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npj Quantum Information

Multiphoton quantum van Cittert-Zernike theorem

Chenglong You, Ashe Miller, Roberto de J. León‐Montiel, Omar S. Magaña‐Loaiza

Published May 26, 2023• 12 citations
Publisher

Abstract

Abstract Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising photon statistics modifications. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence.

DOI
10.1038/s41534-023-00720-w

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Abstract Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising photon statistics modifications. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence.
Recent progress on quantum state engineering has enabled the preparation of quantum photonic systems comprising multiple interacting particles. Interestingly, multiphoton quantum systems can host many complex forms of interference and scattering processes that are essential to perform operations that are intractable on classical systems. Unfortunately, the quantum coherence properties of multiphoton systems degrade upon propagation leading to undesired quantum-to-classical transitions. Furthermore, the manipulation of multiphoton quantum systems requires of nonlinear interactions at the few-photon level. Here, we introduce the quantum van Cittert-Zernike theorem to describe the scattering and interference effects of propagating multiphoton systems. This fundamental theorem demonstrates that the quantum statistical fluctuations, which define the nature of diverse light sources, can be modified upon propagation in the absence of light-matter interactions. The generality of our formalism unveils the conditions under which the evolution of multiphoton systems can lead to surprising classical-to-quantum transitions. Specifically, we show that the implementation of conditional measurements may enable the all-optical preparation of multiphoton systems with attenuated quantum statistics below the shot-noise limit. Remarkably, this effect had not been discussed before and cannot be explained through the classical theory of optical coherence. As such, our work opens new paradigms within the established field of quantum coherence.
Recent advances in quantum optics have highlighted the critical role of spatial propagation in controlling the quantum coherence of light beams. However, the evolution of quantum coherence for light beams undergoing fundamental optical processes at dielectric interfaces remains unexplored. Furthermore, manipulating multiphoton correlations typically requires complex interactions that challenge few-photon level implementation. Here, we introduce a quantum van Cittert-Zernike theorem for light beams, describing how their coherence-polarization properties are influenced by reflection and refraction, as well as how these properties evolve upon subsequent propagation. Our work demonstrates that the quantum statistics of photonic systems can be controllably modified through the inherent polarization coupling arising from reflection and refraction at an interface, without relying on conventional light-matter interactions. Our approach reveals regimes where thermal light can exhibit sub-Poissonian statistics with fluctuations below the shot-noise level through post-selected measurements, and this statistical property can be tuned by the incident angle. Remarkably, this quantum statistical modification is governed by a scaling law linking beam collimation to far-field thermalization. Our work establishes a robust, decoherence-avoiding mechanism for quantum state control, advancing the fundamental understanding of coherence in quantum optics and opening new avenues for applications in quantum information and metrology.
The modification of the quantum properties of coherence of photons through their interaction with matter lies at the heart of the quantum theory of light. Indeed, the absorption and emission of photons by atoms can lead to different kinds of light with characteristic quantum statistical properties. As such, different types of light are typically associated with distinct sources. Here, we report on the observation of the modification of quantum coherence of multiphoton systems in free space. This surprising effect is produced by the scattering of thermal multiphoton wavepackets upon propagation. The modification of the excitation mode of a photonic system and its associated quantum fluctuations result in the formation of different light fields with distinct quantum coherence properties. Remarkably, we show that these processes of scattering can lead to multiphoton systems with subshot-noise quantum properties. Our observations are validated through the nonclassical formulation of the emblematic van Cittert–Zernike theorem. We believe that the possibility of producing quantum systems with modified properties of coherence, through linear propagation, can have dramatic implications for diverse quantum technologies.
Currently, optical technology impacts most of our lives, from light used in scientific measurement to the fiber optic cables that makeup the backbone of the internet. However, as our current optical infrastructure grows, we discover that these technologies are not limitless. However, our current optical technology functions on classical principles, and can be easily improved by incorporating our knowledge of quantum optics. In order to implement quantum technologies, our understanding of quantum coherence must improve. Through this knowledge we can maintain quantum states, and therefore their information, longer. In this dissertation, I will demonstrate that with sufficient knowledge of coherent properties, a simple algebra can be derived which can provide rules for graph reductions on a quantum network graph. Using this knowledge, I then provide a rudimentary algorithm which can find the optimal subgraph for communication on a quantum network. Next, I demonstrate that by measuring the photon statistics and second-order quantum coherence of a field, one can create a neural network capable of distinguishing the light sources on a pixel. Which is then applied to develop an imaging scheme capable of surpassing the Abbe-Rayleigh Criterion. Lastly, I present a multiphoton quantum version of the van Cittert-Zernike theorem. This provides formalism capable of determining the propagation of quantum coherence throughout a system. I then demonstrate the usefulness of the theorem by demonstrating sub-Poissonian statistics created by a linear system with an incident thermal beam, obtainable only by post-selection. Altogether, this provides incite into new applications of coherence to quantum technologies and the formalism to extending our knowledge even further.
Abstract The quantum theory of electromagnetic radiation predicts characteristic statistical fluctuations for light sources as diverse as sunlight, laser radiation, and molecule fluorescence. Indeed, these underlying statistical fluctuations of light are associated with the fundamental physical processes behind their generation. In this contribution, we experimentally demonstrate that the manipulation of the quantum electromagnetic fluctuations of two-mode squeezed vacuum states leads to a family of quantum-correlated multiphoton states with tunable mean photon numbers and degree of correlation. Our technique relies on the use of conditional measurements to engineer the excitation mode of the field through the simultaneous subtraction of photons from two-mode squeezed vacuum states. The experimental generation of nonclassical multiphoton states by means of photon subtraction unveils novel mechanisms to control fundamental properties of light. As a remarkable example, we demonstrate the engineering of a quantum state of light with up to ten photons, exhibiting nearly Poissonian photon statistics, that constitutes an important step towards the generation of entangled lasers. Our technique enables a robust protocol to prepare quantum states with multiple photons in high-dimensional spaces and, as such, it constitutes a novel platform for exploring quantum phenomena in mesoscopic systems.