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arXiv:2607.07546

An analytical solution of a quantum system with non-Markovian behavior: The Bixon-Jortner system in time domain

Osman Cevheroğlu, Arkadaş Özakın

quant-phSubmitted Jul 8, 2026• Announced Jul 9, 2026• 0 citations• Revised Oct 30, 2026 (v2)
v1 · Jul 8, 2026v2 · Oct 30, 2026
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Abstract

Non-Markovian behavior in quantum systems is often studied in the context of bipartite systems consisting of a system of interest and an environment -- tracing over the environment results in non-Markovian behavior for the subsystem of interest. One may get a Markovian limit in certain regimes, which is studied using the Lindblad master equation, and corrections to this behavior can be obtained by techniques such as the Nakajima-Zwanzig formalism. In this paper, we obtain an exact non-Markovian equation for the dynamics of a simple model system that consists of a direct sum rather than a tensor product of two pieces, namely, a discrete state and an infinite ladder. This system, called the Bixon-Jortner model, was first developed in the quantum chemistry literature but has been utilized by the quantum optics community as a model system with interesting behavior, including a Wigner-Weisskopf limit of exponential decay. We attack the time evolution problem of this system directly in time-domain, and start with an integrodifferential equation describing the time evolution of the discrete state. Using tools from mathematical physics, we transform this equation to a delay differential equation, which makes the non-Markovianity completely transparent, and then we solve the delay equation using an intuitive ansatz. This allows us to obtain the analytic form of the dynamics directly in time domain, and demonstrate decay and revival behaviors coming from the aforementioned delay differential equation. We believe the explicit form of the time-domain non-Markovian equation we obtain and the accessibility the solution techniques we use make our results a useful case study of non-Markovianity in quantum systems.

