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arXiv:2607.13296

Unveiling Structured Optical Coherence in Nonlinear Optics

Zihao Pang, Ady Arie

Published Jul 14, 2026• 0 citations
arXivHTMLPDF

Abstract

Nonlinear optical interactions are typically driven by coherent sources. Recently, however, incoherent sources have also been shown to offer new opportunities in nonlinear optics. Here we study the effects of the source incoherence in second harmonic generation. We derive and experimentally validate an analytic expression for the far-field coherence function at the second harmonic frequency, which is a generalization of the well-known van Cittert-Zernike theorem. Unlike the linear optics case, here the results depend not only on the source spatial distribution, but also on the nonlinear structure of the crystal. We further show, by performing Young's double-slit measurement, that the coherence at the second harmonic increases as the light propagates inside the nonlinear crystal. Our results establish nonlinearity as a degree of freedom for optical coherence, opening a new research area at the interface of statistical optics and nonlinear optics.

DOI
10.48550/arxiv.2607.13296

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Nonlinear optical interactions are typically driven by coherent sources. Recently, however, incoherent sources have also been shown to offer new opportunities in nonlinear optics. Here we study the effects of the source incoherence in second harmonic generation. We derive and experimentally validate an analytic expression for the far-field coherence function at the second harmonic frequency, which is a generalization of the well-known van Cittert-Zernike theorem. Unlike the linear optics case, here the results depend not only on the source spatial distribution, but also on the nonlinear structure of the crystal. We further show, by performing Young's double-slit measurement, that the coherence at the second harmonic increases as the light propagates inside the nonlinear crystal. Our results establish nonlinearity as a degree of freedom for optical coherence, opening a new research area at the interface of statistical optics and nonlinear optics.
Nonlinear frequency conversion has traditionally relied on highly coherent light sources. This assumption has deeply shaped the field, yet it overlooks the broader role that spatial incoherence can play in nonlinear optics. In this work, we break that paradigm by demonstrating, for the first time, that second harmonic generation (SHG) can be performed with spatially incoherent light, and more importantly, that the spatial coherence of the generated second harmonic field can be customized with precision. Our work unlocks spatial coherence as an active and designable parameter in nonlinear optics.
Abstract Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising photon statistics modifications. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence.
The effect of the quantum properties of light on nonlinear processes has been well studied theoretically. It has been shown that the efficiency of n-photon nonlinear processes in many cases scales as the normalized n-th order correlation function. For light with high intensity correlation function, the efficiency of the n-th harmonic generation will be considerably higher than for coherent light. The experimental observation of this effect remained difficult until recently, because of the absence of bright sources with strong and fast intensity fluctuations. For the experimental demonstration of statistical effects in optical harmonic generation we use as a pump the radiation of high-gain parametric down conversion. Such light shows quantum properties (e.g. quadrature or two-mode squeezing) and has large number of photons in one mode. The normalized n-th order correlation function for this light is (2n - 1)!!, which makes it more attractive for nonlinear processes than both coherent and thermal light. For the generation of optical harmonics we used broadband parametric down conversion around frequency-degeneracy (1600 nm) produced in 1cm BBO crystal from Ti:Sapphire laser (800 nm, 1.6ps, 5kHz, 3W mean intensity). Due to spectral filtering and post-selection technique we could vary the statistics of light from coherent to super-bunched, which allowed us to demonstrate the efficiency enhancement for second-, third-, and fourth-harmonic generation. The obtained experimental results show a good agreement with the theory.
Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires of nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising classical-to-quantum transitions. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect had not been discussed before and cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence.
In this Letter, we study the second-harmonic (SH) generation of temporally low-coherence light using the statistical optics method. By introducing the statistical characteristics of low-coherence light into the nonlinear coupled wave equation, we predict the self-convolution relationship between the power spectral density of the second-harmonic and that of the fundamental wave and demonstrate it in experiments. The effects of phase matching and group velocity matching on the second-harmonic bandwidth and conversion efficiency are analyzed, which is beneficial to improve the efficiency of low-coherent SH light. Combining the statistics optics and nonlinear optics, our research provides a suitable mathematical model for the study of nonlinear frequency conversion processes of temporally low-coherence light. Due to its statistical characteristics and temporal incoherence, low-coherence SH light would have further applications in uniform illumination, quantum optics, metrology, and so on.
Recent advances in quantum optics have highlighted the critical role of spatial propagation in controlling the quantum coherence of light beams. However, the evolution of quantum coherence for light beams undergoing fundamental optical processes at dielectric interfaces remains unexplored. Furthermore, manipulating multiphoton correlations typically requires complex interactions that challenge few-photon level implementation. Here, we introduce a quantum van Cittert-Zernike theorem for light beams, describing how their coherence-polarization properties are influenced by reflection and refraction, as well as how these properties evolve upon subsequent propagation. Our work demonstrates that the quantum statistics of photonic systems can be controllably modified through the inherent polarization coupling arising from reflection and refraction at an interface, without relying on conventional light-matter interactions. Our approach reveals regimes where thermal light can exhibit sub-Poissonian statistics with fluctuations below the shot-noise level through post-selected measurements, and this statistical property can be tuned by the incident angle. Remarkably, this quantum statistical modification is governed by a scaling law linking beam collimation to far-field thermalization. Our work establishes a robust, decoherence-avoiding mechanism for quantum state control, advancing the fundamental understanding of coherence in quantum optics and opening new avenues for applications in quantum information and metrology.