blockaded Rabi oscillations between a state with two ground-state atoms, which scatter collectively with a superradiant or subradiant rate controlled by the atomic positions, and an entangled state with a single Rydberg excitation, which scatters like a single atom. These capabilities open routes toward networked Rydberg processors, mid-circuit measurements in analog quantum simulators, and many-body quantum optics with entangled emitters coupled collectively to light.
With the advent of laser cooling and trapping, neutral atoms have become a foundational source of accuracy for applications in metrology and are showing great potential for their use as qubits in quantum information. In metrology, neutral atoms provide the most accurate references for the measurement of time and acceleration. The unsurpassed stability provided by these systems make neutral atoms an attractive avenue to explore applications in quantum information and computing. However, to fully investigate the field of quantum information, we require a method to generate entangling interactions between neutral-atom qubits. Recent progress in the use of highly-excited Rydberg states for strong dipolar interactions has shown great promise for controlled entanglement using the Rydberg blockade phenomenon. I report the use of singly-trapped cesium atoms as qubits for applications in metrology and quantum information. Each atom provides a physical basis for a single qubit by encoding the required information into the ground-state hyperfine structure of cesium. Through the manipulation of these qubits with microwave and optical frequency sources, we demonstrate the capacity for arbitrary single-qubit control by driving qubit rotations in three orthogonal directions on the Bloch sphere. With this control, we develop an atom interferometer that far surpasses the force sensitivity of other approaches by applying the well-established technique of light-pulsed atom-matterwave interferometry to single atoms. Following this, we focus on two-qubit interactions using highly-excited Rydberg states. Through the development of a unique single-photon approach to Rydberg excitation using an ultraviolet laser at 319 nm, we observe the Rydberg blockade interaction between atoms separated by 6.6(3) microns. Motivated by the observation of Rydberg blockade, we study the application of Rydberg-dressed states for a quantum controlled-phase gate. Using a realistic simulation of the dressed-state dynamics, we calculate a controlled-phase gate fidelity of 94% that is primarily limited by Doppler frequency shifts. Finally, we employ our single-photon excitation laser to measure the Rydberg-dressed interaction, thus demonstrating the viability of this approach.
In any physical platform, two ingredients are essential for quantum information processing: single-qubit control, and entangling interactions between qubits. Neutral atoms can be individually controlled with high fidelity and are resilient to environmental noise, making them attractive candidates for implementing quantum information protocols. However, achieving strong interactions remains a major obstacle. One way to increase the interaction strength between neutral atoms is to excite them into high-lying Rydberg states, which exhibit large electric dipole moments (and by extension, strong electric dipole-dipole interactions). By slowly ramping up the Rydberg level coupling in a system, one can "dress'' the atomic ground states with some Rydberg character; this maps the Rydberg dipole interaction to an effective interaction between ground states. Such Rydberg-dressed interaction is the focus of this dissertation. After describing the physics of the Rydberg-dressed interaction, we propose three protocols that demonstrate its versatility and provide a framework for considering some of the details of realistic implementation. In all three cases, Rydberg dressing --- along with some form of single-atom control --- is used to generate highly entangled states of interest. Our first proposal relates to the adiabatic model of quantum computing, in which solutions to problems are encoded in the ground states of carefully engineered Hamiltonians. The Rydberg-dressed interaction can provide nonlinear Hamiltonian terms, allowing us to encode NP-hard and other interesting problems. We model this protocol in the presence of decoherence, and find that computational fidelities of ~0.98 for four atoms should be possible with currently realistic experimental parameters. Our second proposal is also related to quantum computing, this time in the circuit model. The Rydberg-dressed interaction can be used to generate a controlled-NOT logic gate which, when interwoven with single-qubit gates, can perform universal quantum computation. Experimentally, noise due to atomic thermal motion has been a primary limitation on the fidelities of these gates. We show that a Doppler-free setup, with counterpropagating lasers, effectively suppresses this type of noise, allowing simulated fidelities of up to ~0.998 per gate. Such strong suppression is only possible because the Doppler-free configuration can harness the natural robustness of adiabatic dressing; other gate schemes using, e.g., resonant pulses, do not exhibit the same degree of improvement. Finally, we consider exploiting the many-body character of the Rydberg-dressed interaction to generate collective entanglement in mesoscopic ensembles of neutral atoms. An atomic ensemble uniformly illuminated by a single Rydberg-exciting laser is isomorphic to the well-known Jaynes-Cummings model. In addition to adapting generic Jaynes-Cummings entanglement protocols developed in other platforms, one can apply microwaves to drive entanglement in a way that is unique to the atomic platform. We prove that by allowing the microwave phase to vary in time, one can generate arbitrary symmetric states of the ensemble. While this method compares favorably with other entanglement protocols in many ways, the required frequency of phase switching presents a fundamental limitation on its effectiveness. To mitigate this, we propose a variant scheme in which parameters are chosen to only allow excitations within the system's dressed-ground subspace; this effectively cuts phase switching demands in half. All three protocols serve to illustrate the power of the Rydberg-dressed interaction and suggest directions for future study.