Quantum emitters coupled to nonlinear one-dimensional waveguides provide a route for quantum-state engineering by utilizing parametric gain accumulation along with modified waveguide-mediated interactions. Since the accumulated squeezing depends on propagation distance, different emitter separations can experience different effective gain, making the spatial structure of connected quantum correlations a central feature of the dynamics. Here we investigate the transient and steady-state connected correlations of emitter arrays coupled to a parametrically driven waveguide. Using an effective master equation for nonlinear waveguide QED, we analyze second- and third-order connected correlations as functions of the squeezing parameter and interparticle distance. In the two-emitter limit, accumulated squeezing drives excitation buildup and generates a nonzero connected second-order correlation. For many-emitter arrays, tuning the interparticle distance switches the dominant local second-order correlation between the bulk and boundary regions, and enables an analogous spatial control of genuine third-order connected correlations. In the steady state, the averaged second-order correlation exhibits sign-changing and nonmonotonic behavior in the squeezing--interparticle distance parameter space, whereas the third-order connected correlation is strongly enhanced by increasing the squeezing parameter. These results identify nonlinear waveguide QED as a tunable platform for spatially controlling connected quantum correlations and provide insights into correlation engineering in open quantum optical arrays. We further show that this local contrast remains visible in both odd and even number of atomic arrays.
Quantum emitters coupled to nonlinear one-dimensional waveguides provide a route for quantum-state engineering by utilizing parametric gain accumulation along with modified waveguide-mediated interactions. Since the accumulated squeezing depends on propagation distance, different emitter separations can experience different effective gain, making the spatial structure of connected quantum correlations a central feature of the dynamics. Here we investigate the transient and steady-state connected correlations of emitter arrays coupled to a parametrically driven waveguide. Using an effective master equation for nonlinear waveguide QED, we analyze second- and third-order connected correlations as functions of the squeezing parameter and interparticle distance. In the two-emitter limit, accumulated squeezing drives excitation buildup and generates a nonzero connected second-order correlation. For many-emitter arrays, tuning the interparticle distance switches the dominant local second-order correlation between the bulk and boundary regions, and enables an analogous spatial control of genuine third-order connected correlations. In the steady state, the averaged second-order correlation exhibits sign-changing and nonmonotonic behavior in the squeezing--interparticle distance parameter space, whereas the third-order connected correlation is strongly enhanced by increasing the squeezing parameter. These results identify nonlinear waveguide QED as a tunable platform for spatially controlling connected quantum correlations and provide insights into correlation engineering in open quantum optical arrays. We further show that this local contrast remains visible in both odd and even number of atomic arrays.
Enhancing interactions in many-body quantum systems, while protecting them from environmental decoherence, is at the heart of many quantum technologies. Waveguide quantum electrodynamics is a promising platform for achieving this, as it hosts infinite-range interactions and decoherence-free subspaces of quantum emitters. However, as coherent interactions between emitters are typically washed out in the wavelength-spacing regime hosting decoherence-free states, coherent control over the latter becomes limited, and many-body Hamiltonians in this important regime remain out of reach. Here we show that by incorporating emitter arrays with nonlinear waveguides hosting parametric gain, we obtain a unique class of many-body interaction Hamiltonians with coupling strengths that increase with emitter spacing, and persist even for wavelength-spaced arrays. We then propose to use these Hamiltonians to coherently generate decoherence-free states directly from the ground state, using only global squeezing drives, without the need for local addressing of individual emitters. Interestingly, we find that the dynamics approaches a unitary evolution in the limit of weak intrawaveguide squeezing, and we discuss potential experimental realizations of this effect. Our results pave the way towards coherent control protocols in waveguide quantum electrodynamics, with applications including quantum computing, simulation, memory, and nonclassical light generation.
The scattering between light and individual saturable quantum emitters can induce strong optical nonlinearities and correlations between individual light quanta. Typically, this leads to an effective attraction that can generate exotic bound states of photons, which form quantum mechanical precursors of optical solitons, as found in many optical media. Here, we study the propagation of light through an optical waveguide that is chirally coupled to three-level quantum emitters. We show that the additional laser coupling to a third emitter state not only enables control of the properties of the bound state but can even eliminate it entirely. This makes it possible to turn an otherwise focusing nonlinearity into a repulsive photon-photon interaction. We demonstrate this emerging photon-photon repulsion by analyzing the quantum dynamics of multiple photons in large emitter arrays and reveal a dynamical fragmentation of incident uncorrelated light fields and self-ordering into regular trains of single photons. These striking effects expand the rich physics of waveguide quantum electrodynamics into the domain of repulsive photons and establish a conceptually simple platform to explore optical self-organization phenomena at the quantum level. We discuss implementations of this setting in cold-atom experiments and propose an approach based on arrays of mesoscopic Rydberg-atom ensembles.
Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions leads to strong correlations of photons arising in transmission, as shown in recent experiments. Here we apply an improved mean-field theory based on higher-order cumulant expansions to describe the experimentally relevant, but theoretically elusive, regime of weak coupling and strong driving of large ensembles. We determine the transmitted power, squeezing spectra and the degree of second-order coherence, and systematically check the convergence of the results by comparing expansions that truncate cumulants of few-particle correlations at increasing order. This reveals the important role of many-body and long-range correlations between atoms in steady state. Our approach allows to quantify the trade-off between anti-bunching and output power in previously inaccessible parameter regimes. Calculated squeezing spectra show good agreement with measured data, as we present here.
Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.
Waveguide QED with cold atoms provides a potent platform for the study of non-equilibrium, many-body, and open-system quantum dynamics. Even with weak coupling and strong photon loss, the collective enhancement of light-atom interactions leads to strong correlations of photons arising in transmission, as shown in recent experiments. Here we apply an improved mean-field theory based on higher-order cumulant expansions to describe the experimentally relevant, but theoretically elusive, regime of weak coupling and strong driving of large ensembles. We determine the transmitted power, squeezing spectra and the degree of second-order coherence, and systematically check the convergence of the results by comparing expansions that truncate cumulants of few-particle correlations at increasing order. This reveals the important role of many-body and long-range correlations between atoms in steady state. Our approach allows to quantify the trade-off between anti-bunching and output power in previously inaccessible parameter regimes. Calculated squeezing spectra show good agreement with measured data, as we present here.
Parametric amplification offers a powerful means to enhance quantum interactions through field squeezing, yet it typically introduces additional noise which accelerates quantum decoherence, a major obstacle for scalable quantum information processing. The squeezing field is implemented in cavities rather than continuous waveguides, thereby limiting its scalability for applications in quantum simulation. Giant atoms, which couple to waveguides at multiple points, provide a promising route to mitigate dissipation via engineered interference, enabling decoherence-free interactions. We extend the squeezing-amplified interaction to a novel quantum platform combining giant atoms with traveling-wave parametric waveguides based on χ(2) nonlinearity. By exploiting destructive interference between different coupling points, the interaction between giant atoms is not only significantly enhanced but also becomes immune to squeezed noise. Unlike conventional waveguide quantum electrodynamics without a squeezing pump, the giant emitters exhibit both exchange and pairing interactions, making this platform particularly suitable for simulating many-body quantum physics. More intriguingly, the strengths of these interactions can be smoothly tuned by adjusting the squeezing and coupling parameters. Our architecture thus provides a versatile and scalable platform for quantum simulation of strongly correlated physics and paves the way toward robust quantum control in many-body regimes.