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arXiv:2608.06160

Simulation of positronium laser cooling using the Lindblad master equation

Kenji Shu, Sohma Shiraishi, Kosuke Yoshioka

Published Aug 6, 2026• 0 citations
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Abstract

We present a formulation and numerical results for positronium (Ps) laser cooling. The formulation is based on the Lindblad master equation and follows the time evolution of the density matrix of Ps atoms. It therefore accounts for atomic coherence, which is necessary to describe the interaction of Ps with the train of short laser pulses generated by the system developed by Shu $\textit{et al.}$ [K. Shu $\textit{et al.}$, Phys. Rev. A $\textbf{109}$, 043520 (2024)]. Using this formulation, we calculate the time evolution of the populations in each internal and momentum state and thereby quantitatively predict the momentum distribution after laser cooling. We present the representative time evolution of the internal-state populations and momentum distribution, together with a comprehensive scan of the laser parameters used to optimize the cooling efficiency. A prominent feature of the simulated distributions is sub-recoil cooling through velocity-selective coherent population trapping, a coherent effect captured by the quantum-mechanical treatment.

DOI
10.48550/arxiv.2608.06160

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We present a formulation and numerical results for positronium (Ps) laser cooling. The formulation is based on the Lindblad master equation and follows the time evolution of the density matrix of Ps atoms. It therefore accounts for atomic coherence, which is necessary to describe the interaction of Ps with the train of short laser pulses generated by the system developed by Shu et al.\textit{et al.}et al. [K. Shu et al.\textit{et al.}et al., Phys. Rev. A 109\textbf{109}109, 043520 (2024)]. Using this formulation, we calculate the time evolution of the populations in each internal and momentum state and thereby quantitatively predict the momentum distribution after laser cooling. We present the representative time evolution of the internal-state populations and momentum distribution, together with a comprehensive scan of the laser parameters used to optimize the cooling efficiency. A prominent feature of the simulated distributions is sub-recoil cooling through velocity-selective coherent population trapping, a coherent effect captured by the quantum-mechanical treatment.
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We propose to extend coherent laser cooling from narrowband to broadband transitions by using trains of ultrashort broadband pulses. We analytically study two possible methods to reduce the momentum spread of a distribution by several units of photon momentum in a single spontaneous emission lifetime. We report on numerical simulations of one-dimensional laser cooling of a two-level system with realistic parameters. With this scheme, coherent laser cooling can in particular be implemented in the case of fast species with a short lifetime such as positronium.
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We present a fully quantum-mechanical analysis of laser cooling of an angular momentum Jg{\mathit{J}}_{\mathit{g}}Jg​=1 to Je{\mathit{J}}_{\mathit{e}}Je​=1 transition in a laser configuration consisting of two counterpropagating linearly polarized laser beams. The essential feature of this configuration is the coexistence of velocity-selective coherent population trapping (VSCPT) and polarization-gradient cooling. The role of polarization-gradient cooling is to provide (i) for short interaction times ``precooling'' of the initial momentum distribution and (ii) in the long-time limit ``confinement of velocities.'' This eventually leads to a larger number of atoms being captured in the dark state when compared with the schme of Aspect et al. [Phys. Rev. Lett. 61, 826 (1988)]. We find that the optimum parameter values for polarization-gradient cooling and VSCPT are in a completely different parameter regime: polarization-gradient cooling works best off resonance and for low intensities, while VSCPT works best on resonance. We can combine the advantages of polarization-gradient cooling and VSCPT in a scheme where we cycle in time between the optimum cooling parameters for both cooling mechanisms.
One-dimensional laser cooling based on velocity-selective coherent population trapping (VSCPT) has been investigated numerically through the solution of the optical Bloch equations and through a Monte Carlo analysis. The 1\ensuremath{\rightarrow}1 and 2\ensuremath{\rightarrow}2 transitions have been examined as a function of the atomic recoil frequency, the spontaneous-emission decay rate, and the Rabi frequency of the cooling laser. It has been found that for a large set of those parameters, the VSCPT cooling process may be described through scaling-law relations. The scaling laws are not valid at long atom-laser interaction times or large Rabi frequencies, where the atomic Doppler shift plays a significant role in the atomic motion evolution. Similar results for two atomic transitions suggest the validity of the scaling law for any one-dimensional VSCPT process. \textcopyright{} 1996 The American Physical Society.