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Non-Markovian behavior in quantum systems is often studied in the context of bipartite systems consisting of a system of interest and an environment -- tracing over the environment results in non-Markovian behavior for the subsystem of interest. One may get a Markovian limit in certain regimes, which is studied using the Lindblad master equation, and corrections to this behavior can be obtained by techniques such as the Nakajima-Zwanzig formalism. In this paper, we obtain an exact non-Markovian equation for the dynamics of a simple model system that consists of a direct sum rather than a tensor product of two pieces, namely, a discrete state and an infinite ladder. This system, called the Bixon-Jortner model, was first developed in the quantum chemistry literature but has been utilized by the quantum optics community as a model system with interesting behavior, including a Wigner-Weisskopf limit of exponential decay. We attack the time evolution problem of this system directly in time-domain, and start with an integrodifferential equation describing the time evolution of the discrete state. Using tools from mathematical physics, we transform this equation to a delay differential equation, which makes the non-Markovianity completely transparent, and then we solve the delay equation using an intuitive ansatz. This allows us to obtain the analytic form of the dynamics directly in time domain, and demonstrate decay and revival behaviors coming from the aforementioned delay differential equation. We believe the explicit form of the time-domain non-Markovian equation we obtain and the accessibility the solution techniques we use make our results a useful case study of non-Markovianity in quantum systems.
The subject of this thesis is the modelling of non-Markovian open quantum systems, in particular those that display memory effects due to time-delayed interactions. I study these systems in the context of a model of an open quantum system that interacts with a bosonic environment by way of particle exchanges. While the model is flexible enough to describe quite general memory effects, this work focuses to a large extent on a single prototypical system. This system emits into a coherent feedback loop with a time delay, and it captures the essential phenomena we aim to model. Within the context of this general model, I develop a general approach to spontaneous emission from singly-excited systems and show how to calculate the corresponding emission spectra. I also evaluate two commonly-used perturbative techniques in the context of spontaneous emission from singly-excited systems, coming to the conclusion that perturbation theory is of limited use in modelling open quantum systems with delayed feedback. I then turn attention to exact equations of motion for more general non-Markovian open quantum systems. I derive Heisenberg–Langevin equations that describe a large class of such systems, and solve these equations analytically for a series of simple bosonic systems. I also use the theory of cascaded open quantum systems to simulate systems with delayed coherent feedback in the limit of long time delay, and compare the results of these simulations with the analytic solutions obtained in the Heisenberg picture. Finally, I show that once we have a solution to a given Heisenberg–Langevin equation we can derive an alternative, time-local equation of motion that describes equivalent dynamics, and that these time-local Heisenberg–Langevin equations can in turn be used to derive corresponding time-local master equations. These master equations provide an exact description of the non-Markovian dynamics, but this treatment is limited to linear, bosonic systems—those systems for which the Heisenberg–Langevin equations can be solved in closed form. I discuss the prospect of generalising these master equations to take into account nonlinear and fermionic systems.
We study the decoherence properties of an entangled bipartite qubit system, represented by two two-level atoms that are individually coupled to non-Markovian reservoirs. This coupling ensures that the dynamical equations of the atoms can be treated independently. The non-Markovian reservoirs are described by a model which leads to an exact non-Markovian master equation of the Nakajima-Zwanzig form [J. Salo, S. M. Barnett, and S. Stenholm, Optics Commun. 259, 772 (2006)]. We consider the evolution of the entanglement of a two-atom state that is initially completely entangled, quantified by its concurrence. Collapses and revivals in the concurrence, induced by the memory effects of the reservoir, govern the dynamics of the entangled quantum system. These collapses and revivals in the concurrence are a strong manifestation of the non-Markovian reservoir.
The precise characterization of dynamics in open quantum systems often presents significant challenges, leading to the introduction of various approximations to simplify a model. One commonly used strategy involves Markovian approximations, assuming a memoryless environment. In this study, such approximations are not used and an analytical dynamical depiction of an open quantum system is provided. The system under consideration is an oscillator that is surrounded by a bath of oscillators. The resulting dynamics are characterized by an integrodifferential equation, which can be solved numerically. Remarkably, an exactly analytical solution exists when its reservoir spectral density is Lorentzian. Furthermore, this analytical solvability remains when rectangular pulse control is applied to the system, though with different parameters due to the pulses. Moreover, distinct dynamical regions emerge, depending on certain parameter values. Notably, the steady-state average excitation number (AEN) of the system shows rapid escalation with increasing non-Markovianity, reflecting the intricacies of real-world dynamics. In cases where there is detuning between the system frequency and the environmental central frequency within a non-Markovian regime, the AEN maintains its initial value for an extended period. Interestingly, the exact analytical solution with pulse control inherently protects the quantum system from decoherence effects without using approximations, while this protection fades as the system approaches the Markovian regime. The pulse control can not only prolong the relaxation time of the oscillator, but can also be used to speed up the relaxation process, depending on the specifications of the pulse.
An open quantum system is a quantum system that interacts with some environment whose degrees of freedom have been coarse grained away. This model describes non-equilibrium processes more general than scattering-matrix formulations. Furthermore, the microscopically-derived environment provides a model of noise, dissipation and decoherence far more general than Markovian (white noise) models. The latter are fully characterized by Lindblad equations and can be motivated phenomenologically. Non-Markovian processes consistently account for backreaction with the environment and can incorporate effects such as finite temperature and spatial correlations. We consider linear systems with bilinear coupling to the environment, or quantum Brownian motion, and nonlinear systems with weak coupling to the environment. For linear systems we provide exact solutions with analytical results for a variety of spectral densities. Furthermore, we point out an important mathematical subtlety which led to incorrect master-equation coefficients in earlier derivations, given nonlocal dissipation. For nonlinear systems we provide perturbative solutions by translating the formalism of canonical perturbation theory into the context of master equations. It is shown that unavoidable degeneracy causes an unfortunate reduction in accuracy between perturbative master equations and their solutions. We also extend the famous theorem of Lindblad, Gorini, Kossakowski and Sudarshan on completely positivity to non-Markovian master equations. Our application is primarily to model atoms interacting via a common electromagnetic field. The electromagnetic field contains correlations in both space and time, which are related to its relativistic (photon-mediated) nature. As such, atoms residing in the same field experience different environmental effects depending upon their relative position and orientation. Our more accurate solutions were necessary to assess sudden death of entanglement at zero temperature. In contrast to previous claims, we found that all initial states of two-level atoms undergo finite-time disentanglement. We were also able to access regimes which cannot be described by Lindblad equations and other simpler methods, such as near resonance. Finally we revisit the infamous Abraham-Lorentz force, wherein a single particle in motion experiences backreaction from the electromagnetic field. This leads to a number of well-known problems including pre-acceleration and runaway solutions. We found a more a more-suitable open-system treatment of the nonrelativistic particle to be perfectly causal and dissipative without any extraneous requirements for finite size of the particle, weak coupling to the field, etc..
We present a non-Markovian master equation for a qubit interacting with a general reservoir, which is derived according to the Nakajima—Zwanzig and the time convolutionless projection operator technique. The non-Markovian solutions and Markovian solution of dynamical decay of a qubit are compared. The results indicate the validity of non-Markovian approach in different coupling regimes and also show that the Markovian master equation may not precisely describe the dynamics of an open quantum system in some situation. The non-Markovian solutions may be effective for many qubits independently interacting with the heated reservoirs.
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