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arXiv:2608.05426

Qutrit entanglement and joint multi-parameter estimation in an optical clock platform

Ohad Lib, Shuheng Liu, Maximilian Ammenwerth, Hendrik Timme, Shijia Sun, Qiongyi He, Marcus Huber, Giuseppe Vitagliano, Immanuel Bloch, Johannes Zeiher

quant-phSubmitted Aug 5, 2026• Announced Aug 7, 2026• 0 citations
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Abstract

Quantum metrology harnesses entanglement to improve measurement precision beyond classical limits. While standard protocols rely on two-level qubits to estimate a single parameter, extending them to entangled multi-level qudits enables the optimal simultaneous estimation of multiple parameters within a single probe. However, generating such multi-level entanglement and harnessing it for joint multi-parameter estimation in atomic clocks has remained an outstanding challenge. Here, we experimentally demonstrate genuine qutrit entanglement and joint multi-parameter estimation in an optical clock platform. Leveraging control over the ground state and two fine-structure clock states of $^{88}\text{Sr}$ atoms trapped in triple-magic optical tweezers, we generate a maximally entangled two-qutrit state with a loss-postselected fidelity of F = 0.85(1), certifying genuine multi-level entanglement. Taking advantage of this high-dimensional entanglement, we theoretically construct and experimentally realize an optimal two-qutrit metrological probe state and noise-robust readout circuit to simultaneously estimate injected phases on two optical clock transitions. We observe a joint estimation variance below the ideal individual two-level sensing threshold, and show theoretically that this advantage persists at state-of-the-art atom numbers under circuit-level noise. These results demonstrate the key building blocks towards quantum information science with high-dimensional states encoded in the internal energy levels of neutral atoms.

