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arXiv:2405.20241 · Physical Review Research

Decoherence-free many-body Hamiltonians in nonlinear waveguide quantum electrodynamics

Aviv Karnieli, Offek Tziperman, Charles Roques‐Carmes, Shanhui Fan

Published Jan 21, 2025• 6 citations
arXivHTMLPDF

Abstract

Enhancing interactions in many-body quantum systems, while protecting them from environmental decoherence, is at the heart of many quantum technologies. Waveguide quantum electrodynamics is a promising platform for achieving this, as it hosts infinite-range interactions and decoherence-free subspaces of quantum emitters. However, as coherent interactions between emitters are typically washed out in the wavelength-spacing regime hosting decoherence-free states, coherent control over the latter becomes limited, and many-body Hamiltonians in this important regime remain out of reach. Here we show that by incorporating emitter arrays with nonlinear waveguides hosting parametric gain, we obtain a unique class of many-body interaction Hamiltonians with coupling strengths that increase with emitter spacing, and persist even for wavelength-spaced arrays. We then propose to use these Hamiltonians to coherently generate decoherence-free states directly from the ground state, using only global squeezing drives, without the need for local addressing of individual emitters. Interestingly, we find that the dynamics approaches a unitary evolution in the limit of weak intrawaveguide squeezing, and we discuss potential experimental realizations of this effect. Our results pave the way towards coherent control protocols in waveguide quantum electrodynamics, with applications including quantum computing, simulation, memory, and nonclassical light generation.

DOI
10.1103/physrevresearch.7.l012014

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Parametric amplification offers a powerful means to enhance quantum interactions through field squeezing, yet it typically introduces additional noise which accelerates quantum decoherence, a major obstacle for scalable quantum information processing. The squeezing field is implemented in cavities rather than continuous waveguides, thereby limiting its scalability for applications in quantum simulation. Giant atoms, which couple to waveguides at multiple points, provide a promising route to mitigate dissipation via engineered interference, enabling decoherence-free interactions. We extend the squeezing-amplified interaction to a novel quantum platform combining giant atoms with traveling-wave parametric waveguides based on χ(2)χ^{(2)}χ(2) nonlinearity. By exploiting destructive interference between different coupling points, the interaction between giant atoms is not only significantly enhanced but also becomes immune to squeezed noise. Unlike conventional waveguide quantum electrodynamics without a squeezing pump, the giant emitters exhibit both exchange and pairing interactions, making this platform particularly suitable for simulating many-body quantum physics. More intriguingly, the strengths of these interactions can be smoothly tuned by adjusting the squeezing and coupling parameters. Our architecture thus provides a versatile and scalable platform for quantum simulation of strongly correlated physics and paves the way toward robust quantum control in many-body regimes.
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Waveguide quantum electrodynamics (QED) studies the interaction between quantum emitters and guided photons in one dimension. When the waveguide hosts interacting photons, it becomes a platform to explore many-body quantum optics. However, the influence of photonic correlations on emitter dynamics remains poorly understood. In this work, we study the collective decay and coherent interactions of quantum emitters coupled to a one-dimensional Bose-Hubbard waveguide, an array of coupled photonic modes with repulsive on-site interactions that supports superfluid and Mott insulating phases. We show that photon-photon interactions alone can trigger a superradiant burst, independent of emitter spacing and transition frequency. In the off-resonant regime, emitters exhibit two distinct types of mediated interactions. Delocalized superfluid excitations yield persistent, long-range couplings, challenging the noninteracting paradigm, where long-range (dissipative) couplings occur in band, whereas short-range and coherent interactions occur in a bandgap. In the Mott limit, quasiparticles generate short-range interactions mediated by doublons and holons. Our work bridges many-body physics and waveguide QED, revealing how photonic many-body states shape emitter dynamics.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.