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Quantum metrology harnesses entanglement to improve measurement precision beyond classical limits. While standard protocols rely on two-level qubits to estimate a single parameter, extending them to entangled multi-level qudits enables the optimal simultaneous estimation of multiple parameters within a single probe. However, generating such multi-level entanglement and harnessing it for joint multi-parameter estimation in atomic clocks has remained an outstanding challenge. Here, we experimentally demonstrate genuine qutrit entanglement and joint multi-parameter estimation in an optical clock platform. Leveraging control over the ground state and two fine-structure clock states of 88Sr^{88}\text{Sr}88Sr atoms trapped in triple-magic optical tweezers, we generate a maximally entangled two-qutrit state with a loss-postselected fidelity of F = 0.85(1), certifying genuine multi-level entanglement. Taking advantage of this high-dimensional entanglement, we theoretically construct and experimentally realize an optimal two-qutrit metrological probe state and noise-robust readout circuit to simultaneously estimate injected phases on two optical clock transitions. We observe a joint estimation variance below the ideal individual two-level sensing threshold, and show theoretically that this advantage persists at state-of-the-art atom numbers under circuit-level noise. These results demonstrate the key building blocks towards quantum information science with high-dimensional states encoded in the internal energy levels of neutral atoms.
The optical clock states of alkaline earth and alkaline earthlike atoms are the fundament of state-of-the-art optical atomic clocks. An important prerequisite for the operation of optical clocks is the magic trapping conditions where electronic and motional dynamics decouple. Here, we identify and experimentally demonstrate simultaneous magic trapping for two clock transitions in ^{88}Sr, realizing so-called triple-magic conditions at a specially chosen magic angle. Under these conditions, we operate an all-optical qutrit comprising the ground state ^{1}S_{0}, and the two metastable clock states ^{3}P_{0} and ^{3}P_{2}. We demonstrate fast optical control in an atom array using two- and three-photon couplings to realize high-fidelity manipulation between all qutrit states. At the magic angle, we probe the coherence achievable in magic-angle-tuned traps and find atom-atom coherence times between the metastable states as long as 715(30) ms. Our work opens several new directions, including qutrit-based quantum metrology on optical transitions and high-fidelity and high-coherence manipulation on the ^{88}Sr fine-structure qubit.
The optical clock states of alkaline earth and alkaline earthlike atoms are the fundament of state-of-theart optical atomic clocks.An important prerequisite for the operation of optical clocks is the magic trapping conditions where electronic and motional dynamics decouple.Here, we identify and experimentally demonstrate simultaneous magic trapping for two clock transitions in 88 Sr, realizing so-called triple-magic conditions at a specially chosen magic angle.Under these conditions, we operate an all-optical qutrit comprising the ground state 1 S 0 , and the two metastable clock states 3 P 0 and 3 P 2 .We demonstrate fast optical control in an atom array using two-and three-photon couplings to realize high-fidelity manipulation between all qutrit states.At the magic angle, we probe the coherence achievable in magic-angle-tuned traps and find atom-atom coherence times between the metastable states as long as 715(30) ms.Our work opens several new directions, including qutrit-based quantum metrology on optical transitions and high-fidelity and high-coherence manipulation on the 88 Sr fine-structure qubit.
Building scalable quantum systems that demonstrate genuine performance enhancement based on entanglement is a major scientific goal for fields including computing, networking, simulations, and metrology. The tremendous challenge arises from the fragility of entanglement in increasingly larger sized quantum systems. Optical atomic clocks utilizing a large number of atoms have pushed the frontier of measurement science, building on precise engineering of quantum states and control of atomic interactions. However, today's state-of-the-art optical atomic clocks are limited by the quantum projection noise (QPN) defined by many uncorrelated atoms. Pioneering work on producing spin squeezed states of atoms has shown a path towards integrating entanglement into the best performing clocks. However, to directly demonstrate advantage of quantum entanglement in a working clock we must prevent backaction effects that degrade quantum coherence and introduce uncontrolled perturbations, as well as minimize the influence of technical noise arising from the interrogating clock laser. Here we present a new optical clock platform integrated with collective strong-coupling cavity QED for quantum non-demolition (QND) measurement. Optimizing the competition between spin measurement precision and loss of coherence, we measure a Wineland parameter of -1.8(7) dB for 1.9x104^44 atoms, thus verifying the presence of entanglement. Furthermore, a moving lattice allows the cavity to individually address two independent sub-ensembles, enabling us to spin squeeze two clock ensembles successively and compare their performance. This differential comparison between the two squeezed clocks directly verifies enhanced clock stability of 2.0(3) dB below QPN, and 0.6(3) dB above the standard quantum limit (SQL), at the measurement precision level of 10−17^{-17}−17, without subtracting any technical noise contributions.
Quantum-enhanced sensing with atomic ensembles has predominantly focused on qubit-based protocols, despite the growing ability of many experimental platforms to coherently control and entangle multi-level systems. Here, we investigate quantum-enhanced sensing with qutrit ensembles by introducing three experimentally feasible qutrit generalisations of the one-axis twisting (OAT) model that involve entangling operations only between two levels, while the third level primarily acts as a spectator. We characterize the metrological utility of the dynamically generated states using the quantum Fisher information toolbox. We find numerically that all three models offer considerable freedom in encoding direction for quantum-enhanced sensing, with up to 6 out of 8 possible directions exhibit near-Heisenberg scaling after a short evolution time. We discuss experimental access to this enhanced metrological precision via effective time-reversal protocols. Furthermore, we examine the practical issues of estimation ambiguity and local dissipation, and show that they can be largely overcome by optimizing the sensor operating point. Finally, we show that the measurement incompatibility in estimating multiple parameters simultaneously encoded in different directions with near-Heisenberg scaling of precision is suppressed at the zero operating point as the system size increases. In the process, we find that one of the models enables near-Heisenberg scaling metrology with a pair of commuting generators, a possibility that arises from the su(3)su(3)su(3) algebra and is thus absent in qubit-ensemble based sensors of collective SU(2)SU(2)SU(2) rotations.
In quantum metrology, entangled states of many-particle systems are investigated to enhance measurement precision of the most precise clocks and field sensors. Whereas single-parameter quantum metrology is well established, joint multiparameter estimation poses conceptual challenges and has been explored only theoretically. We experimentally demonstrated multiparameter quantum metrology with an array of entangled atomic ensembles. By splitting a spin-squeezed ensemble, we created an atomic sensor array featuring intersensor entanglement that can be flexibly configured to enhance measurement precision of multiple parameters jointly. Using an optimal estimation protocol, we achieved substantial gains over the standard quantum limit in key multiparameter estimation tasks, thus grounding the concept of quantum enhancement of field sensor arrays and imaging devices.
Entanglement is a fundamental feature of quantum mechanics and holds great promise for enhancing metrology and communications. Much of the focus of quantum metrology so far has been on generating highly entangled quantum states that offer better sensitivity, per resource, than what can be achieved classically. However, to reach the ultimate limits in multi-parameter quantum metrology and quantum information processing tasks, collective measurements, which generate entanglement between multiple copies of the quantum state, are necessary. Here, we experimentally demonstrate theoretically optimal single- and two-copy collective measurements for simultaneously estimating two non-commuting qubit rotations. This allows us to implement quantum-enhanced sensing, for which the metrological gain persists for high levels of decoherence, and to draw fundamental insights about the interpretation of the uncertainty principle. We implement our optimal measurements on superconducting, trapped-ion and photonic systems, providing an indication of how future quantum-enhanced sensing networks may look.